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We present a density functional theory study of the low-temperature structural, magnetic, and proposed charge-quadrupolar ordering in the double perovskite, Ba$_2$MgReO$_6$. Ba$_2$MgReO$_6$ is a spin-orbit-driven Mott insulator with a…

Materials Science · Physics 2025-07-22 Aria Mansouri Tehrani , Nicola A. Spaldin

Based on density functional theory calculations and group theoretical analysis, we have studied NaLaMnWO$_{6}$ compound which has been recently synthesized [Phys. Rev. B 79, 224428 (2009)] and belongs to the $AA'BB'{\rm O}_{6}$ family of…

Materials Science · Physics 2017-09-13 T. Fukushima , A. Stroppa , S. Picozzi , J. M. Perez-Mato

We report the comprehensive experimental results identifying the magnetic spin ordering and the magnetization dynamics of a double perovskite Pr2CoFeO6 by employing the (dc and ac) magnetization, powder neutron diffraction (NPD) and X-ray…

We have studied the atomic ordering of B-site transition metals and magnetic properties in the pulsed-laser deposited films of La2CrFeO6 (LCFO) and La2VMnO6 (LVMO), whose bulk materials are known to be single perovskites with random…

Materials Science · Physics 2015-06-12 Akira Ohtomo , Suvankar Chakraverty , Hisanori Mashiko , Takayoshi Oshima , Masashi Kawasaki

The electronic and magnetic properties of monoclinic double perovskite Sr$_2$CeIrO$_6$ were examined based on both experiments and first-principles density functional theory calculations. From the calculations we conclude that…

Materials Science · Physics 2016-07-13 Sudipta Kanungo , Kailash Mogare , Binghai Yan , Claudia Felser , Martin Jansen

In the Fe-Mo based B-site ordered double-perovskite, A2FeMoO6.0, with iron in the mixed-valence II/III state, the valence value of Fe is not precisely fixed at 2.5 but may be fine-tuned by means of applying chemical pressure at the A-cation…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Yasukawa , M. Karppinen , J. Linden , T. S. Chan , R. S. Liu , H. Yamauchi

We report and compare the structural, magnetic, and optical properties of ordered La2NiMnO6 thin films and its disordered LaNi0.5Mn0.5O3 counterpart. An x-ray diffraction study reveals that the B-site Ni/Mn ordering induces additional XRD…

Materials Science · Physics 2015-05-13 M. P. Singh , K. D. Truong , S. Jandl , P. Fournier

Perovskite-type iron oxides with Fe4+ ions have attracted much attention for their versatile helimagnetic phases. While the introduction of a layered A-site ordered structure to AFeO3 with Fe4+ ions potentially lead to novel helimagnetic…

Materials Science · Physics 2025-03-17 Masaho Onose , Hidefumi Takahashi , Hajime Sagayama , Yuichi Yamasaki , Shintaro Ishiwata

By means of density-functional simulations for half-doped manganites, such as pseudocubic Pr0.5Ca0.5MnO3 and bilayer PrCa2Mn2O7, we discuss the occurrence of ferroelectricity and we explore its crucial relation to the crystal structure and…

Strongly Correlated Electrons · Physics 2013-10-07 Kunihiko Yamauchi , Silvia Picozzi

We present a novel multiferroic double perovskite compound, CaZnFeOsO$_6$ (CZFOO), exhibiting combined ferroelectric and ferrimagnetic properties. Through ab initio density functional theory calculations, we predict CZFOO as a unique…

Materials Science · Physics 2024-08-22 Deepti Rajpoot , Paresh C. Rout , Nikita Acharya , Varadharajan Srinivasan

Anti-site disordering in Sr2FeMoO6 double perovskites (containing Mo atoms at Fe positions, and viceversa) has recently been shown to have a dramatic influence in their magnetic and magnetotransport properties. In the present study, two…

Re-based double perovskites (DPs) exhibit a complex interplay of structural and metal-insulator transitions. Here we systematically study the ground state electronic and structural properties for a family of Re-based DPs $A_2B$ReO$_6$…

Strongly Correlated Electrons · Physics 2018-01-10 Alex Taekyung Lee , Chris A. Marianetti

We use first-principles density functional theory-based calculations to investigate structural instabilities in the high symmetry cubic perovskite structure of rare-earth (R $=$ La, Y, Lu) and Bi-based biferroic chromites, focusing on…

Materials Science · Physics 2009-11-13 Nirat Ray , Umesh V. Waghmare

In the family of double perovskites, colossal magnetoresistance (CMR) has been so far observed only in half-metallic ferrimagnets such as the known case Sr$_2$FeMoO$_6$ where it has been assigned to the tunneling MR at grain boundaries due…

Strongly Correlated Electrons · Physics 2019-10-02 Lei Ding , Dmitry D. Khalyavin , Pascal Manuel , Joseph Blake , Fabio Orlandi , Wei Yi , Alexei A. Belik

We have investigated the peculiar structure of charge and spin ordering in the half-doped layered perovskite oxide La$_{1.5}$Sr$_{0.5}$CoO$_4$ by elastic neutron scattering. Two samples with different preparation histories were studied. We…

Strongly Correlated Electrons · Physics 2010-07-28 I. A. Zaliznyak , J. M. Tranquada , G. Gu , R. W. Erwin , Y. Moritomo

In electronic solids with strong spin-orbit interactions (SOIs), the spin and orbital degrees of freedom of an electron are quantum mechanically entangled, which may result in an exotic multipolar order instead of a conventional dipolar…

Strongly Correlated Electrons · Physics 2020-07-01 Daigorou Hirai , Hajime Sagayama , Shang Gao , Hiroyuki Ohsumi , Gang Chen , Taka-hisa Arima , Zenji Hiroi

Spin crossover plays a central role in the structural instability, net magnetic moment modification, metallization, and even in superconductivity in corresponding materials. Most reports on the pressure-induced spin crossover with a large…

Single phase polycrystalline sample of perovskite Sr2TiMnO6 (STMO) has been successfully synthesized via solid state reaction route. Its detailed structural and physical properties have been studied using x-ray diffraction, transmission…

Materials Science · Physics 2016-09-06 Shivani Sharma , R. Rawat , N. P. Lalla

Epitaxial La3/4Ca1/4MnO3/MgO(100) (LCMO) thin films show unusual rhombohedral (R-3c) structure with a new perovskite superstructure due to unique ordering of La and Ca at the A-site positions. Very sharp insulator-metal and…

Strongly Correlated Electrons · Physics 2009-11-11 V. Moshnyaga , L. Sudheendra , O. I. Lebedev , K. Gehrke , O. Shapoval , A. Belenchuk , S. A. Koester , B. Damaschke , G. van Tendeloo , K. Samwer

Double perovskites extend the design space for new materials, and they often host phenomena that don't exist in their parent perovskite compounds. Here, we present a detailed first principles study of the correlated double perovskite…

Strongly Correlated Electrons · Physics 2020-08-05 Arpita Paul , Turan Birol