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The Asakura-Oosawa model for colloid-polymer mixtures is studied by Monte Carlo simulations at densities inside the two-phase coexistence region of fluid and solid. Choosing a geometry where the system is confined between two flat walls,…

Soft Condensed Matter · Physics 2015-06-04 Debabrata Deb , Alexander Winkler , Peter Virnau , Kurt Binder

One versatile route to the creation of two-dimensional crystal structures on the nanometer to micrometer scale is the self-assembly of colloidal particles at an interface. Here, we explore the crystal phases that can be expected from the…

Soft Condensed Matter · Physics 2020-05-29 Etienne Fayen , Anuradha Jagannathan , Giuseppe Foffi , Frank Smallenburg

A density functional of fundamental measure type for a lattice model of anisotropic particles with hard-core repulsions and effective attractions is derived in the spirit of the Asakura-Oosawa model. Through polymeric lattice particles of…

Soft Condensed Matter · Physics 2017-10-11 Mostafa Mortazavifar , Martin Oettel

We calculate for the first time the full phase-diagram of an asymmetric non-additive hard-sphere mixture. The non-additivity strongly affects the crystallization and the fluid-fluid phase-separation. The global topology of the phase-diagram…

Soft Condensed Matter · Physics 2009-10-31 A. A. Louis , R. Finken , J. P. Hansen

Within a second virial theory, we study bulk phase diagrams as well as the free planar isotropic-nematic interface of binary mixtures of nonadditive thin and thick hard rods. For species of the same type the excluded volume is determined…

Soft Condensed Matter · Physics 2009-11-10 K. Shundyak , R. van Roij , P. van der Schoot

Relaxation of the additivity condition on the interaction length between unlike species in a binary mixture of soft disks opens up a rich variety of structures in both crystal and amorphous states with an associated diverse range of…

Soft Condensed Matter · Physics 2014-02-17 Asaph Widmer-Cooper , Peter Harrowell

Using a fundamental measure density functional theory we investigate both bulk and inhomogeneous systems of the binary non-additive hard sphere model. For sufficiently large (positive) non-additivity the mixture phase separates into two…

Soft Condensed Matter · Physics 2010-07-30 Paul Hopkins , Matthias Schmidt

A fluid in equilibrium in a finite volume $V$ with particle number $N$ at a density $\rho = N/V$ exceeding the onset density $\rho_f $ of freezing may exhibit phase coexistence between a crystalline nucleus and surrounding fluid. Using a…

Statistical Mechanics · Physics 2015-06-23 Antonia Statt , Peter Virnau , Kurt Binder

We investigate the phase diagram of a two-component associating fluid mixture in the presence of selectively adsorbing substrates. The mixture is characterized by a bulk phase diagram which displays peculiar features such as closed loops of…

Statistical Mechanics · Physics 2009-11-07 J. M. Romero-Enrique , L. F. Rull , U. Marini Bettolo Marconi

We investigate the phase behavior of a single-component system in 3 dimensions with spherically-symmetric, pairwise-additive, soft-core interactions with an attractive well at a long distance, a repulsive soft-core shoulder at an…

Soft Condensed Matter · Physics 2009-11-07 G. Franzese , G. Malescio , A. Skibinsky , S. V. Buldyrev , H. E. Stanley

It is well known that the increase of the spatial dimensionality enhances the fluid-fluid demixing of a binary mixture of hard hyperspheres, i.e. the demixing occurs for lower mixture size asymmetry as compared to the three-dimensional…

Soft Condensed Matter · Physics 2015-05-19 Luis Lafuente , Yuri Martinez-Raton

A general class of nonadditive sticky-hard-sphere binary mixtures, where small and large spheres represent the solvent and the solute, respectively, is introduced. The solute-solute and solvent-solvent interactions are of hard-sphere type,…

Soft Condensed Matter · Physics 2015-06-16 Riccardo Fantoni , Achille Giacometti , Andrés Santos

While the realistically modeling of the thermodynamic behavior of fluids usually demands elaborated atomistic models, much have been learned from simplified ones. Here, we investigate a model where point-like particles (with activity $z_0$)…

Soft Condensed Matter · Physics 2019-07-15 Nathann T. Rodrigues , Tiago J. Oliveira

We report the grand-canonical solution of a ternary mixture of discrete hard spheres defined on a Husimi lattice built with cubes, which provides a mean-field approximation for this system on the cubic lattice. The mixture is composed by…

Soft Condensed Matter · Physics 2020-06-02 Nathann T. Rodrigues , Tiago J. Oliveira

Liquid crystals in two dimensions undergo a first-order isotropic-to-quasi-nematic transition, provided the particle interactions are sufficiently ``sharp and narrow''. This implies phase coexistence between isotropic and quasi-nematic…

Statistical Mechanics · Physics 2009-11-13 R. L. C. Vink

The possibility to induce demixing in a colloidal mixture by adding small polymers, or other equivalent depletant agents, is theoretically investigated. By use of Mean Field Theory, suitably generalized to deal with short range effective…

Soft Condensed Matter · Physics 2015-10-28 Alberto Parola , Luciano Reatto

We study the thermodynamic stability of fluid-fluid phase separation in binary nonadditive mixtures of hard-spheres for moderate size ratios. We are interested in elucidating the role played by small amounts of nonadditivity in determining…

Soft Condensed Matter · Physics 2011-10-25 G. Pellicane , F. Saija , C. Caccamo , P. V. Giaquinta

We present a scaled particle density functional study of two-dimensional binary mixtures of hard convex particles with one or both species being ellipses. In particular, we divide our study into two parts. The first part is devoted to the…

Soft Condensed Matter · Physics 2022-06-07 Yuri Martinez-Raton

Scaled particle theory for a binary mixture of hard discorectangles and for a binary mixture of hard rectangles is used to predict possible liquid-crystal demixing scenarios in two dimensions. Through a bifurcation analysis from the…

Soft Condensed Matter · Physics 2009-11-11 Yuri Martinez-Raton , Enrique Velasco , Luis Mederos

The phase-field-crystal model is used to access the structure and thermodynamics of interfaces between two coexisting liquid crystalline phases in two spatial dimensions. Depending on the model parameters there is a variety of possible…

Soft Condensed Matter · Physics 2014-01-28 Simon Praetorius , Axel Voigt , Raphael Wittkowski , Hartmut Löwen
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