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Identifying two-dimensional heterostructures with exceptional electronic and optical properties remains an active area of research in advanced optoelectronics. Here, we present a comprehensive first-principles investigation of the…

Van der Waals (vdW) heterobilayers formed by two-dimensional (2D) transition metal dichalcogenides (TMDCs) created a promising platform for various electronic and optical properties. ab initio band results indicate that the band offset of…

Materials Science · Physics 2020-09-04 Yuanyuan Wang , Fengping Li , Wei Wei , Baibiao Huang , Ying Dai

Van der Waals heterobilayers based on 2D transition metal dichalcogenides have been recently shown to support robust and long-lived valley polarization for potential valleytronic applications. However, the role of the band structure and…

In van der Waals heterostructures of two-dimensional transition-metal dichalcogenides (2D TMDCs) electron and hole states are spatially localized in different layers forming long-lived interlayer excitons. Here, we have investigated, from…

Materials Science · Physics 2020-11-03 Muhammad S. Ramzan , Jens Kunstmann , Agnieszka B. Kuc

Analogous to conventional charge-based electronics, valleytronics aims at encoding data via the valley degree of freedom, enabling new routes for information processing. Long-lived interlayer excitons (IXs) in van der Waals heterostructures…

Applied Physics · Physics 2021-03-30 Tong Ye , Yongzhuo Li , Junze Li , Hongzhi Shen , Junwen Ren , Cun-Zheng Ning , Dehui Li

The nanoscale periodic potentials introduced by moir\'{e} patterns in semiconducting van der Waals (vdW) heterostructures provide a new platform for designing exciton superlattices. To realize these applications, a thorough understanding of…

Controlling matter-light interactions with cavities is of fundamental importance in modern science and technology. It is exemplified in the strong-coupling regime, where matter-light hybrid modes form, with properties controllable via the…

Mesoscale and Nanoscale Physics · Physics 2021-11-03 Long Zhang , Fengcheng Wu , Shaocong Hou , Zhe Zhang , Yu-Hsun Chou , Kenji Watanabe , Takashi Taniguchi , Stephen R. Forrest , Hui Deng

Excitons are key to the optoelectronic applications of van der Waals semiconductors with the potential for versatile on-demand tuning of properties. Yet, their electrical manipulation is complicated by their inherent charge neutrality and…

Mesoscale and Nanoscale Physics · Physics 2024-04-16 Sarthak Das , Ding Huang , Ivan Verzhbitskiy , Zi-En Ooi , Chit Siong Lau , Rainer Lee , Calvin Pei Yu Wong , Kuan Eng Johnson Goh

Monolayer (ML) transition metal dichalcogenides (TMDs) integrated in optical microcavities host exciton-polaritons as a hallmark of the strong light-matter coupling regime. Analogous concepts for hybrid light-matter systems employing…

Excitons dominate the optics of atomically-thin transition metal dichalcogenides and 2D van der Waals heterostructures. Interlayer 2D excitons, with an electron and a hole residing in different layers, form rapidly in heterostructures…

Mesoscale and Nanoscale Physics · Physics 2021-04-20 M. G. Burdanova , M. Liu , M. Staniforth , Y. Zheng , R. Xiang , S. Chiashi , A. Anisimov , E. I. Kauppinen , S. Maruyama , J. Lloyd-Hughes

Excitons in van der Waals heterostructures come in many different forms. In bilayer structures, the electron and hole may be localized on the same layer or they may be separated forming an interlayer exciton with a finite out-of-plane…

Mesoscale and Nanoscale Physics · Physics 2024-06-17 Thorsten Deilmann , Kristian Sommer Thygesen

Many-body exciton interactions shape the optoelectronic response of atomically-thin transition metal dichalcogenides, yet optical control of these interactions remains largely unexplored. To date, modulation of exciton-exciton interactions…

Vertically stacked van der Waals structures are promising platforms that enable layer engineering, opening new avenues for the quantum control of elementary excitations, including optically generated bound electron-hole pairs. Here we…

Mesoscale and Nanoscale Physics · Physics 2025-07-16 Alexandre R. Rocha , Rodrigo G. Amorim , Wanderlã L. Scopel , Cesar E. P. Villegas

Atomically-thin layers of two-dimensional materials can be assembled in vertical stacks held together by relatively weak van der Waals forces, allowing for coupling between monolayer crystals with incommensurate lattices and arbitrary…

Lateral heterostructures of 2D transition metal dichalcogenide offer a powerful platform to investigate photonic and electronic phenomena at atomically sharp interfaces. However, their controlled engineering, including tuning lateral domain…

Moire superlattices in van der Waals (vdW) heterostructures could trap strongly bonded and long lived interlayer excitons. Assumed to be localized, these moire excitons could form ordered quantum dot arrays, paving the way for novel…

Computational Physics · Physics 2021-01-22 Hongli Guo , Xu Zhang , Gang Lu

Due to a strong Coulomb interaction, excitons dominate the excitation kinetics in 2D materials. While Coulomb-scattering between electrons has been well studied, the interaction of excitons is more challenging and remains to be explored. As…

Materials Science · Physics 2021-01-27 Daniel Erkensten , Samuel Brem , Ermin Malic

Exciton-exciton interactions are key to understanding non-linear optical and transport phenomena in van der Waals heterobilayers, which emerged as versatile platforms to study correlated electronic states. We present a combined…

Interlayer excitons (IXs) in hetero-bilayers of transition metal dichalcogenides (TMDs) represent an exciting emergent class of long-lived dipolar composite bosons in an atomically thin, near-ideal two-dimensional (2D) system. The…

Semiconductor heterostructures provide a powerful platform for the engineering of excitons. Here we report the excitonic properties of two-dimensional (2D) heterostructures that consist of monolayer MoS2 and WS2 stacked epitaxially or…