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We present a formal analysis of nonlinear response functions in terms of correlation functions in real- and imaginary-time domains. In particular, we show that causal nonlinear response functions, expressed in terms of nested commutators in…

Mesoscale and Nanoscale Physics · Physics 2021-07-07 Habib Rostami , Mikhail I. Katsnelson , Giovanni Vignale , Marco Polini

The formalism of the reduced density matrix is pursued in both length and velocity gauges of the perturbation to the crystal Hamiltonian. The covariant derivative is introduced as a convenient representation of the position operator. This…

It is well-known that exciton effects are determinant to understand the optical absorption spectrum of low-dimensional materials. However, the role of excitons in nonlinear optical responses has been much less investigated at an…

Mesoscale and Nanoscale Physics · Physics 2024-06-21 J. J. Esteve-Paredes , M. A. García-Blázquez , A. J. Uría-Álvarez , M. Camarasa-Gómez , J. J. Palacios

Optical responses of atomically thin 2D materials are greatly influenced by electron-hole interactions. It is by far established that exciton signatures can be well-identified in the optical absorption spectrum of quasi-2D materials.…

Mesoscale and Nanoscale Physics · Physics 2023-10-30 Yu-Tzu Chang , Yang-Hao Chan

We study the linear optical absorption of bulk semiconductors in the presence of a homogeneous constant (dc) electric field with an approach suitable for including excitonic effects while working with many-band models. The absorption…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Federico Duque-Gomez , J. E. Sipe

There is an incompatibility between gauge invariance and the semi-classical time-dependent perturbation theory commonly used to calculate light absorption and scattering cross-sections. There is an additional incompatibility between…

Strongly Correlated Electrons · Physics 2018-01-17 Nadejda Bouldi , Christian Brouder

An excitonic approach to the ultrafast optical response of confined semiconductors at elevated densities below the Mott transition is presented. The theory is valid from the coherent regime, where coherent excitonic transitions and…

Mesoscale and Nanoscale Physics · Physics 2026-02-17 Henry Mittenzwey , Oliver Voigt , Andreas Knorr

Nonlinear electrical response permits a unique window into effects of band structure geometry. It can be calculated either starting from a Boltzmann approach for small frequencies, or using Kubo's formula for resonances at finite frequency.…

Mesoscale and Nanoscale Physics · Physics 2023-04-26 Daniel Kaplan , Tobias Holder , Binghai Yan

Gauge invariance is essential for making physically meaningful predictions. In superconductors, mean-field Hamiltonians that explicitly break $U(1)$ symmetry often yield gauge-dependent results. While this issue has been resolved for linear…

Superconductivity · Physics 2025-05-19 Sena Watanabe , Haruki Watanabe

We propose an analytical approach for calculating the linear and nonlinear optical (NLO) responses of monolayer transition metal dichalcogenides (TMDs) including excitonic effects. An effective Hamiltonian reproducing the trigonal warping…

Mesoscale and Nanoscale Physics · Physics 2019-07-03 Alireza Taghizadeh , T. G. Pedersen

We use the scattering approach to investigate the nonlinear current-voltage characteristic of mesoscopic conductors. We discuss the leading nonlinearity by taking into account the self-consistent nonequilibrium potential. We emphasize…

Condensed Matter · Physics 2009-10-28 T. Christen , M. Buttiker

We adapted a recently proposed framework to characterize the optical response of interacting electrons in solids in order to expedite its computation without compromise in accuracy at the microscopic level. Our formulation is based on…

Materials Science · Physics 2021-03-02 Emilia Ridolfi , Paolo E. Trevisanutto , Vitor M. Pereira

We compute the nonlinear optical response of doped mono- and bilayer graphene using the full dispersion based on tight-binding models. The response is derived with the density matrix formalism using the length gauge and is valid for any…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 F. Hipolito , Alireza Taghizadeh , T. G. Pedersen

The nonlinear optical response of an excitonic insulator coupled to lattice degrees of freedom is shown to depend in strong and characteristic ways on whether the insulating behavior originates primarily from electron-electron or…

Strongly Correlated Electrons · Physics 2021-01-04 Denis Golez , Zhiyuan Sun , Yuta Murakami , Antoine Georges , Andrew J. Millis

Nonlinear density response theory is revisited focusing on the harmonically perturbed finite temperature uniform electron gas. Within the non-interacting limit, brute force quantum kinetic theory calculations for the quadratic, cubic,…

Quantum Gases · Physics 2023-05-23 Panagiotis Tolias , Tobias Dornheim , Zhandos A. Moldabekov , Jan Vorberger

Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…

Mesoscale and Nanoscale Physics · Physics 2024-08-05 Anna M. Grudinina , Nina S. Voronova

The interaction of optical fields sculpted on the nano-scale with matter may not be described by the dipole approximation since the fields vary appreciably across the molecular length scale. Rather than incrementally adding higher…

Quantum Physics · Physics 2015-10-28 Vladimir Y. Chernyak , Prasoon Saurabh , Shaul Mukamel

The gauging of equations method, introduced in the preceding paper, is applied to the four-dimensional integral equations describing the strong interactions of three identical relativistic particles. In this way we obtain gauge invariant…

Nuclear Theory · Physics 2009-10-31 A. N. Kvinikhidze , B. Blankleider

We discuss a semiclassical calculation of low energy charge transport in one-dimensional (1d) insulators with a focus on Mott insulators, whose charge degrees of freedom are gapped due to the combination of short range interactions and a…

Strongly Correlated Electrons · Physics 2009-11-13 Bernd Rosenow

We theoretically investigate the nonlinear optical pulse responses of excitons in a thin film where the excitonic center-of-mass motion is confined. A large interaction volume between excitons and radiation yields particular coupled states…

Materials Science · Physics 2017-04-19 Takashi Kinoshita , Hajime Ishihara
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