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The relationship between the molecular structure and the formation of the NTB phase is still at an early stage of development. This is mainly related to molecular geometry, while the correlation between the NTB phase and the electronic…

Chemical Physics · Physics 2021-01-04 Katarzyna Merkel , Barbara Loska , Chris Welch , Georg H. Mehl , Antoni Kocot

The long coherence time of a single nitrogen vacancy (NV) center spin in diamond is a crucial advantage for implementing quantum information processing. However, the realization of strong coupling between single NV spins is challenging.…

Quantum Physics · Physics 2021-05-19 Wei Xiong , Jiaojiao Chen , Baolong Fang , Mingfeng Wang , Liu Ye , J. Q. You

Alkaline-earth-like transition-metal atoms such as Zn and Cd are promising candidates for precision measurements and quantum many-body physics experiments. Here, we theoretically investigate the properties of diatomic molecules containing…

Atomic Physics · Physics 2021-11-02 Klaudia Zaremba-Kopczyk , Michał Tomza

Infrared spectroscopy (IR) and quantum chemistry calculations, based on density functional theory (DFT) were used to study the structure and the molecular interactions in the nematic (N) and twist-bend (NTB) phases of thioether-linked…

Soft Condensed Matter · Physics 2022-06-16 Katarzyna Merkel , Barbara Loska , Yuki Arakawa , Georg H. Mehl , Jakub Karcz , Antoni Kocot

We present a theoretical analysis of the electron spin decoherence in single Nitrogen-Vacancy defects in ultra-pure diamond. The electron spin decoherence is due to the interactions with Carbon-13 nuclear spins in the diamond lattice. Our…

Other Condensed Matter · Physics 2009-11-13 J. R. Maze , J. M. Taylor , M. D. Lukin

The coupling between defects in diamond and a superconducting microwave resonator is studied in the nonlinear regime. Both negatively charged nitrogen-vacancy and P1 defects are explored. The measured cavity mode response exhibits strong…

Quantum Physics · Physics 2018-06-13 Nir Alfasi , Sergei Masis , Roni Winik , Demitry Farfurnik , Oleg Shtempluck , Nir Bar-Gill , Eyal Buks

We develop a quantum theory for a variety of nuclear spin dynamics such as dephasing, relaxation, squeezing, and narrowing due to the hyperfine interaction with a generic, dissipative electronic system. The first-order result of our theory…

Quantum Physics · Physics 2014-09-05 Ping Wang , Jiangfeng Du , Wen Yang

The negatively charged nitrogen-vacancy (NV) center in diamond is a leading solid-state quantum emitter, offering spin-photon interfaces over a wide temperature range with applications from electromagnetic sensing to bioimaging. While NV…

We describe how to prepare an electrically levitated nanodiamond in a superposition of orientations via microwave driving of a single embedded nitrogen-vacancy (NV) center. Suitably aligning the magnetic field with the NV center can serve…

Due to its superior coherent and optical properties at room temperature, the nitrogen-vacancy (N-V ) center in diamond has become a promising quantum probe for nanoscale quantum sensing. However, the application of N-V containing…

We theoretically characterize interactions, energetics, and chemical reaction paths in ionic two-body and three-body systems of alkali-metal and alkaline-earth-metal atoms in the context of modern experiments with cold hybrid ion-atom…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

Optically-pumped color centers in semiconductor powders can potentially induce high levels of nuclear spin polarization in surrounding solids or fluids at or near ambient conditions, but complications stemming from the random orientation of…

The limitation of simultaneous measurements of noncommuting observables can be eliminated when the measured particle is maximally entangled with a quantum memory. We present a proposal for testing this quantum-memory-assisted entropic…

Quantum Physics · Physics 2012-12-27 Z. Y. Xu , S. Q. Zhu , W. L. Yang

This study utilises linear-scaling density functional theory (DFT) and develops a new machine-learning potential for carbon and nitrogen (GAP-CN), based on the carbon potential (GAP20), to investigate the interaction between carbon…

Computational Physics · Physics 2025-01-22 Guangzhao Chen , Joseph C. A. Prentice , Jason M. Smith

We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional…

We propose an efficient quantum measurement protocol for the hyperfine interaction between the electron spin and the $^{15}$N nuclear spin of a diamond nitrogen-vacancy center. In this protocol, a sequence of quantum operations of…

Quantum Physics · Physics 2012-05-24 Kilhyun Bang , Wen Yang , L. J. Sham

The Mott insulator $\beta'$-EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ belongs to a class of charge transfer solids with highly-frustrated triangular lattice of $S=1/2$ molecular dimers and a quantum-spin-liquid ground state. Our experimental and ab…

Strongly Correlated Electrons · Physics 2018-06-27 P. Lazić , M. Pinterić , D. Rivas Góngora , A. Pustogow , K. Treptow , T. Ivek , O. Milat , B. Gumhalter , N. Došlić , M. Dressel , S. Tomić

The ground state spin of the negatively charged nitrogen-vacancy center in diamond has many exciting applications in quantum metrology and solid state quantum information processing, including magnetometry, electrometry, quantum memory and…

Materials Science · Physics 2012-06-05 M. W. Doherty , F. Dolde , H. Fedder , F. Jelezko , J. Wrachtrup , N. B. Manson , L. C. L. Hollenberg

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Coherence of spins of electrons confined in III-V quantum dots is strongly affected by their hyperfine interaction with the nuclei. In this paper an introduction to this subject will be given. Some theoretical approaches to the problem will…

Mesoscale and Nanoscale Physics · Physics 2016-04-18 Łukasz Cywiński