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Colloidal quantum dots (QDs) are an attractive medium for nonlinear optics and deterministic heterogeneous integration with photonic devices. Their intrinsic nonlinearities can be strengthened further by coupling QDs to low mode-volume…
Optical properties of periodic arrays of nanoholes of a triangular shape with experimentally realizable parameters are examined in both linear and nonlinear regimes. Utilizing fully vectorial three-dimensional approach based on the…
We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is…
Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…
The emergence of strong-field nanoplasmonics brings extreme laser field-matter interaction into the realm of nanoscale science, unveiling exciting new physics. Highly nonlinear interaction is enabled by tightly confined electric fields in…
In this work, we utilize thin dielectric meta-atoms placed on a silver substrate to efficiently enhance and manipulate the third harmonic generation. We theoretically and experimentally reveal that when the structural symmetry of the…
Second harmonic generation (SHG) is a fundamental nonlinear optical phenomenon widely used both for experimental probes of materials and for application to optical devices. Even-order nonlinear optical responses including SHG generally…
Inspired by geometrically frustrated magnetic systems, we present the optical response of three cases of hexagonal lattices of plasmonic nanoelements. All of them were designed using a metal-insulator-metal configuration to enhance…
Optical nonlinearity, especially the second harmonic generation (SHG), is generally weak in materials but has the potential to be applied in high-speed optical computers and energy-efficient artificial intelligence systems. In order to…
Highly-tunable coherent light generation is crucial for many important photonic applications. Second-harmonic generation (SHG) is a dominant approach for this purpose, which, however, exhibits a trade-off between the conversion efficiency…
The 3D structure of light scattering from dark-field illuminated live 3T3 cells marked with 40 nm gold nanomarkers is explored. For this purpose, we use a high resolution holographic microscope combining the off-axis heterodyne geometry and…
We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and…
The architecture of novel metallic mesostructures obtained via self-organization of growing nanowires has been investigated. Seashell, fungus and lotus leafshaped structures are reproducibly formed by programmable pulse current…
We show that second harmonic generation can be enhanced by Fano resonant coupling of asymmetric plasmonic metal nanostructures. We develop a theoretical model examining the effects of electromagnetic interaction between two metal…
The pressure-induced metallic states of light elements attract significant attention, because of potential applications as high-temperature superconductor and high-energy-density material, especially for hydrogen and nitrogen1-10. Several…
The emerging two-dimensional (2D) materials exhibit a wide range of electronic properties, ranging from insulating hexagonal boron nitride, semiconducting transition metal dichalcogenides such as molybdenum disulfide, to semi-metallic…
Second harmonic generation (SHG) is a coherent nonlinear phenomenon that plays an important role in laser color conversion. Lithium niobate (LN), which features both a large band gap and outstanding second-order nonlinearities, acts as an…
Two dimensional transition metal dichalcogenides exhibit strong excitonic responses, direct bandgaps, and remarkable nonlinear optical properties, making them highly attractive for integrated photonic, optoelectronic, and quantum…
We show that a dimer made of two gold nanospheres exhibits a remarkable efficiency for second-harmonic generation under femtosecond optical excitation. The detectable nonlinear emission for the given particle size and excitation wavelength…
Optical second-harmonic generation (SHG) is studied for the confined geometry of a circular cylindrical waveguide or optical fiber. A model situation of high symmetry is considered where the material with nonlinear susceptibility is…