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Spontaneous entry of water molecules inside single-wall carbon nanotubes (SWCNTs) has been confirmed by both simulations and experiments. Using molecular dynamics simulations, we have studied the thermodynamics of filling of a (6,6) carbon…

Mesoscale and Nanoscale Physics · Physics 2015-01-27 Hemant Kumar , Chandan Dasgupta , Prabal K. Maiti

In order to accommodate an increasing demand for carbon nanotubes (CNTs) with desirable characteristics one has to understand the origin of helicity of their structures. Here, through in situ microscopy we demonstrate that the nucleation of…

Materials Science · Physics 2014-08-12 Rahul Rao , Renu Sharma , Frank Abild-Pedersen , Jens K. Nørskov , Avetik R. Harutyunyan

A mechanically bistable single-walled carbon nanotube can act as a variable-shaped capacitor with a voltage-controlled transition between collapsed and inflated states. This external control parameter provides a means to tune the system so…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Oleg E. Shklyaev , Eric Mockensturm , Vincent H. Crespi

The evolution of a continuous Fe(NO3)3 catalyst film was observed by in-situ annealing in a Transmission Electron Microscope (TEM). Such catalysts are routinely used in the catalytic growth of carbon nanotubes. The experiments reveal that…

Materials Science · Physics 2015-07-20 Christian Klinke , Jean-Marc Bonard , Klaus Kern

Through a careful modeling of interactions, collisions, and the catalytic behavior, one can obtain important information about the initial stage of growth of single-wall carbon nanotubes (SWCNTs), where a state-of-the-art semi-empirical…

Materials Science · Physics 2012-01-17 I. Chaudhuri , Ming Yu , C. S. Jayanthi , S. Y. Wu

Various diameters of alumina-supported Fe catalysts are used to grow single-walled carbon nanotubes (SWCNTs) with chemical vapor decomposition. We find that the reduction of the catalyst size requires an increase of the minimum temperature…

Materials Science · Physics 2009-11-13 A. R. Harutyunyan , N. Awasthi , A. Jiang , W. Setyawan , E. Mora , T. Tokune , K. Bolton , S. Curtarolo

Growth of carbon nanotubes (CNTs) was performed by atmospheric pressure chemical vapour deposition (APCVD) of propane on Si(111) with a pre-treated Ni overlayer acting as a catalyst. Prior to the growth of CNTs, a thin film of Ni was…

Materials Science · Physics 2019-06-04 J Sengupta , SK Panda , C Jacob

The carbon rich phase diagrams of nickel-carbon nanoparticles, relevant to catalysis and catalytic chemical vapor deposition synthesis of carbon nanotubes, are calculated for system sizes up to about 3 nanometers (807 Ni atoms). A tight…

Atomic and Molecular Clusters · Physics 2015-06-11 Yann Magnin , Alexandre Zappelli , Hakim Amara , François Ducastelle , Christophe Bichara

In this study, the synthesis of multi-walled carbon nanotubes (MWCNTs) was carried out by chemical vapor deposition (CVD) using propane as the carbon source and Si as the catalyst support. The effect of CVD process variables such as…

Applied Physics · Physics 2018-08-21 Joydip Sengupta

We present a novel floating catalyst synthesis route for individual, i.e. non-bundled, small diameter single-walled carbon nanotubes (SWCNTs) with a narrow chiral angle distribution peaking at high chiralities near the armchair species. An…

We investigate experimentally the transport properties of single-walled carbon nanotube bundles as a function of temperature and applied current over broad intervals of these variables. The analysis is performed on arrays of nanotube…

Materials Science · Physics 2009-11-13 M. Salvato , M. Cirillo , M. Lucci , S. Orlanducci , I. Ottaviani , M. L. Terranova , F. Toschi

The nucleation of carbon nanotubes on small nickel clusters is studied using a tight binding model coupled to grand canonical Monte Carlo simulations. This technique closely follows the conditions of the synthesis of carbon nanotubes by…

Materials Science · Physics 2007-05-23 Hakim Amara , Christophe Bichara , François Ducastelle

This investigation deals with the effect of growth temperature on the growth behavior of Fe filled multiwalled carbon nanotubes (MWCNTs). Carbon nanotube (CNT) synthesis was carried out in a thermal chemical vapor deposition (CVD) reactor…

Materials Science · Physics 2019-08-07 Joydip Sengupta , Chacko Jacob

Multiwalled carbon nanotubes are shown to be ballistic conductors at room temperature, with mean free paths of the order of tens of microns. These experiments follow and extend the original experiments by Frank et al (Science, 280 1744…

Materials Science · Physics 2007-05-23 Philippe Poncharal , Claire Berger , Yan Yi , Z. L. Wang , Walt A. de Heer

Carbon nanotubes are nano-objects with quite anisotropic properties, for example the mechanical properties in longitudinal and radial directions differ significantly. This feature of the carbon nanotubes yields many interesting phenomena…

Mesoscale and Nanoscale Physics · Physics 2023-10-26 Alexander V. Savin , Margarita Kovaleva

Three typical one-dimensional (1D)/quasi-1D nanocarbons, linear carbon chains, carbon nanotubes, and graphene nanoribbons have been proven to grow inside single-wall carbon nanotubes. This gives rise to three types of hybrid materials whose…

Materials Science · Physics 2021-01-29 Weili Cui , Takeshi Saito , Paola Ayala , Thomas Pichler , Lei Shi

Chiral crystals exhibit useful handedness-dependent properties, including spin selectivity and circularly polarized light sensitivity, yet controlling which enantiomer forms during synthesis remains a central challenge. Existing approaches…

The dynamical conductance of electrically contacted single-walled carbon nanotubes is measured from dc to 10 GHz as a function of source-drain voltage in both the low-field and high-field limits. The ac conductance of the nanotube itself is…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Z. Yu , P. J. Burke

We use electrostatic force microscopy and scanned gate microscopy to probe the conducting properties of carbon nanotubes at room temperature. Multi-walled carbon nanotubes are shown to be diffusive conductors, while metallic single-walled…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 A. Bachtold , M. S. Fuhrer , S. Plyasunov , M. Forero , Erik H. Anderson , A. Zettl , Paul L. McEuen

The material and electrical properties of the CNT single vias and array vias grown by microwave plasma-enhanced chemical vapor deposition were investigated. The diameters of multiwall carbon nanotubes (MWNTs) grown on the bottom electrode…

Materials Science · Physics 2007-08-10 J. -H. Ting , C. -C. Chiu , F. -Y. Huang