Related papers: Low-frequency vibrational modes of stable glasses
The anharmonic soft modes studied in recent numerical work in the glass phase of simple liquids have an unstable core, stabilized by the positive restoring forces of the surrounding elastic medium. The present paper formulates an unstable…
In molecular dynamics simulations of soft glass-formers interacting via repulsions, we find that the glass transition temperature, dynamical heterogeneity, and glass fragility reach their maxima at the same crossover pressure $P_d$. Our…
In a recent publication we established an analogy between the free energy of a hard sphere system and the energy of an elastic network [1]. This result enables one to study the free energy landscape of hard spheres, in particular to define…
Despite the presence of topological disorder, phonons seem to exist also in glasses at very high frequencies (THz) and they remarkably persist into the supercooled liquid. A universal feature of such a systems is the Boson peak, an excess…
We compare the harmonic and anharmonic properties of the vibrational modes in 3-dimensional jammed packings of frictionless spheres interacting via repulsive, finite range potentials. A crossover frequency is apparent in the density of…
Implications of reduction procedures applied to the low energy part of the vibrational density of states in glasses and supercooled liquids are considered by advancing a detailed comparison between the excess - over the Debye limit -…
The concept of vibrational density of states in glasses has been mirrored in liquids by the instantaneous-normal-mode spectrum. While in glasses instantaneous configurations correspond to minima of the potential-energy hypersurface and all…
We apply a recently developed theory of the nonphononic vibrational density of states (DOS) in glasses to investigate the impact of local frozen-in stresses on the low-temperature specific heat. Using a completely harmonic description we…
In the three-dimensional Heisenberg spin glass in a random field we study the properties of the inherent structures that are obtained by an instantaneous cooling from infinite temperature. For not too large field the density of states…
We investigate correlations between low-frequency vibrational modes and rearrangements in two-dimensional colloidal glasses composed of thermosensitive microgel particles which readily permit variation of sample packing fraction. At each…
We study the spectrum of a system of coupled disordered harmonic oscillators in the thermodynamic limit. This Euclidean random matrix ensemble has been suggested as model for the low-temperature vibrational properties of glass. Exact…
We study the relation between short-time vibrational modes and long-time relaxational dynamics in a kinetically constrained lattice gas with harmonic interactions between neighbouring particles. We find a correlation between the location of…
Low-frequency Raman and inelastic neutron scattering of amorphous bis-phenol A polycarbonate is measured at low temperature, and compared. The vibrational density of states and light-vibration coupling coefficient are determined. The…
We poorly understand the properties of amorphous systems at small length scales, where a continuous elastic description breaks down. This is apparent when one considers their vibrational and transport properties, or the way forces propagate…
It is now established that glasses feature low-frequency, nonphononic excitations, in addition to phonons that follow Debye's vibrational density of state (VDoS). Extensive computer studies demonstrated that these nonphononic, glassy…
We introduce an algorithm that constructs disordered mass-spring networks whose elastic properties mimic that of glasses by tuning the fluctuations of the local elastic properties, keeping fixed connectivity and controlling the prestress.…
A hallmark of glasses is an excess of low-frequency, nonphononic vibrations, in addition to phonons. It is associated with the intrinsically nonequilibrium and disordered nature of glasses, and is generically manifested as a THz peak -- the…
We use computer simulations to study the glass transition of dense fluids made of polydisperse, repulsive spheres. For hard particles, we vary the volume fraction, phi, and use compressible particles to explore finite temperatures, T>0. In…
We present in this paper a numerical study of the vibrational eigenvectors of a two-dimensional amorphous material, previously deeply studied from the point of view of mechanical properties and vibrational eigen-frequencies [7-10].…
High Entropy Alloys (HEAs) are designed by mixing multiple metallic species in nearly the same amount to obtain crystalline or amorphous materials with exceptional mechanical properties. Here we use molecular dynamics simulations to…