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We discuss how to construct a tight binding model Hamiltonan for the simplest possible solid, composed of hydrogen-like atoms. A single orbital per atom is not sufficient because the on-site electron-electron repulsion mixes in higher…

Strongly Correlated Electrons · Physics 2014-09-09 J. E. Hirsch

We present a multigrid algorithm for self consistent solution of the Kohn-Sham equations in real space. The entire problem is discretized on a real space mesh with a high order finite difference representation. The resulting self consistent…

Materials Science · Physics 2009-10-31 Jian Wang , Thomas L. Beck

In numerical simulations of many charged systems at the micro/nano scale, a common theme is the repeated solution of the Poisson-Boltzmann equation. This task proves challenging, if not entirely infeasible, largely due to the nonlinearity…

Numerical Analysis · Mathematics 2018-08-29 Lijie Ji , Yanlai Chen , Zhenli Xu

We describe recent progress in developing practical ab initio methods for which the computer effort is proportional to the number of atoms: linear scaling or O(N) methods. It is shown that the locality property of the density matrix gives a…

Condensed Matter · Physics 2007-05-23 D. R. Bowler , I. J. Bush , M. J. Gillan

Accurate and fast calculations of localized surface plasmon resonances (LSPR) in metallic nanoparticles is essential for applications in sensing, nano-optics, and energy harvesting. Although full-wave numerical techniques such as the…

Accurately modeling the electronic structure of water across scales, from individual molecules to bulk liquid, remains a grand challenge. Traditional computational methods face a critical trade-off between computational cost and efficiency.…

Chemical Physics · Physics 2025-04-02 Xinyuan Liang , Renxi Liu , Mohan Chen

Three-dimensional charge density maps computed by first-principles methods provide information about atom positions and the bonds between them, data which is particularly valuable when trying to understand the properties of point defects,…

Materials Science · Physics 2008-10-22 Christoph T. Koch

This paper presents a numerical method for variable coefficient elliptic PDEs with mostly smooth solutions on two dimensional domains. The PDE is discretized via a multi-domain spectral collocation method of high local order (order 30 and…

Numerical Analysis · Mathematics 2016-12-09 Tracy Babb , Adrianna Gillman , Sijia Hao , Per-Gunnar Martinsson

We present a method to discretize the Kohn-Sham Hamiltonian matrix in the pseudopotential framework by a small set of basis functions automatically contracted from a uniform basis set such as planewaves. Each basis function is localized…

Computational Physics · Physics 2015-06-03 Lin Lin , Lexing Ying

A recently developed linear algebraic method for the computation of perturbation expansion coefficients to large order is applied to the problem of a hydrogenic atom in a magnetic field. We take as the zeroth order approximation the $D…

chem-ph · Physics 2009-10-22 Timothy C. Germann , Dudley R. Herschbach , Bruce M. Boghosian

Complex eigenvalues, resonances, play an important role in large variety of fields in physics and chemistry. For example, in cold molecular collision experiments and electron scattering experiments, autoionizing and pre-dissociative…

Quantum Physics · Physics 2016-09-28 Arie Landau , Idan Haritan , Petra Ruth Kaprálová-Žďánská , Nimrod Moiseyev

Evaluating the total energy of an extended distribution of point charges, which interact through the Coulomb potential, is central to the study of condensed matter. With near ubiquity, the summation required is carried out using Ewald's…

Materials Science · Physics 2018-01-24 Chris J. Pickard

An exact arithmetic, memory efficient direct solution method for finite element method (FEM) computations is outlined. Unlike conventional black-box or low-rank direct solvers that are opaque to the underlying physical problem, the proposed…

Computational Engineering, Finance, and Science · Computer Science 2020-02-13 Javad Moshfegh , Marinos N. Vouvakis

We consider a finite element method for elliptic equation with heterogeneous and possibly high-contrast coefficients based on primal hybrid formulation. A space decomposition as in FETI and BDCC allows a sequential computations of the…

Numerical Analysis · Mathematics 2024-04-29 Alexandre L. Madureira , Marcus Sarkis

We present a subspace projection technique to conduct large-scale Kohn-Sham density functional theory calculations using spectral finite-element discretization. The proposed method treats both metallic and insulating materials in a single…

Computational Physics · Physics 2015-10-26 Phani Motamarri , Vikram Gavini

We introduce a discontinuous Galerkin method for the mixed formulation of the elasticity eigenproblem with reduced symmetry. The analysis of the resulting discrete eigenproblem does not fit in the standard spectral approximation framework…

Numerical Analysis · Mathematics 2018-01-29 Felipe Lepe , Salim Meddahi , David Mora , Rodolfo Rodríguez

Discrete gradient methods are a powerful tool for the time discretization of dynamical systems, since they are structure-preserving regardless of the form of the total energy. In this work, we discuss the application of discrete gradient…

Numerical Analysis · Mathematics 2026-01-06 Philipp L. Kinon , Riccardo Morandin , Philipp Schulze

Modern multi-core systems have a large number of design parameters, most of which are discrete-valued, and this number is likely to keep increasing as chip complexity rises. Further, the accurate evaluation of a potential design choice is…

Distributed, Parallel, and Cluster Computing · Computer Science 2015-07-15 Neha V. Karanjkar , Madhav P. Desai

Nucleon-deuteron ($Nd$) scattering can be used to constrain three-nucleon forces in chiral effective field theory ($\chi$EFT). However, high-fidelity calculations, such as the Hyperspherical Harmonic (HH) method, are computationally…

The rapid development of ab initio nuclear structure methods towards doubly open-shell nuclei, heavy nuclei and greater accuracy occurs at the price of evermore increased computational costs, especially RAM and CPU time. While most of the…

Nuclear Theory · Physics 2026-01-19 Alberto Scalesi , Thomas Duguet , Mikael Frosini , Vittorio Somà