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Related papers: Exciton-phonon coupling in MoSe2 monolayers

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We present a theory of optical absorption by interlayer excitons in a heterobilayer formed from transition metal dichalcogenides. The theory accounts for the presence of small relative rotations that produce a momentum shift between…

Mesoscale and Nanoscale Physics · Physics 2018-01-24 Fengcheng Wu , Timothy Lovorn , A. H. MacDonald

In the strong light-matter coupling regime realized e.g. by integrating semiconductors into optical microcavities, polaritons as new hybrid light-matter quasi-particles are formed. The corresponding change in the dispersion relation has a…

Materials Science · Physics 2022-09-08 Beatriz Ferreira , Roberto Rosati , Ermin Malic

Nonlinear interactions between excitons strongly coupled to light are key for accessing quantum many-body phenomena in polariton systems. Atomically-thin two-dimensional semiconductors provide an attractive platform for strong light-matter…

Long-lived interlayer excitons with distinct spin-valley physics in van der Waals heterostructures based on transition metal dichalcogenides make them promising for information processing in next-generation devices. While the emission…

Mesoscale and Nanoscale Physics · Physics 2021-10-18 Alberto Ciarrocchi , Dmitrii Unuchek , Ahmet Avsar , Kenji Watanabe , Takashi Taniguchi , Andras Kis

Monolayers of transition-metal dichalcogenides (TMDs) are characterized by an extraordinarily strong Coulomb interaction giving rise to tightly bound excitons with binding energies of hundreds of meV. Excitons dominate the optical response…

Materials Science · Physics 2018-05-30 Samuel Brem , Gunnar Berghaeuser , Malte Selig , Ermin Malic

We report resonant Raman spectroscopy of neutral excitons X$^0$ and intravalley trions X$^-$ in hBN-encapsulated MoS$_2$ monolayer embedded in a nanobeam cavity. By temperature tuning the detuning between Raman modes of MoS$_2$ lattice…

Mesoscale and Nanoscale Physics · Physics 2023-03-24 Chenjiang Qian , Viviana Villafañe , Marko M. Petrić , Pedro Soubelet , Andreas V. Stier , Jonathan J. Finley

Two-dimensional (2D) materials, such as graphene1, boron nitride2, and transition metal dichalcogenides (TMDs)3-5, have sparked wide interest in both device physics and technological applications at the atomic monolayer limit. These 2D…

In bilayers of semiconducting transition metal dichalcogenides, the twist angle between layers can be used to introduce a highly regular periodic potential modulation on a length scale that is large compared to the unit cell. In such…

Materials Science · Physics 2022-04-27 N. Götting , F. Lohof , C. Gies

We examine a mechanism by which excitons are generated via the LO (longitudinal optical) phonon-assisted scattering process after optical excitation of monolayer transition metal dichalcogenides. The exciton formation time is computed as a…

Materials Science · Physics 2016-10-12 A. Thilagam

We discuss the linear and two-photon spectroscopic selection rules for spin-singlet excitons in monolayer transition-metal dichalcogenides. Our microscopic formalism combines a fully $k$-dependent few-orbital band structure with a many-body…

Materials Science · Physics 2015-08-12 Timothy C. Berkelbach , Mark S. Hybertsen , David R. Reichman

Establishing a coherent interaction between a material resonance and an optical cavity is a necessary first step for the development of semiconductor quantum optics. Here we demonstrate a coherent interaction between the neutral exciton in…

Charged excitons, or X$^{\pm}$-trions, in monolayer transition metal dichalcogenides have binding energies of several tens of meV. Together with the neutral exciton X$^0$ they dominate the emission spectrum at low and elevated temperatures.…

Excitons -- elementary excitations formed by bound electron-hole pairs -- govern the optical properties and excited-state dynamics of materials. In two-dimensions (2D), excitons are theoretically predicted to have a linear energy-momentum…

Materials Science · Physics 2025-03-14 Luna Y. Liu , Steffi Y. Woo , Jinyuan Wu , Bowen Hou , Cong Su , Diana Y. Qiu

Condensation of bosons into a macroscopic quantum state belongs to the most intriguing phenomena in nature. It was first realized in quantum gases of ultra-cold atoms, but more recently became accessible in open-dissipative, exciton-based…

The weakly screened electron-hole interactions in an atomically thin semiconductor not only downshift its excitation spectrum from a quasiparticle one, but also redistribute excitation energies and wavefunction characters with profound…

Mesoscale and Nanoscale Physics · Physics 2018-10-24 Yuanxi Wang , Bruno R. Carvalho , Vincent H. Crespi

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

We present an \textit{ab initio} method to calculate phonon-assisted absorption and emission spectra in the presence of strong excitonic effects. We apply the method to bulk hexagonal BN which has an indirect band gap and is known for its…

Materials Science · Physics 2019-05-15 Fulvio Paleari , Henrique P. C. Miranda , Alejandro Molina-Sánchez , Ludger Wirtz

We explore a nonlinear field model to describe the interplay between the ability of excitons to be Bose-condensed and their interaction with other modes of a crystal. We apply our consideration to the long-living para-excitons in Cu2O.…

Strongly Correlated Electrons · Physics 2009-10-31 D. Roubtsov , Y. Lepine

Atomically thin heterostructures formed by twisted transition metal dichalcogenides can be used to create periodic moir\'e patterns. The emerging moir\'e potential can trap interlayer excitons into arrays of strongly interacting bosons,…

Mesoscale and Nanoscale Physics · Physics 2024-03-21 Samuel Brem , Ermin Malic

Two dimensional materials and their heterostructures constitute a promising platform to study correlated electronic states as well as many body physics of excitons. Here, we present experiments that unite these hitherto separate efforts and…

Mesoscale and Nanoscale Physics · Physics 2020-05-12 Yuya Shimazaki , Ido Schwartz , Kenji Watanabe , Takashi Taniguchi , Martin Kroner , Ataç Imamoğlu