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We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

Understanding the limits to the spin-coherence of the nitrogen-vacancy (NV) center in diamond is vital to realizing the full potential of this quantum system. We show that relaxation on the $|m_{s}=-1\rangle \leftrightarrow…

Mesoscale and Nanoscale Physics · Physics 2021-02-17 M. C. Cambria , A. Gardill , Y. Li , A. Norambuena , J. R. Maze , S. Kolkowitz

The unpolarized spin environment surrounding a central spin qubit is typically considered as an incoherent source of dephasing, however, precise characterization and control of the spin bath can yield a resource for storing and sensing with…

Quantum Physics · Physics 2023-12-01 R. M. Goldblatt , A. M. Martin , A. A. Wood

Various theories beyond the Standard Model predict new particles with masses in the sub-eV range with very weak couplings to ordinary matter. I present both measured and projected limits on the strengths of two possible interactions that…

Nuclear Experiment · Physics 2014-11-18 Chris Haddock

The nitrogen-vacancy (N-V) center in diamond is a promising atomic-scale system for solid-state quantum information processing. Its spin-dependent photoluminescence has enabled sensitive measurements on single N-V centers, such as: electron…

Other Condensed Matter · Physics 2015-06-25 R. J. Epstein , F. M. Mendoza , Y. K. Kato , D. D. Awschalom

The ability to perform nanoscale electric field imaging of elementary charges at ambient temperatures will have diverse interdisciplinary applications. While the nitrogen-vacancy (NV) center in diamond is capable of high-sensitivity…

Mesoscale and Nanoscale Physics · Physics 2021-04-28 M. S. J Barson , L. M. Oberg , L. P. McGuinness , A. Denisenko , N. B. Manson , J. Wrachtrup , M. W. Doherty

We experimentally demonstrate the use of a single electronic spin to measure the quantum dynamics of distant individual nuclear spins from within a surrounding spin bath. Our technique exploits coherent control of the electron spin,…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Shimon Kolkowitz , Quirin P. Unterreithmeier , Steven D. Bennett , Mikhail D. Lukin

Nanodiamonds containing negatively charged nitrogen vacancy centres (${\text{NV}}^{-}$) have applications as localized sensors in biological material and have been proposed as a platform to probe the macroscopic limits of spatial…

Chemical sensors with high sensitivity that can be used in extreme conditions and can be miniaturized are of high interest in science and industry. The Nitrogen-vacancy (NV) center in diamond is an ideal candidate as a nanosensor due to the…

Quantum Physics · Physics 2021-02-16 Hossein T. Dinani , Enrique Muñoz , Jeronimo R. Maze

We report a study of the magnetic field dependence of photoluminescence of NV$^-$ centers (negatively charged nitrogen-vacancy centers) in diamond single crystals. In such a magnetic field dependence characteristic sharp features are…

Quantum Physics · Physics 2017-09-27 Sergei V. Anishchik , Konstantin L. Ivanov

Exchange interactions between isolated pairs of spin centers in diamond have been calculated, based on an accurate atomistic electronic structure for diamond and any impurity atoms, for spin-center separations up to 2~nm. The exchange…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 V. R. Kortan , C. Şahin , M. E. Flatté

Interfacial interactions are crucial in a variety of fields and can greatly affect the electric, magnetic, and chemical properties of materials. Among them, interface orbital hybridization plays a fundamental role in the properties of…

We show that electric field noise from surface charge fluctuations can be a significant source of spin decoherence for near-surface nitrogen-vacancy (NV) centers in diamond. This conclusion is based on the increase in spin coherence…

Mesoscale and Nanoscale Physics · Physics 2015-08-26 M. Kim , H. J. Mamin , M. H. Sherwood , K. Ohno , D. D. Awschalom , D. Rugar

We report on measurements of the photoluminescence (PL) properties of single nitrogen-vacancy (NV) centers in diamond at temperatures between 4-300 K. We observe a strong reduction of the PL intensity and spin contrast between ca. 10-100 K…

Mesoscale and Nanoscale Physics · Physics 2023-09-01 Stefan Ernst , Patrick J. Scheidegger , Simon Diesch , Luca Lorenzelli , Christian L. Degen

We present experimental observations and a study of quantum dynamics of strongly interacting electronic spins, at room temperature in the solid state. In a diamond substrate, a single nitrogen vacancy (NV) center coherently interacts with…

Quantum Physics · Physics 2018-06-20 Emma L. Rosenfeld , Linh M. Pham , Mikhail D. Lukin , Ronald L. Walsworth

Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 Abdelghani Laraoui , Daniela Pagliero , Carlos A. Meriles

The negatively charged nitrogen-vacancy (NV-) center in diamond has realized new frontiers in quantum technology. Here, the center's optical and spin resonances are observed under hydrostatic pressures up to 60 GPa. Our observations…

We use tunable dipolar-interactions between the spins of nitrogen-vacancy (NV) centers in diamond to rotate a diamond crystal. Specifically, we employ cross-relaxation between the electronic spin of pairs of NV centers in a trapped diamond…

Mesoscale and Nanoscale Physics · Physics 2021-09-22 C. Pellet-Mary , P. Huillery , M. Perdriat , G. Hétet

Electron spins of diamond nitrogen-vacancy (NV) centers are important quantum resources for nanoscale sensing and quantum information. Combining NV spins with levitated optomechanical resonators will provide a hybrid quantum system for…

Quantum Physics · Physics 2016-07-21 Thai M. Hoang , Jonghoon Ahn , Jaehoon Bang , Tongcang Li

Using an optical tweezers apparatus, we demonstrate three-dimensional control of nanodiamonds in solution with simultaneous readout of ground-state electron-spin resonance (ESR) transitions in an ensemble of diamond nitrogen-vacancy (NV)…

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