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Changes in atomic coordination numbers at high pressures are fundamental to condensed-matter physics because they initiate the emergence of unexpected structures and phenomena. Silicon is capable of forming eight-, nine-, and…

Materials Science · Physics 2021-07-08 Shicong Ding , Pan Zhang , Kang Yang , Cailong Liu , Jian Hao , Wenwen Cui , Jingming Shi , Yinwei Li

Density functional theory calculations have been used to identify stable layered Li-$M$-B crystal structure phases derived from a recently proposed binary metal-sandwich (MS) lithium monoboride superconductor. We show that the MS lithium…

Superconductivity · Physics 2009-11-13 Aleksey N. Kolmogorov , Matteo Calandra , Stefano Curtarolo

We report the theoretical prediction of two high-performing hydride superconductors BaSiH$_8$ and SrSiH$_8$. They are thermodynamically stable above pressures of $130$ and $174\,\text{GPa}$, respectively, and metastable below that.…

Superconductivity · Physics 2022-05-31 Roman Lucrezi , Simone Di Cataldo , Wolfgang von der Linden , Lilia Boeri , Christoph Heil

Binary hydrides formed by the pnictogens of phosphorus, arsenic and antimony are studied at high pressures using first principles methods. Stable structures are predicted and their electronic, vibrational and superconducting properties are…

Ternary hydrides have emerged as the primary focus of the new wave of research into superconducting hydrides. In this work, Mg-Ti-H ternary hydrides are explored under high pressures up to 300 GPa using the prediction method of the particle…

Materials Science · Physics 2026-02-10 Pan Min , Wang Yujie , Hu Kaige , Deng Huiqiu

We review five years of experimental and theoretical attempts (2020-2025) to enhance the superconducting critical temperature ($\textit{T$_c$}$) of hydrogen-rich compounds by alloying binary superhydrides with additional elements. Despite…

We report an ab-initio study of the stability and electronic properties of transition metal silicides in order to study their potential for high temperature thermoelectric applications. We focus on the family M5Si3 (M = Ta, W) which is…

Materials Science · Physics 2015-06-03 P. Jund , X. Tao , R. Viennois , C. Colinet , J. -C. Tedenac

The discovery of high-temperature superconductivity above 240 K in binary La-H and Y-H systems inspired further predictions of even higher transition temperatures in compounds such as YH10 and MgH6, which are likely to be dynamically…

Exploring high-temperature superconducting (high-$T_c$) material at ambient pressure holds immense significance for physics, chemistry, and materials science. In this study, we perform a high-throughput screening of strong electron-phonon…

Ternary or more complex hydrogen-rich hydrides are the main hope of reaching room-temperature superconductivity at high pressures. Their chemical space is vast and its exploration is challenging. Here we report the investigation of the…

Superconductivity · Physics 2023-12-13 Grigoriy Shutov , Dmitrii Semenok , Ivan A. Kruglov , Artem R. Oganov

We investigate the high-pressure behaviour of beryllium, magnesium and calcium difluorides using ab initio random structure searching and density functional theory (DFT) calculations, over the pressure range 0-70 GPa. Beryllium fluoride…

Materials Science · Physics 2017-03-01 J. R. Nelson , R. J. Needs , C. J. Pickard

It is well known that pressure causes profound changes in the properties of atoms and chemical bonding, leading to the formation of many unusual materials. Here we systematically explore all stable calcium carbides at pressures from ambient…

Materials Science · Physics 2015-05-14 Yan-Ling Li , Sheng-Nan Wang , Artem R. Oganov , Huiyang Gou , Jesse S. Smith , Timothy A. Strobel

Manganese nitrides should be with amazing properties and promised application, because manganese atom is particular for its magnetism, valence states, high electron density, etc., and N atoms in compounds form different substructures. It is…

Materials Science · Physics 2021-11-04 Li Li , Kuo Bao , Xingbin Zhao , Tian Cui

In this work, global search for crystal structures of ternary Mg-Sc-H hydrides (Mg$_x$Sc$_y$H$_z$) under high pressure ($100 \le P \le 200$ GPa) were performed using the evolutionary algorithm and first-principles calculations. Based on…

Motivated by advances in hydrogen-rich superconductors in the past decades, we conducted variable-composition structural searches in Mo-H binary system at high pressure. A new composition-pressure phase diagram of thermodynamically stable…

Superconductivity · Physics 2024-01-31 Aiqin Yang , Xiangru Tao , Yundi Quan , Peng Zhang

Only several compounds bearing Ag(II) cation and other transition metal cation have been known. Herein, we predict stability and crystal structures of hypothetical ternary silver(II) fluorides with copper, nickel and cobalt in 1:1…

Materials Science · Physics 2021-07-29 Mateusz A. Domański , Mariana Derzsi , Wojciech Grochala

We present a theoretical investigation, based on ab initio calculations and the quasi-harmonic approximation, on the stability properties of magnesium (MgCO$_3$) and calcium (CaCO$_3$) carbonates at high temperatures and pressures. The…

Materials Science · Physics 2018-11-20 Samuel S. M. Santos , Michel L. Marcondes , João F. Justo , Lucy V. C. Assali

Solid hydrogen sulfide is well known as a typical molecular crystal but its stability under pressure is still under debate. Particularly, Eremets et al. found the high pressure superconductivity with $T_{c}\approx$ 190 K in a H$_{2}$S…

Superconductivity · Physics 2015-05-20 Defang Duan , Xiaoli Huang , Fubo Tian , Da Li , Hongyu , Yu , Yunxian Liu , Yanbin Ma , Bingbing Liu , Tian Cui

The stability of different stoichiometric H$_n$Br ($n$=1-7) compounds under pressure are extensively studied using density functional theory calculations. Five new energetically stable stoichiometries of H$_2$Br, H$_3$Br, H$_4$Br, H$_5$Br,…

Superconductivity · Physics 2015-04-07 Defang Duan , Fubo Tian , Xiaoli Huang , Da Li , Hongyu Yu , Yunxian Liu , Yanbin Ma , Bingbing Liu , Tian Cui

High-pressure hydrogen-rich compounds have long been regarded as promising room-temperature superconductor candidates; however, their practical applications are limited by their reliance on extreme compression. This study explores…

Superconductivity · Physics 2026-02-04 Qun Wei , Xinyu Wang , Jing Luo , Meiguang Zhang , Bing Wei