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We examine the high-frequency optical mode of {\alpha}-Fe2O3 and report that Dzyaloshinskii-Moriya (DM) interaction generates a new type of torque on the magnetic resonance. Using a continuous-wave terahertz interferometer, we measure the…

Materials Science · Physics 2023-07-11 Qiyao Liu , Taeheon Kim , Kyusup Lee , Dongsheng Yang , Dushyant Kumar , Fanrui Hu , Hyunsoo Yang

The ultrafast switching of magnetization in multiferroic materials by a femtosecond laser could provide various advantages in photonics and magnonics. An efficient approach to control the light matter interaction is the modulation of…

We demonstrate a new approach for directly measuring the ultrafast energy transfer between elec- trons and magnons, enabling us to track spin dynamics in an antiferromagnet (AFM). In multiferroic HoMnO3, optical photoexcitation creates hot…

Strongly Correlated Electrons · Physics 2016-10-05 P. Bowlan , S. A. Trugman , J. Bowlan , J. -X. Zhu , N. J. Hur , A. J. Taylor , D. A. Yarotski , R. P. Prasankumar

We present a comparative far-infrared reflection spectroscopy study of phonons, phase transitions, spin-phonon and electron-phonon interactions in isostructural multiferroic iron borates of gadolinium and terbium. The behavior of phonon…

Strongly Correlated Electrons · Physics 2016-03-02 S. A. Klimin , A. B. Kuzmenko , M. A. Kashchenko , M. N. Popova

Elastic and inelastic neutron scattering studies reveal details of the antiferromagnetic tansition and intriguing spin-dynamics in the magneto-electric effect single crystal LiMnPO$_4$. The elastic scattering studies confirm the system is…

Strongly Correlated Electrons · Physics 2015-05-13 Jiying Li , Wei Tian , Ying Chen , Jerel L. Zarestky , Jeffrey W. Lynn , David Vaknin

Magnetic order parameters in altermagnets can couple to quantized lattice vibration via both piezomagnetic and magnetoelastic effects, leading to the renormalization of phonon dispersion. Here, we demonstrate photo-induced dynamic frequency…

The spin wave excitations of the geometrically frustrated triangular lattice antiferromagnet (TLA) $\rm CuFeO_2$ have been measured using high resolution inelastic neutron scattering. Antiferromagnetic interactions up to third nearest…

Strongly Correlated Electrons · Physics 2007-10-08 F. Ye , J. A. Fernandez-Baca , R. S. Fishman , Y. Ren , H. J. Kang , Y. Qiu , T. Kimura

EuTiO3 (ETO) has recently experienced an enormous revival of interest because of its possible multiferroic properties which are currently in the focus of research. Unfortunately ETO is an unlikely candidate for enlarged multifunctionality…

Materials Science · Physics 2015-06-05 A. Bussmann-Holder , Z. Guguchia , J. Köhler , H. Keller , A. Shengelaya , A. R. Bishop

We report inelastic neutron scattering measurements of the phonon spectra in a pure powder sample of the multiferroic material BiFeO3. A high-temperature range was covered to unravel the changes in the phonon dynamics across the Neel (T_N ~…

Materials Science · Physics 2015-03-19 M. Zbiri , H. Schober , N. Choudhury , R. Mittal , S. L. Chaplot , S. J. Patwe , S. N. Achary , A. K. Tyagi

In NaNiO2, Ni3+ ions form a quasi two dimensional triangular lattice of S = 1=2 spins. The magnetic order observed below 20K has been described as an A type antiferromagnet with ferro- magnetic layers weakly coupled antiferromagnetically.…

Strongly Correlated Electrons · Physics 2009-11-11 Sophie De Brion , C. Darie , M. Hopzapfel , D. Talbayev , L. Mihaly , F. Simon , A. Janossy , G. Chouteau

We have performed extensive ab initio calculations to investigate phonon dynamics and their possible role in superconductivity in BaFe2As2 and related systems. The calculations are compared to inelastic neutron scattering data that offer…

