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Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

Measuring the delay for an electron to emerge from different states is one of the major achievements of attosecond science. This delay can have two origins - the electron wave packet is reshaped during departure by the electrostatic field…

Atomic Physics · Physics 2020-10-14 Graham G. Brown , Dong Hyuk Ko , Chunmei Zhang , P. B. Corkum

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

A new method to coherently control the electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the…

Atomic Physics · Physics 2015-04-06 Pengfei Lan , Peixiang Lu , Wei Cao , Yuhua Li , Xinlin Wang

A new method for efficiently generating an isolated single-cycle attosecond pulse is proposed. It is shown that the ultraviolet (UV) attosecond pulse can be utilized as a robust tool to control the dynamics of electron wave packets (EWPs).…

Atomic Physics · Physics 2009-11-13 Pengfei Lan , Peixiang Lu , Wei Cao , Xinlin Wang

Ultraviolet and extreme ultraviolet electric-fields produced by relativistic electrons in an undulator of a synchrotron light source are characterized by using spectral phase interferometry for direct electric-field reconstruction (SPIDER).…

We present an innovative beamline for extreme ultraviolet (XUV)-infrared (IR) pump-probe reflection spectroscopy in solids with attosecond temporal resolution. The setup uses an actively stabilized interferometer, where attosecond pulse…

The advancement of the ultrafast pulse shaping and waveform synthesis allowed to coherently control the atomic and electronic motions in matter. The temporal resolution of the waveform synthesis is inversely proportional to the broadening…

Optics · Physics 2024-06-04 Husain Alqattan , Dandan Hui , Vladimir Pervak , Mohammed Th. Hassan

The attosecond streaking technique is normally utilized to characterize the attosecond pulses in extreme ultraviolet spectrum, while the pulse simulation and reconstruction schemes turn out to be unreliable for extremely short sub-100as…

Optics · Physics 2018-09-05 Renzhi Shao , Bin Li

We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.

Optics · Physics 2016-08-16 Antoine Monmayrant , Béatrice Chatel , Bertrand Girard

A compact high repetition rate attosecond light source based on a standard laser oscillator combined with plasmonic enhancement is presented. At repetition rates of tens of MHz, we predict focusable pulses with durations of ~< 300…

Optics · Physics 2014-05-19 Mattia Lupetti , Matthias F. Kling , Armin Scrinzi

Attosecond x-ray pulse with known spectro-temporal information is an essential tool for the investigation of ultrafast electron dynamics in quantum systems. Ultrafast free-electron lasers (FELs) have the unique advantage on unprecedented…

Accelerator Physics · Physics 2023-04-17 Yaozong Xiao , Hao Sun , Bo Liu , Zhentang Zhao , Chao Feng

Comprehending the unique characteristics of structured ultrafast optical pulses is essential to the physics, applications and instrumentations of ultrafast lasers. However, full-vectrorial characterizations of the pulses remain challenging…

Optics · Physics 2020-02-03 Tiancheng Huo , Li Qi , Janson J. Chen , Yusi Miao , Zhongping Chen

Attosecond science has been transforming our understanding of electron dynamics in atoms, molecules and solids. However, to date almost all of the attoscience experiments have been based on spectroscopic measurements because attosecond…

The generation of ultrashort light pulses is essential for the advancement of attosecond science. Here, we show that attosecond pulses approaching the Fourier limit can be generated through optimized optical driving of tunneling particles…

Mesoscale and Nanoscale Physics · Physics 2024-02-19 Shohei Imai , Atsushi Ono

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

In this paper, we propose a new method to characterize the temporal structure of arbitrary optical laser pulses with low pulse energies. This approach is based on strong field photoelectron holography with the glory rescattering effect as…

Atomic Physics · Physics 2020-04-29 J. F. Tao , J. Cai , Q. Z. Xia , J. Liu

Many experiments in attosecond science will benefit from attosecond pulses at high repetition rates with sufficient photon flux for pump-probe experiments. We use 7fs, 800nm pulses from a non-collinear optical parametric chirped pulse…