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Nuclear magnetic resonance (NMR), neutron diffaction (ND), x-ray diffraction, magnetic susceptibility and specific heat measurements on the frustrated A-site spinel CoAl2O4 compound reveal a collinear antiferromagnetic ordering below Tn =…

Strongly Correlated Electrons · Physics 2016-11-26 B. Roy , Abhishek Pandey , Q. Zhang , T. W. Heitmann , D. Vaknin , D. C. Johnston , Y. Furukawa

We have identified TbOF as a unique frustrated and mixed-anion lattice, hosting unconventional magnetism. By means of magnetization, specific heat and neutron diffraction measurements down to 90 mK, as well as DFT calculations, we present a…

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

High resolution time-of-flight neutron scattering measurements on Tb2Ti2O7 reveal a rich low temperature phase diagram in the presence of a magnetic field applied along [110]. In zero field at T=0.4 K, terbium titanate is a highly…

The thermal equilibrium properties of the spin-ice material DTO, including specific heat, magnetization, and spin correlations, could be successfully reproduced by a model featuring magnetic interactions up to the third nearest neighbor and…

Strongly Correlated Electrons · Physics 2025-04-14 Mariano Marziali Bermudez , R. A. Borzi , D. A. Tennant , S. A. Grigera

Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…

Statistical Mechanics · Physics 2016-01-19 P. Henelius , T. Lin , M. Enjalran , Z. Hao , J. G. Rau , J. Altosaar , F. Flicker , T. Yavors'kii , M. J. P. Gingras

We present results from muon spin relaxation/rotation, magnetization, neutron scattering and transport measurements on polycrystalline samples of the pyrochlore iridates Y2Ir2O7 (Y-227) and Yb2Ir2O7 (Yb-227). Well-defined spontaneous…

Strongly Correlated Electrons · Physics 2012-08-08 S. M. Disseler , Chetan Dhital , A. Amato , S. R. Giblin , Clarina de la Cruz , Stephen D. Wilson , M. J. Graf

Gd2GaSbO7 and Gd2InSbO7 pyrochlore compounds exhibit quantum fluctuations in a spin ice-like state. These compounds have not been adequately studied based on the concept of magnetic frustration. Here, we have synthesised and characterised…

Strongly Correlated Electrons · Physics 2024-08-06 S. Nallamuthu , Andrea Dzubinska , K. Arun , Vimaljith A. R , Marian Reiffers , R. Nagalakshmi , Ivan Curlik , Sergej Ilkovic

Dy2Ti2O7 is a geometrically frustrated magnetic material with a strongly correlated spin ice regime that extends from 1 K down to as low as 60 mK. The diffuse elastic neutron scattering intensities in the spin ice regime can be remarkably…

Statistical Mechanics · Physics 2008-08-02 Taras Yavors'kii , Tom Fennell , Michel J. P. Gingras , Steven T. Bramwell

When the transition temperature of a continuous phase transition is tuned to absolute zero, new ordered phases and physical behaviour emerge in the vicinity of the resulting quantum critical point. Sr3Ru2O7 can be tuned through quantum…

Strongly Correlated Electrons · Physics 2021-10-25 C. Lester , S. Ramos , R. S. Perry , T. P. Croft , M. Laver , R. I. Bewley , T. Guidi , A. Hiess , A. Wildes , E. M. Forgan , S. M. Hayden

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

The pyrochlore Ho2Ge2O7 is a new highly correlated spin ice material. Physical property measurements including x-ray diffraction, dc susceptibility and ac susceptibility, confirm that it shares the distinctive characteristics of other known…

The structural and magnetic properties of the face-centered cubic double perovskite Ba2MnWO6 were investigated using neutron powder diffraction, DC-magnetometry, muon spin relaxation and inelastic neutron scattering. Ba2MnWO6 undergoes Type…

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

Strongly Correlated Electrons · Physics 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

A new pyrochlore compound, NaCaNi$_2$F$_7$, was recently synthesized and has a single magnetic site with spin-1 Ni$^{2+}$. We present zero field (ZF) and longitudinal field (LF) muon spin rotation ($\mu$SR) measurements on this pyrochlore.…

Strongly Correlated Electrons · Physics 2018-09-26 Y. Cai , M. N. Wilson , A. M. Hallas , L. Liu , B. A. Frandsen , S. R. Dunsiger , J. W. Krizan , R. J. Cava , Y. J. Uemura , O. Rubel , G. M. Luke

We report a quasi-one-dimensional S = 1 spin chain compound BaNiTe2O7. This magnetic system has been investigated by magnetic susceptibility, specific heat, and neutron powder diffraction. These results indicate that BaNiTe2O7 develops a…

Specific heat and muon spin rotation and relaxation data are presented for two geometrically frustrated systems: Gd2Ti2O7 which antiferromagnetically orders and Yb2Ti2O7 which presents dynamical short range correlations at low temperature.…

Strongly Correlated Electrons · Physics 2009-11-11 P. Dalmas de Reotier , V. Glazkov , C. Marin , A. Yaouanc , P. C. M. Gubbens , S. Sakarya , P. Bonville , A. Amato , C. Baines , P. J. C. King

Magnetic properties of a one-dimensional frustrated quantum spin system Rb2Cu2Mo3O12 is investigated by the muon spin relaxation (muSR) technique. Although this system shows an incommensurate spin correlation in neutron scattering, it has…

Strongly Correlated Electrons · Physics 2018-04-04 Seiko Ohira-Kawamura , Keisuke Tomiyasu , Akihiro Koda , Dita P. Sari , Retno Asih , Sungwon Yoon , Isao Watanabe , Kenji Nakajima

In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner