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We present a new theoretical approach to the study of second and third harmonic generation from metallic nanostructures and nanocavities filled with a nonlinear material, in the ultrashort pulse regime. We model the metal as a two-component…
Recent years have witnessed significant developments in the study of nonlinear properties of various optical materials at the nanoscale. However, in most cases experimental results on harmonic generation from nanostructured materials are…
High harmonic generation (HHG) in solids could enable attosecond and ultraviolet light sources with high compactness, great controllability and rich functions. However, the HHG process is accompanied by a quite large wavevector mismatch…
High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…
High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…
Significant effort has been expended in the search for materials with ultra-fast nonlinear-optical susceptibilities, but most fall far below the fundamental limits. This work applies a theoretical materials development program that has…
Plasmon resonances are known to amplify the electromagnetic fields near metallic nanostructures. Therefore, they are considered to provide a promising scheme to generate extreme-ultraviolet harmonics, using low power drivings. During…
Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…
Here we apply the optical nanocircuit concepts to design and analyze in detail a three-dimensional (3-D) plasmonic nanotransmission line network that may act as a negative-refraction broadband metamaterial at infrared and optical…
The random laser action with coherent feedback by second-harmonic generation (SHG) was experimentally demonstrated in this paper. Compared with the conventional random laser action based on photoluminescence effect, which needs strong…
Remarkable optical and electrical properties of two-dimensional (2D) materials, such as graphene and transition-metal dichalcogenide (TMDC) monolayers, offer vast technological potential for novel and improved optoelectronic nanodevices,…
Supraparticles are coordinated assemblies of discrete nanoscale building blocks into complex and hierarchical colloidal superstructures. Holistic optical responses in such assemblies are not observed in an individual building block or in…
We study nonlinear optical responses in superconducting systems with inversion ($\mathcal{I}$) symmetry-breaking order parameters. We first show that any superconducting system with $\mathcal{I}$ and time-reversal ($\mathcal{T}$) symmetries…
Plasmons facilitate a strong confinement and enhancement of near-field light, offering exciting opportunities to enhance nonlinear optical responses at the nanoscale. However, despite significant advancements, the electrically tunable range…
Second-order nonlinear optics is the base for a large variety of devices aimed at the active manipulation of light. However, physical principles restrict its occurrence to non-centrosymmetric, anisotropic matter. This significantly limits…
2D materials provide a platform for strong light--matter interactions, creating wide-ranging design opportunities via new-material discoveries and new methods for geometrical structuring. We derive general upper bounds to the strength of…
Hierarchical self-assembly arranges nanostructures at different length scales. It gradually becomes an effective method of fabricating artificial metamaterials from composite nanostructures tailored for a particular response. Hierarchical…
The second-order nonlinear optical (NLO) processes, such as the photogalvanic effect and second-order harmonic generation (SHG), play crucial roles in probing and controlling light-matter interactions for energy and device applications. To…
Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…
There is an active demand to develop efficient nanoscale nonlinear sources for applications in photonic circuitry, quantum optics and biosensing. To this end, plasmonic systems have been utilized to boost the nonlinear signal generation,…