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Resonant inelastic x-ray scattering (RIXS) is an evolving tool for investigating spin dynamics of strongly correlated materials, which complements inelastic neutron scattering. Both techniques have found that non-spin-conserving (NSC)…

One-dimensional (1D) magnetic insulators have attracted significant interest as a platform for studying emergent phenomena such as quasiparticle fractionalization and quantum criticality. The antiferromagnetic Heisenberg chain of spins-1/2…

Strongly Correlated Electrons · Physics 2018-12-20 J. Schlappa , U. Kumar , K. J. Zhou , S. Singh , M. Mourigal , V. N. Strocov , A. Revcolevschi , L. Patthey , H. M. Rønnow , S. Johnston , T. Schmitt

We theoretically investigate the resonant inelastic X-ray scattering (RIXS) spectra in a quasi-1D chain of weakly coupled frustrated spin-1/2 trimers, as realized in Na$_{2}$Cu$_{3}$Ge$_{4}$O$_{12}$, with Cu $d^{9}$ 1/2 spins. We compute…

Strongly Correlated Electrons · Physics 2024-10-22 Prabhakar , Subhajyoti Pal , Umesh Kumar , Manoranjan Kumar , Anamitra Mukherjee

We investigate the excitation spectra of a spin-1/2 antiferromagnetic Heisenberg trimer spin chain by employing a combination of numerical and theoretical techniques. Utilizing the Krylov-space correction-vector method in density matrix…

Strongly Correlated Electrons · Physics 2025-01-17 Junli Li , Jun-Qing Cheng , Trinanjan Datta , Dao-Xin Yao

Resonant inelastic x-ray spectroscopy (RIXS) has emerged as an important tool to explore magnetism in two-dimensional (2D) antiferromagnet realized in strongly correlated materials. Here we consider the Heisenberg model with nearest and…

Strongly Correlated Electrons · Physics 2023-12-12 Subhajyoti Pal , Umesh Kumar , Prabhakar , Anamitra Mukherjee

We report a Cu $K$-edge resonant inelastic x-ray scattering (RIXS) study of spin excitations in the $S$=1/2 antiferromagnetic chain system Sr$_2$CuO$_3$. The spectral weight observed below the charge-transfer gap appears in two-spinon…

Strongly Correlated Electrons · Physics 2025-10-31 Kenji Ishii , Kenji Tsutsui , Takayuki Kawamata , Yoji Koike

We present a resonant inelastic x-ray scattering (RIXS) study of spin and charge excitations in overdoped La1.77Sr0.23CuO4 along two high-symmetry directions. The line shape of these excitations is analyzed and they are shown to be highly…

Superconductivity · Physics 2016-02-05 C. Monney , T. Schmitt , C. E. Matt , J. Mesot , V. N. Strocov , O. J. Lipscombe , S. M. Hayden , J. Chang

We study two-magnon excitations in resonant inelastic x-ray scattering (RIXS) at the transition-metal $K$-edge. Instead of working with effective Heisenberg spin models, we work with a Hubbard-type model ($d$-$p$ model) for a typical…

Strongly Correlated Electrons · Physics 2017-10-18 Takuji Nomura

Measurements of spin excitations are essential for an understanding of spin-mediated pairing for superconductivity; and resonant inelastic X-ray scattering (RIXS) provides a considerable opportunity to probe high-energy spin excitations.…

We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to \emph{collective} magnetic excitations in $S=1$ systems by probing the Ni $L_3$-edge of La$_{2-x}$Sr$_x$NiO$_4$ ($x = 0, 0.33,…

How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering…

Strongly Correlated Electrons · Physics 2015-02-27 C. J. Jia , E. A. Nowadnick , K. Wohlfeld , Y. F. Kung , C. -C. Chen , S. Johnston , T. Tohyama , B. Moritz , T. P. Devereaux

Taking spinon excitations in the quantum antiferromagnet CaCu2O3 as an example, we demonstrate that femtosecond dynamics of magnetic excitations can be probed by direct resonant inelastic x-ray scattering (RIXS). To this end, we isolate the…

Resonant inelastic X-ray scattering (RIXS) is a powerful probe of elementary excitations in solids. It is now widely applied to study magnetic excitations. However, its complex cross-section means that RIXS has been more difficult to…

Strongly Correlated Electrons · Physics 2021-06-30 H. C. Robarts , M. Garcia-Fernandez , J. Li , A. Nag , A. C. Walters , N. E. Headings , S. M. Hayden , Ke-Jin Zhou

Recent experiments show that indirect resonant inelastic X-ray scattering (RIXS) is a new probe of spin dynamics. Here I derive the cross-section for magnetic RIXS and determine the momentum dependent four-spin correlation function that it…

Strongly Correlated Electrons · Physics 2015-06-25 Jeroen van den Brink

Using resonant inelastic x-ray scattering (RIXS) at the Cu $L$-absorption edge, we have observed intense, dispersive spin excitations in highly overdoped Tl$_2$Ba$_2$CuO$_{6+\delta}$ (superconducting $T_c =6$ K), a compound whose…

We propose that resonant inelastic X-ray scattering (RIXS) is an effective probe of the fractionalized excitations in three-dimensional (3D) Kitaev spin liquids. While the non-spin-conserving RIXS responses are dominated by the gauge-flux…

Strongly Correlated Electrons · Physics 2017-09-06 Gábor B. Halász , Brent Perreault , Natalia B. Perkins

Resonant inelastic X-ray scattering (RIXS) at the $L$-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the $K$-edge of…

We study the magnetic excitation spectra in L-edge resonant inelastic x-ray scattering (RIXS) from undoped cuprates. We analyze the second-order dipole allowed process that the strong perturbation works through the intermediate state in…

Strongly Correlated Electrons · Physics 2013-05-30 Jun-ichi Igarashi , Tatsuya Nagao

Low-energy electron excitation spectra were measured on a single crystal of a typical iron-based superconductor PrFeAsO$_{0.7}$ using resonant inelastic X-ray scattering (RIXS) at the Fe-$L_3$ edge. Characteristic RIXS features are clearly…

Strongly Correlated Electrons · Physics 2016-07-18 T. Nomura , Y. Harada , H. Niwa , K. Ishii , M. Ishikado , S. Shamoto , I. Jarrige

Magnetic excitations in the optimally doped high-$T_\mathrm{c}$ superconductor Bi$_{1.5}$Pb$_{0.55}$Sr$_{1.6}$La$_{0.4}$CuO$_{6+\delta}$ (OP-Bi2201, $T_\mathrm{c}\simeq 34$ K) are investigated by Cu $L_3$ edge resonant inelastic x-ray…

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