Related papers: Hyperfine-Structure-Induced Depolarization of Impu…
The requirement of high space-time resolution and brightness is a great challenge for imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright tabletop laser, x-ray and electron sources have enabled the…
We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…
The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…
Light-induced rotation of absorbing microscopic particles by transfer of angular momentum from light to the material raises the possibility of optically driven micromachines. The phenomenon has been observed using elliptically polarized…
We introduce a new scheme for controlling the sense of molecular rotation. By varying the polarization and the delay between two ultrashort laser pulses, we induce unidirectional molecular rotation, thereby forcing the molecules to rotate…
We demonstrate strong adiabatic laser alignment and mixed-field orientation at kHz repetition rates. We observe degrees of alignment as large as cos\Theta=0.94 at 1 kHz operation for iodobenzene. The experimental setup consist of a kHz…
The alignment dependence of the ionization behavior of H$_2$ exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schr\"odinger equation within the fixed-nuclei and dipole…
In this work, we focus on the fabrication of highly uniform laser-induced periodic surface structures (LIPSS) on bulk polycarbonate (PC) using 258 nm femtosecond laser pulses. A systematic approach was pursued to investigate the influence…
Generation of highly-polarized high-energy brilliant $\gamma$-rays via laser-plasma interaction has been investigated in the quantum radiation-reaction regime. We employ a quantum-electrodynamics particle-in-cell code to describe…
The capability of generating two intense, femtosecond x-ray pulses with controlled time delay opens the possibility of performing time-resolved experiments for x-ray induced phenomena. We have applied this capability to study the…
Alpha particles emitted from an excited projectile-like fragment (PLF*) formed in a peripheral collision of two intermediate-energy heavy ions exhibit a strong preference for emission towards the target-like fragment (TLF). The interplay of…
We present a detailed theoretical and experimental study of the rotation of the plane of polarization of light traveling through a gas of fast-spinning molecules. This effect is similar to the polarization drag phenomenon predicted by Fermi…
The hybrid Stimulated Raman Scattering - Two Plasmon Decay instability had shown to play the dominant role for plasma waves excitation and energy absorption at interaction of very intense femtosecond obliquely incident $p$-polarized laser…
In this work, we observe a novel resonant mechanism, namely the modulation-induced Feshbach resonance. By applying a far-detuned laser to the cesium D2 transition with intensity modulation, we periodically shake the energy levels of atomic…
Confocal microscopy of fluorescent labeled particles has been used to study the dynamical and structural properties of colloidal and granular matter in real space. Localization algorithms allow for a fully automatized determination of the…
We characterize the temporal profile of the high-order harmonic emission from ablation plasma plumes using cross-correlations with the infrared (IR) laser beam provided by 2-photon harmonic+IR ionization of rare gas atoms. We study both…
We develop a model for predicting fine- and hyperfine intensities in the direct photoionization of molecules based on the separability of electron and nuclear spin states from vibrational-electronic states. Using spherical tensor algebra,…
The impulsive limit (the "sudden approximation") has been widely employed to describe the interaction between molecules and short, far-off-resonant laser pulses. This approximation assumes that the timescale of the laser--molecule…
For a long time transverse and longitudinal optical forces are used for non-contact and noninvasive manipulation of small individual particles. The following question arises: What is the impact of these forces on the ensemble of thousand…
Two mechanisms of two-color (\omega + 2\omega) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While…