Superconductivity · Physics 2009-11-13 M. Zbiri , H. Schober , M. R. Johnson , S. Rols , R. Mittal , Y. Su , M. Rotter , D. Johrendt

Electron-phonon interaction in copper oxide superconductors is still enigmatic. Strong coupling for certain optic phonons is now well established experimentally, but theoretical understanding is challenging. Scattering of electrons near the…

Superconductivity · Physics 2019-10-14 A. M. Merritt , J. -P. Castellan , T. Keller , S. R. Park , J. A. Fernandez-Baca , G. D. Gu , D. Reznik

The present work reports the preparation of polycrystalline multiferroic $GdFeO_3$ (GdFO) and characterization with x-ray diffraction (XRD), magnetization, temperature dependent Raman spectroscopy, temperature and magnetic field dependent…

Materials Science · Physics 2021-12-06 Anjali Panchwanee , V. Raghavendra Reddy , Ajay Gupta , V. G. Sathe

We have measured near normal incidence far infrared (FIR) reflectivity spectra of a single crystal of TbMnO3 from 10K to 300K in the spectral range of 50 cm$^{-1}$ to 700 cm$^{-1}$. Fifteen transverse optic (TO) and longitudinal optic (LO)…

Materials Science · Physics 2015-05-13 Pradeep Kumar , Surajit Saha , C. R. Serrao , A. K. Sood , C. N. R. Rao

Using a combination of first-principles and magnetization-dynamics calculations, we study the effect of the intense optical excitation of phonons on the magnetic behavior in insulating magnetic materials. Taking the prototypical…

Strongly Correlated Electrons · Physics 2018-06-13 M. Fechner , A. Sukhov , L. Chotorlishvili , C. Kenel , J. Berakdar , N. A. Spaldin

Inelastic neutron scattering experiments were performed on single crystals of the heavy-fermion compound CeIn$_{3}$ for temperatures below and above the N\'eel temperature, $T_N$. In the antiferromagnetically ordered phase, well-defined…

Strongly Correlated Electrons · Physics 2009-11-10 W. Knafo , S. Raymond , B. Fak , G. Lapertot , P. C. Canfield , J. Flouquet

Spin and lattice dynamics of CaMn7O12 ceramics were investigated using infrared, THz and inelastic neutron scattering (INS) spectroscopies in the temperature range 2 to 590 K, and, at low temperatures, in applied magnetic fields of up to 12…

We present time-of-flight inelastic neutron scattering measurements of $La_{1.965}Ba_{0.035}CuO_{4}$ (LBCO), a lightly doped member of the high temperature superconducting La-based cuprate family. By using time-of-flight neutron…

Superconductivity · Physics 2015-09-30 J. J. Wagman , D. Parshall , M. B. Stone , A. T. Savici , Y. Zhao , H. A. Dabkowska , B. D. Gaulin

A neutron scattering study of the Mott-Hubbard insulator LaTiO$_{3}$ (T$_{{\rm N}}=132$ K) reveals a spin wave spectrum that is well described by a nearest-neighbor superexchange constant $J=15.5$ meV and a small Dzyaloshinskii-Moriya…

Strongly Correlated Electrons · Physics 2009-10-31 B. Keimer , D. Casa , A. Ivanov , J. W. Lynn , M. v. Zimmermann , J. P. Hill , D. Gibbs , Y. Taguchi , Y. Tokura

We have investigated spin-wave excitations in a four-sublattice (4SL) magnetic ground state of a frustrated magnet CuFeO2, in which `electromagnon' (electric-field-active magnon) excitation has been discovered by recent terahertz…

Strongly Correlated Electrons · Physics 2015-05-30 Taro Nakajima , Azusa Suno , Setsuo Mitsuda , Noriki Terada , Shojiro Kimura , Koji Kaneko , Hiroki Yamauchi