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Variational methods are used to calculate structural and thermodynamical properties of a titrating polyelectrolyte in a discrete representation. The Coulomb interactions are emulated by harmonic repulsive forces, the force constants being…

chem-ph · Physics 2008-02-03 B. Jönsson , M. Ullner , C. Peterson , O. Sommelius , B. Söderberg

We propose a new explicit pseudo-energy and momentum conserving scheme for the time integration of Hamiltonian systems. The scheme, which is formally second-order accurate, is based on two key ideas: the integration during the time-steps of…

Numerical Analysis · Mathematics 2020-08-14 Frédéric Marazzato , Alexandre Ern , Christian Mariotti , Laurent Monasse

A new symbolic algorithmic implementation of the general scheme of the exponentially convergent functional-discrete (FD-) method is developed and justified for the Sturm-Liouville problem on a finite interval for the Schr\"odinger equation…

Numerical Analysis · Mathematics 2018-06-26 Volodymyr Makarov , Nataliia Romaniuk

The increasing use of high-throughput density-functional theory (DFT) calculations in the computational design and optimization of materials requires the availability of a comprehensive set of soft and transferable pseudopotentials. Here we…

Materials Science · Physics 2013-12-10 Kevin F. Garrity , Joseph W. Bennett , Karin M. Rabe , David Vanderbilt

Analytic and approximate solutions for the energy eigenvalues generated by a confined softcore Coulomb potentials of the form a/(r+\beta) in d>1 dimensions are constructed. The confinement is effected by linear and harmonic-oscillator…

Mathematical Physics · Physics 2015-06-22 Richard L Hall , Nasser Saad

We describe a new algorithm for trajectory optimization of mechanical systems. Our method combines pseudo-spectral methods for function approximation with variational discretization schemes that exactly preserve conserved mechanical…

Systems and Control · Computer Science 2017-05-26 Akshay Srinivasan , Madhusudhan Venkadesan

Depending on the behaviour of the complex-valued electromagnetic potential in the neighbourhood of infinity, pseudomodes of one-dimensional Dirac operators corresponding to large pseudoeigenvalues are constructed. This is a first systematic…

Mathematical Physics · Physics 2022-08-22 David Krejcirik , Tho Nguyen Duc

In many applications it is important to understand the sensitivity of eigenvalues of a matrix polynomial to perturbations of the polynomial. The sensitivity commonly is described by condition numbers or pseudospectra. However, the…

Numerical Analysis · Mathematics 2017-04-06 Silvia Noschese , Lothar Reichel

We derive the expressions for configurational forces in Kohn-Sham density functional theory, which correspond to the generalized variational force computed as the derivative of the Kohn-Sham energy functional with respect to the position of…

Computational Physics · Physics 2018-04-25 Phani Motamarri , Vikram Gavini

In this article, we combine the periodic sinc basis set with a curvilinear coordinate system for electronic structure calculations. This extension allows for variable resolution across the computational domain, with higher resolution close…

Computational Physics · Physics 2024-07-09 Michael Lindsey , Sandeep Sharma

Linear-scaling electronic structure methods based on the calculation of moments of the underlying electronic Hamiltonian offer a computationally efficient and numerically robust scheme to drive large-scale atomistic simulations, in which…

Materials Science · Physics 2017-01-09 Eunan J. McEniry , Ralf Drautz

Pseudo-Newtonian potentials are a tool often used in theoretical astrophysics to capture some key features of a black-hole space-time in a Newtonian framework. As a result, one can use Newtonian numerical codes, and Newtonian formalism in…

General Relativity and Quantum Cosmology · Physics 2017-06-08 Vojtech Witzany , Claus Laemmerzahl

We have optimized the exponents of Gaussian s and p basis functions for the elements H, B-F, and Al-Cl using the pseudopotentials of Goedecker, Teter, and Hutter [Phys. Rev. B 54, 1703 (1996)] by minimizing the total energy of dimers. We…

Other Condensed Matter · Physics 2007-12-21 Eeuwe S. Zijlstra , Nils Hunteman , Alan Kalitsov , Martin E. Garcia , Ulf von Barth

The modified Becke-Johnson exchange potential combined with local-density approximation correlation (mBJLDA) has recently attracted interest because it provides highly improved band gaps at a very low computational cost. In this work we…

Materials Science · Physics 2022-04-04 Hazem Abu-Farsakh , Abdallah Qteish

We present analytically the exact energy bound-states solutions of the Schrodinger equation in D-dimensions for an alternative (often used) pseudo-Coulomb potential-plus- ring-shaped potential of the form $V(r)=-%…

Quantum Physics · Physics 2008-07-15 Sameer M. Ikhdair , Ramazan Sever

The paper addresses an escape of a classical particle from a potential well under harmonic forcing. Most dangerous/efficient escape dynamics reveals itself in conditions of 1:1 resonance and can be described in the framework of isolated…

Dynamical Systems · Mathematics 2022-03-02 Pavel Kravetc , Oleg Gendelman

Polymer self-consistent field theory techniques are used to find radial electron densities and total binding energies for isolated atoms. Quantum particles are modelled as Gaussian threads with ring-polymer architecture in a four…

Quantum Physics · Physics 2022-11-30 Russell B. Thompson

A scheme is developed for creating pseudopotentials for use in correlated-electron calculations. Pseudopotentials for the light elements H, Li, Be, B, C, N, O, and F, are reported, based on data from high-level quantum chemical…

Materials Science · Physics 2014-05-05 J. R. Trail , R. J. Needs

An expression is given for the electronic polarization of an insulating crystal within the ultrasoft pseudopotential scheme. The pseudopotential charge-augmentation terms modify the usual Berry-phase expression, and also give rise to a…

Materials Science · Physics 2007-05-23 David Vanderbilt , R. D. King-Smith

A linear-algebraic theory called 'multiple Arnoldi method' is presented and realizes large-scale (order-N) electronic structure calculation with generalized eigen-value equations. A set of linear equations, in the form of (zS-H) x = b, are…

Materials Science · Physics 2012-04-04 T. Hoshi , S. Yamamoto , T. Fujiwara , T. Sogabe , S. -L. Zhang
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