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A detailed treatment of an electro-optical trap for polar molecules, realized by embedding an optical trap within a uniform electrostatic field, is presented and the trap's properties analyzed and discussed. The electro-optical trap offers…

Atomic Physics · Physics 2022-06-15 Bretislav Friedrich

Tightly focused optical dipole traps induce vector light shifts ("fictitious magnetic fields") which complicate their use for single-atom trapping and manipulation. The problem can be mitigated by adding a larger, real magnetic field, but…

Atomic Physics · Physics 2018-02-14 Sébastien Garcia , Jakob Reichel , Romain Long

We demonstrate long rotational coherence of individual polar molecules in the motional ground state of an optical trap. In the present, previously unexplored regime, the rotational eigenstates of molecules are dominantly quantized by…

State-dependent optical tweezers can be used to trap a pair of molecules with a separation much smaller than the wavelength of the trapping light, greatly enhancing the dipole-dipole interaction between them. Here we describe a general…

Atomic Physics · Physics 2021-04-05 L. Caldwell , M. R. Tarbutt

Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…

Quantum Physics · Physics 2011-01-04 Svetlana Kotochigova , David DeMille

We demonstrate that the differential ac-Stark shift of a ground-state hyperfine transition in an optical trap can be eliminated by using properly polarized trapping light. We use the vector polarizability of an alkali-metal atom to produce…

Atomic Physics · Physics 2015-06-17 Huidong Kim , Hyok Sang Han , D. Cho

Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most…

Atomic Physics · Physics 2014-12-01 Rosa Glöckner , Alexander Prehn , Gerhard Rempe , Martin Zeppenfeld

We show theoretically and demonstrate experimentally that highly absorbing particles can be trapped and manipulated in a single highly focused Gaussian beam. Our studies of the effects of polarized light on such particles show that they can…

Focusing optics for neutral molecules finds application in shaping and steering molecular beams. Here we present an electrostatic elliptical mirror for polar molecules consisting of an array of microstructured gold electrodes deposited on a…

We consider the practical feasibility of using the direct, electric dipole-dipole interaction between co-trapped molecular ions for robust quantum logic without the need for static polarizing fields. The use of oscillating dipole moments,…

Atomic Physics · Physics 2018-10-31 Eric R. Hudson , Wesley C. Campbell

Superpositions of rotational states in polar molecules induce strong, long-range dipolar interactions. Here we extend the rotational coherence by nearly one order of magnitude to 8.7(6) ms in a dilute gas of polar $^{23}$Na$^{40}$K…

We show how state-dependent optical potentials can be used to trap a pair of molecules in different internal states at a separation much smaller than the wavelength of the trapping light. This close spacing greatly enhances the…

Atomic Physics · Physics 2021-04-05 L. Caldwell , M. R. Tarbutt

Proposals for quantum computing using rotational states of polar molecules as qubits have previously considered only diatomic molecules. For these the Stark effect is second-order, so a sizable external electric field is required to produce…

Quantum Physics · Physics 2015-05-30 Qi Wei , Sabre Kais , Bretislav Friedrich , Dudley Herschbach

In this paper we show that it is possible to switch the spin polarization of the photocurrent signal obtained from a single self-assembled quantum dot photodiode under the effect of elliptically polarized light by just increasing the light…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. M. Villas-Boas , Sergio E. Ulloa , A. O. Govorov

We use the polarized Fock states to describe the coupled molecule-cavity hybrid system in quantum electrodynamics. The molecular permanent dipoles polarize the photon field by displacing its vector potential, leading to non-orthogonality…

Quantum Physics · Physics 2020-05-04 Arkajit Mandal , Sebastian Montillo Vega , Pengfei Huo

This paper describes a method for the explicit reconstruction and visualization of various polarization ellipses from the intensities measured after a rotating polarizer. The state of polarization of a light beam is represented by the…

Optics · Physics 2022-11-29 Ramonika Sengupta , Brijesh Tripathi , Asha Adhiya

In conventional optical Stark-shift spectroscopy, molecules are exposed to spatially homogeneous static electric fields that shift the energies of their spectral lines. These shifts are attributed to the molecular electronic properties,…

We study the cancellation of differential ac Stark shifts in the 5s and 5p states of rubidium atom using the linearly and circularly polarized lights by calculating their dynamic polarizabilities. Matrix elements were calculated using a…

Atomic Physics · Physics 2015-06-11 Bindiya Arora , B. K. Sahoo

We show that colloidal molecular crystal states interacting with a periodic substrate, such as an optical trap array, and a rotating external field can undergo a rapid pattern switching in which the orientation of the crystal changes. In…

Soft Condensed Matter · Physics 2015-05-13 C. Reichhardt , C. J. Olson Reichhardt

Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution…

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