Related papers: Probing dynamics in quantum materials with femtose…
The quantum vacuum constitutes a fascinating medium of study, in particular since near-future laser facilities will be able to probe the nonlinear nature of this vacuum. There has been a large number of proposed tests of the low-energy,…
The parallel or antiparallel arrangement of electron spins plays a pivotal role in determining the properties of a physical system. To meet the demands for innovative technological solutions, extensive efforts have been dedicated to…
We show that, in optical pump-probe experiments on bulk samples, the statistical distribution of the intensity of ultrashort light pulses after the interaction with a nonequilibrium complex material can be used to measure the time-dependent…
Over the last few years, tremendous progress has been gained in the generation and application of ultrashort radiation pulses. Recently, free-electron lasers generating ultrashort pulses with high peak power from the extreme ultraviolet…
We explore the novel capabilities offered by attosecond extreme ultraviolet and x-ray pulses that can be now generated by free-electron lasers and high-harmonics generation sources for probing photon-induced electron dynamics in molecules.…
Nonlinear processes lie at the heart of many technologies such as frequency converters and entangled photon sources. Historically, observation and manipulation of these processes, for instance through nanostructures, has been limited to…
We investigate the quantum dynamics of fermionic particles interacting with a laser field in a gaseous medium, in the regime of inelastic diffraction scattering on the phase lattice of a slowed travelling wave, below the critical field of…
Advancements in quantum optics and squeezed light generation have transformed various domains of quantum science and technology. However, real-time quantum dynamics remain an underexplored frontier. Here, we extend quantum optics into the…
The electron motion in atoms and molecules is at the heart of all phenomena in nature that occur outside the nucleus. Recently, ultrafast electron and X-ray imaging tools have been developed to image the ultrafast dynamics of matter in real…
The guiding and control of ultrahigh flux, femtosecond relativistic electron pulses through solid density matter is of great importance for many areas of high energy density science. Efforts so far include the use of magnetic fields…
Quantum materials are driving a technology revolution in sensing, communication, and computing, while simultaneously testing many core theories of the past century. Materials such as topological insulators, complex oxides, quantum dots,…
Ultra-intense lasers that ionize and accelerate electrons in solids to near the speed of light can lead to kinetic instabilities that alter the laser absorption and subsequent electron transport, isochoric heating, and ion acceleration.…
The quantum cascade laser (QCL) has evolved to be a compact, powerful source of coherent mid-infrared (mid-IR) light. However, its fast gain dynamics strongly restricts the formation of ultrashort pulses. As such, the shortest pulses…
Coherent control of ultrafast quantum phenomena benefits from pulse-shaping capabilities allowing to modulate the envelope and instantaneous phase of optical fields on femtosecond time scales. While such control is available for optical…
Non-equilibrium quantum matter generated by ultrafast laser light opens new pathways in fundamental condensed matter physics, as well as offering rich control possibilities in "tailoring matter by light". Here we explore the coupling…
Arbitrary manipulation of the temporal and spectral properties of X-ray pulses at free-electron lasers (FELs) would revolutionize many experimental applications. At the Linac Coherent Light Source at Stanford National Accelerator…
An intense femtosecond-laser excitation of a solid induces highly nonthermal conditions. In materials like silicon, laser-induced bond-softening leads to a highly incoherent ionic motion and eventually nonthermal melting. But is this…
Nonequilibrium electron dynamics in solids is an important subject from both fundamental and technological points of view. The recent development of laser technology has enabled us to study ultrafast electron dynamics in the time domain.…
Optomechanical systems provide a means for studying and controlling quantum effects in the motion of macroscopic objects. To date, quantum optomechanical effects have been studied in objects made from solids and gases. Here we describe…
Imaging the quantum motion of electrons not only in real-time, but also in real-space is essential to understand for example bond breaking and formation in molecules, and charge migration in peptides and biological systems. Time-resolved…