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Motivated by recent realizations of Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ spin ice thin films, and more generally by the physics of confined gauge fields, we study a model of spin ice thin film with surfaces perpendicular to…

Statistical Mechanics · Physics 2017-05-24 L. D. C. Jaubert , T. Lin , T. S. Opel , P. C. W. Holdsworth , M. J. P. Gingras

We carried out x-ray absorption spectroscopy (XAS) and x-ray magnetic circular dichroism (XMCD) spectroscopy and investigated cation valence states and spin and orbital magnetic moments in the inverse-spinel ferrimagnet…

CaFe2O4 is a highly anisotropic antiferromagnet reported to display two spin arrangements with up-up-down-down (phase A) and up-down-up-down (phase B) configurations. The relative stability of these phases is ruled by the competing…

Materials Science · Physics 2020-09-01 Silvia Damerio , Pavan Nukala , Jean Juraszek , Pim Reith , Hans Hilgenkamp , Beatriz Noheda

CoFe2O4 thin films (5 nm and 20 nm thick) were grown by oxygen assisted molecular beam epitaxy on Pt(111) at 523~K and subsequently annealed at 773 K in vacuum or oxygen. They were characterized in-situ using Auger Electron Spectroscopy,…

Materials Science · Physics 2022-02-28 G. D. Soria , K. Freindl , J. E. Prieto , A. Quesada , J. de la Figuera , N. Spiridis , J. Korecki , J. F. Marco

We report the synthesis of Ca$_2$RuO$_4$ thin films on NdCaAlO$_{4}$ (110), LaAlO$_3$ (100) and LaSrAlO$_4$ (001) substrates and show that epitaxial strain induces a transition from the Mott-insulating phase of bulk Ca$_2$RuO$_4$ into a…

Strongly Correlated Electrons · Physics 2018-01-18 C. Dietl , S. K. Sinha , G. Christiani , Y. Khaydukov , T. Keller , D. Putzky , S. Ibrahimkutty , P. Wochner , G. Logvenov , P. A. van Aken , B. J. Kim , B. Keimer

We report a magnetotransport study of spin relaxation in 1.4-21.2 nm epitaxial SrIrO$_3$ thin films coherently strained on SrTiO$_3$ substrates. Fully charge compensated semimetallic transport has been observed in SrIrO$_3$ films thicker…

Strongly Correlated Electrons · Physics 2020-06-16 L. Zhang , X. Jiang , X. Xu , X. Hong

Calcium vanadate CaV$_2$O$_4$ has a crystal structure of quasi-one-dimensional zigzag chains composed of orbital-active V$^{3+}$ ions and undergoes successive structural and antiferromagnetic phase transitions at $T_s\sim 140$ K and $T_N…

Strongly Correlated Electrons · Physics 2020-06-17 T. Watanabe , S. Kobayashi , Y. Hara , J. Xu , B. Lake , J. -Q. Yan , A. Niazi , D. C. Johnston

Despite the low resistivity (~ 1 mohm cm), the metallic electrical transport has not been commonly observed in the inverse spinel NiCo2O4, except in certain epitaxial thin films. Previous studies have stressed the effect of valence mixing…

Materials Science · Physics 2019-04-30 Congmian Zhen , XiaoZhe Zhang , Wengang Wei , Wenzhe Guo , Ankit Pant , Xiaoshan Xu , Jian Shen , Li Ma , Denglu Hou

Spin-orbit coupling and breaking of inversion symmetry are necessary ingredients to enable a pure spin current-based manipulation of the magnetization via the spin-orbit torque effect. Currently, magnetic insulator oxides with…

Recently, rutile RuO$_2$ has attracted renewed interest due to expectations of prominent altermagnetic spin-splitting. However, accumulating experimental evidence suggests that in its bulk and thick-film forms, RuO$_2$ does not display any…

The ferrimagnetic spinel oxide Zn(x)Fe(3-x)O(4) combines high Curie temperature and spin polarization with tunable electrical and magnetic properties, making it a promising functional material for spintronic devices. We have grown epitaxial…

CuAl2O4 is a normal spinel oxide having quantum spin, S=1/2 for Cu2+. It is a rather unique feature that the Cu2+ ions of CuAl2O4 sit at a tetrahedral position, not like the usual octahedral position for many oxides. At low temperatures, it…

We present a neutron diffraction study of FeV2O4, which is rare in exhibiting spin and orbital degrees of freedom on both cation sublattices of the spinel structure. Our data confirm the existence of three structural phase transitions…

Strongly Correlated Electrons · Physics 2012-09-03 G. J. MacDougall , V. O. Garlea , A. A. Aczel , H. D. Zhou , S. E. Nagler

A systematic study is performed on the spinel oxide, i.e. LiTi2O4 thin films oriented along [111]-, [110]-, and [001]-directions, to reveal the crystallographic dependence of transport properties. With decreasing temperature, the LiTi2O4…

Superconductivity · Physics 2016-08-25 Yanli Jia , Ge He , Heshan Yu , Wei Hu , Zhenzhong Yang , Jinan Shi , Zefeng Lin , Jie Yuan , Beiyi Zhu , Kai Liu , Lin Gu , Hong Li , Kui Jin

Hund's metallicity in 3$d$ transition metal oxides constitutes a rare class of compounds, since they have been long understood considering the dominance of Hubbard $U$. $\mathrm{LiV_2O_4}$\& $\mathrm{Sr_2CoO_4}$ belong to this rare class of…

Strongly Correlated Electrons · Physics 2025-10-07 Shivani Bhardwaj , Sudhir K. Pandey

We have grown thin films of the Heusler compound Co_2FeSi by RF magnetron sputtering. On (100)-oriented MgO substrates we find fully epitaxial (100)-oriented and L2_1 ordered growth. On Al_2O_3 (11-20) substrates, the film growth is…

Epitaxial thin films of LaCoO_{3} (E-LCO) exhibit ferromagnetic order with a transition temperature T_c = 85 K, while polycrystalline thin LaCoO_{3} films (P-LCO) remain paramagnetic. The temperature-dependent spin-state structure for both…

Strongly Correlated Electrons · Physics 2009-11-13 C. Pinta , D. Fuchs , M. Merz , M. Wissinger , E. Arac , A. Samartsev , P. Nagel , S. Schuppler

The large spin-orbit coupling in iridium oxides plays a significant role in driving novel physical behaviors, including emergent phenomena in the films and heterostructures of perovskite and Ruddlesden-Popper iridates. In this work, we…

Over the past few years, intensive studies of ultrathin epitaxial films of perovskite oxides have often revealed exciting properties like giant magnetoresistive tunnelling and electric field effects. Spinel oxides appear as even more…

$\gamma$-triclinic and $\alpha$-monoclinic polymorphs of CoV$_{2}$O$_{6}$ are two of the few known transition metal ion based materials that display stepped $1/3$ magnetization plateaus at low temperatures. Neutron diffraction [M. Markkula…

Strongly Correlated Electrons · Physics 2015-12-23 F. Wallington , A. M. Arevalo-Lopez , J. W. Taylor , J. R. Stewart , V. Garcia-Sakai , J. P. Attfield , C. Stock