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This dissertation unifies one of the central methods of classical rate calculation, `Transition-State Theory' (TST), with quantum mechanics, thereby deriving a rigorous `Quantum Transition-State Theory' (QTST). The resulting QTST is…

Chemical Physics · Physics 2014-08-06 Timothy J. H. Hele

We give a path integral construction of the quantum mechanical partition function for gauged finite groups. Our construction gives the quantization of a system of $d$, $N\times N$ matrices invariant under the adjoint action of the symmetric…

High Energy Physics - Theory · Physics 2024-02-06 Denjoe O'Connor , Sanjaye Ramgoolam

With the development of low order scaling methods for performing Kohn-Sham Density Functional Theory, it is now possible to perform fully quantum mechanical calculations of systems containing tens of thousands of atoms. However, with an…

Chemical Physics · Physics 2020-04-03 William Dawson , Stephan Mohr , Laura E. Ratcliff , Takahito Nakajima , Luigi Genovese

We present a novel numerical method for solving the elliptic partial differential equation problem for the electrostatic potential with piecewise constant conductivity. We employ an integral equation approach for which we derive a system of…

Numerical Analysis · Mathematics 2022-06-01 Kyle Bower , Kirill Serkh , Spyros Alexakis , Adam R Stinchcombe

We derive the semiclassical series for the partition function in Quantum Statistical Mechanics (QSM) from its path integral representation. Each term of the series is obtained explicitly from the (real) minima of the classical action. The…

Quantum Physics · Physics 2009-10-31 C. A. A. de Carvalho , R. M. Cavalcanti

We carry out highly accurate \emph{ab initio} path integral Monte Carlo (PIMC) simulations to directly estimate the free energy of various warm dense matter systems including the uniform electron gas and hydrogen without any nodal…

Quantum Gases · Physics 2024-07-02 Tobias Dornheim , Zhandos Moldabekov , Sebastian Schwalbe , Jan Vorberger

The computational cost of preparing a quantum state can be substantial depending on the structure of data to be encoded. Many quantum algorithms require repeated sampling to find the answer, mandating reconstruction of the same input state…

We develop an analytical technique to derive explicit forms of thermodynamical quantities within the asymptotic approach to non-extensive quantum distribution functions. Using it, we find an expression for the number of particles in a boson…

Statistical Mechanics · Physics 2009-10-31 Ugur Tirnakli , Diego F. Torres

We present a method aimed at sampling charge density fluctuations in Coulomb systems. The derivation follows from a functional integral representation of the partition function in terms of charge density fluctuations. Starting from the…

Soft Condensed Matter · Physics 2016-03-21 Frédéric Poitevin , Marc Delarue , Henri Orland

Quantum computing (QC) provides a promising avenue toward enabling quantum chemistry calculations, which are classically impossible due to a computational complexity that increases exponentially with system size. As fully fault-tolerant…

Quantum mechanics in conical space is studied by the path integral method. It is shown that the curvature effect gives rise to an effective potential in the radial path integral. It is further shown that the radial path integral in conical…

Mathematical Physics · Physics 2011-11-28 Akira Inomata , Georg Junker

We propose a path integral formulation for scale invariant quantum field theories. We do it by modifying the functional integration measure in such a way that the partition function is always exactly scale invariant, at the cost of having…

High Energy Physics - Theory · Physics 2020-07-10 Mario Herrero-Valea

We propose an approach for approximating the partition function which is based on two steps: (1) computing the partition function of a simplified model which is obtained by deleting model edges, and (2) rectifying the result by applying an…

Machine Learning · Computer Science 2012-06-18 Arthur Choi , Adnan Darwiche

We present a quantum-number projection technique which enables us to exactly treat spin, momentum and other symmetries embedded in the Hubbard model. By combining this projection technique, we extend the path-integral renormalization group…

Strongly Correlated Electrons · Physics 2007-05-23 Takahiro Mizusaki , Masatoshi Imada

We present the results of the first photonic implementation of a new method for quantum process tomography. The method (originally presented by A. Bendersky et al, Phys. Rev. Lett 100, 190403 (2008)) enables the estimation of any element of…

Quantum Physics · Physics 2010-02-25 Christian Tomás Schmiegelow , Miguel Antonio Larotonda , Juan Pablo Paz

An accurate description of electron transport at a molecular level requires a precise treatment of quantum effects. These effects play a crucial role in determining the electron transport properties of single molecules, such as…

Quantum Physics · Physics 2020-12-18 Soran Jahangiri , Juan Miguel Arrazola , Alain Delgado

The continuous quantum measurement within the probability representation of quantum mechanics is discussed. The partial classical propagator of the symplectic tomogram associated to a particular measurement outcome is introduced, for which…

Quantum Physics · Physics 2021-08-03 Yan Przhiyalkovskiy

Efficient and accurate algorithm for partition function, free energy and thermal entropy calculations is of great significance in statistical physics and quantum many-body physics. Here we present an unbiased but low-technical-barrier…

Statistical Mechanics · Physics 2024-11-19 Yi-Ming Ding , Jun-Song Sun , Nvsen Ma , Gaopei Pan , Chen Cheng , Zheng Yan

Quantum machine learning is a rapidly advancing discipline that leverages the features of quantum mechanics to enhance the performance of computational tasks. Quantum reservoir processing, which allows efficient optimization of a single…

The path-integral formulation of the statistical mechanics of quantum many-body systems is described, with the purpose of introducing practicaltechniques for the simulation of solids. Monte Carlo and molecular dynamics methods for…

Materials Science · Physics 2014-03-11 Carlos P. Herrero , Rafael Ramirez