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While 3$d$-containing materials display strong electron correlations, narrow band widths, and robust magnetism, 5$d$ systems are recognized for strong spin-orbit coupling, increased hybridization, and more diffuse orbitals. Combining these…

It has recently been demonstrated that dynamical magnetic correlations measured by neutron scattering in iron chalcogenides can be described with models of short-range correlations characterized by particular {choices of four-spin…

We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…

The parent compounds of iron-based superconductors are magnetically-ordered bad metals, with superconductivity appearing near a putative magnetic quantum critical point. The presence of both Hubbard repulsion and Hund's coupling leads to…

Parent compounds of Fe-based superconductors undergo a structural phase transition from a tetragonal to an orthorhombic structure. We investigated the temperature dependence of the frequencies of transverse acoustic (TA) phonons that…

Superconductivity · Physics 2015-05-13 D. Parshall , L. Pintschovius , D. Lamago , J. -P. Castellan , J. L. Niedziela , Th. Wolf , D. Reznik

We reported the quasiparticle relaxation dynamics of an optimally doped triclinic iron-based superconductor (Ca$_{0.85}$La$_{0.15}$)$_{10}$(Pt$_3$As$_8$)(Fe$_2$As$_2$)$_5$ with bulk $T_c$ = 30 K using polarized ultrafast optical pump-probe…

We review neutron scattering investigations of the crystal structures, magnetic structures, and spin dynamics of the iron-based RFe(As,P)O (R=La, Ce, Pr, Nd), (Ba,Sr,Ca)Fe2As2, and Fe1+x(Te-Se) systems. On cooling from room temperature all…

Superconductivity · Physics 2009-05-20 Jeffrey W. Lynn , Pengcheng Dai

Recently it has been suggested that the role of electron-phonon coupling in the mechanism of iron-based superconductors may have been underestimated and that the antiferromagnetism and the induced xy potential may even have a dramatic…

Superconductivity · Physics 2021-03-09 Chi Ho Wong , Rolf Lortz

We report here first extensive measurements of the temperature dependence of phonon density of states of BaFe2As2, the parent compound of the newly discovered FeAs-based superconductors, using inelastic neutron scattering. The experiments…

Superconductivity · Physics 2008-09-17 R. Mittal , Y. Su , S. Rols , T. Chatterji , S. L. Chaplot , H. Schober , M. Rotter , D. Johrendt , Th. Brueckel

Reproducing the electronic structure of AM$_4$X$_8$ lacunar spinels with a breathing pyrochlore lattice is a great theoretical challenge due to the interplay of various factors. The character of the M$_4$X$_4$ cluster orbitals is critically…

Strongly Correlated Electrons · Physics 2020-02-20 S. Reschke , F. Meggle , F. Mayr , V. Tsurkan , L. Prodan , H. Nakamura , J. Deisenhofer , C. A. Kuntscher , I. Kézsmárki

The iron-based high temperature superconductors exhibit a rich phase diagram reflecting a complex interplay between spin, lattice, and orbital degrees of freedom [1-4]. The nematic state observed in many of these compounds epitomizes this…

A family of molecular Mott insulators on triangular lattice provided a few S=1/2 triangular quantum spin liquid candidates, with $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ being the most studied material of this group. The large number…

Strongly Correlated Electrons · Physics 2024-10-08 Jesse Liebman , Kazuya Miyagawa , Kazushi Kanoda , Natalia Drichko

We investigate the spin dynamics in the superconducting phase of UTe$_{2}$ by triple-axis inelastic neutron scattering on a single crystal sample. At the wave-vector $\bf{k_1}$=(0, 0.57, 0), where the normal state antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-11-03 S. Raymond , W. Knafo , G. Knebel , K. Kaneko , J. -P. Brison , J. Flouquet , D. Aoki , G. Lapertot

We report an inelastic x-ray scattering investigation of phonons in FeSe superconductor. Comparing the experimental phonon dispersion with density functional theory (DFT) calculations in the non-magnetic state, we found a significant…

Inelastic neutron scattering measurements on the molecular dimer-Mott insulator $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl reveal a phonon anomaly in a wide temperature range. Starting from $T_{\rm ins}\sim50$-$60$ K where the charge gap…

We study the spin resonance peak in recently discovered iron-based superconductors. The resonance peak observed in inelastic neutron scattering experiments agrees well with predicted results for the extended $s$-wave ($s_\pm$) gap symmetry.…

Superconductivity · Physics 2016-08-09 M. M. Korshunov , Yu. N. Togushova , I. Eremin , P. J. Hirschfeld

We report a $^{75}$As nuclear magnetic resonance study in LaFeAsO single crystals, which undergoes nematic and antiferromagnetic transitions at $T_\text{nem}\sim 156$ K and $T_N \sim 138$ K, respectively. Below $T_\text{nem}$, the $^{75}$As…

Strongly Correlated Electrons · Physics 2018-05-30 J. M. Ok , S. -H. Baek , D. V. Efremov , R. Kappenberger , S. Aswartham , J. S. Kim , J. van den Brink , B. Büchner

We report the direct observation of a "resonance" mode in the lowest-energy optic phonon very near the zone center around (111) in the multiferroic BiFeO$_3$ using neutron scattering methods. The phonon scattering intensity is enhanced when…

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

Strongly Correlated Electrons · Physics 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

Mechanism of unconventional superconductivity in FeSe has been intensely scrutinized recently because of a variety of exotic properties unprecedented for other iron-based superconductors. A central unanswered question concerns the origin of…