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Related papers: Comparative study of DFT+$U$ functionals for non-c…

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The magnetic ground state of FeRh is highly sensitive towards the lattice constant. This, in addition to partially filled d-shells of Fe and Rh, posed a significant challenge for Density Functional Theory (DFT) calculations in the past.…

Materials Science · Physics 2024-01-24 Shishir Kumar Pandey , Saikat Debnath , Zhanghao Zhouyina , Qiangqiang Gu

A nonlocal Landau-type free energy functional of the spin density is developed to model the large variety of magnetic states which occur in the magnetic field-temperature phase diagram of magnetoelectric CuFeO$_2$. Competition among…

Statistical Mechanics · Physics 2009-11-13 M. L. Plumer

Noncollinear magnets are notoriously difficult to describe within first-principles approaches based on density-functional theory (DFT) because of the presence of low-lying spin excitations. At the level of ground-state calculations, several…

Materials Science · Physics 2026-03-09 Miquel Royo , Massimiliano Stengel

A combination of small-cluster exact-diagonalization calculations and a well-controlled approximative method is used to study the ground-state phase diagram of the spin-one-half Falicov-Kimball model extended by the spin-dependent on-site…

Strongly Correlated Electrons · Physics 2009-11-11 Pavol Farkasovsky , Hana Cencarikova

We investigate the DFT+U approach as a viable solution to describe the low-lying states of ligated and unligated iron heme complexes. Besides their central role in organometallic chemistry, these compounds represent a paradigmatic case…

Soft Condensed Matter · Physics 2007-05-23 Damian A. Scherlis , Matteo Cococcioni , Patrick Sit , Nicola Marzari

Accurate modeling of spin-orbit coupling and noncollinear magnetism requires noncollinear density functionals within the two-component generalized Kohn-Sham (GKS) framework, yet constructing and implementing noncollinear functionals remains…

Materials Science · Physics 2025-11-26 Xiaoyu Zhang , Taoni Bao

Theoretical and experimental investigation of the electronic and magnetic structure of transition metal atoms on an insulating interface with a metallic substrate at low temperatures is quite challenging. In this paper, we show a density…

Motivated by recent experiments on volborthite single crystals showing a wide 1/3-magnetization plateau, we perform microscopic modeling by means of density functional theory (DFT) with the single-crystal structural data as a starting…

Strongly Correlated Electrons · Physics 2016-07-14 O. Janson , S. Furukawa , T. Momoi , P. Sindzingre , J. Richter , K. Held

Clarifying the origin of nematic state in FeSe is one of urgent problems in the field of iron-based superconductivity. Motivated by the discovery of a nematic solution in the density-functional theory implemented by on-site Coulomb…

Strongly Correlated Electrons · Physics 2021-10-14 Takemi Yamada , Takami Tohyama

We present in full detail a newly developed formalism enabling density functional perturbation theory (DFPT) calculations from a DFT+$U$ ground state. The implementation includes ultrasoft pseudopotentials and is valid for both insulating…

Strongly Correlated Electrons · Physics 2020-02-21 Andrea Floris , Iurii Timrov , Burak Himmetoglu , Nicola Marzari , Stefano de Gironcoli , Matteo Cococcioni

The on-site Coulomb potential, U, and the covalent state of electronic orbitals play key roles for the Cooper pair symmetry and exotic electromagnetic properties of high-Tc superconducting cuprates. In this paper, we demonstrate a way to…

The electronic and magnetic properties of neutral substitutional transition-metal dopants in dia- mond are calculated within density functional theory using the generalized gradient approximation to the exchange-correlation potential. Ti…

Materials Science · Physics 2015-06-03 Thomas Chanier , Craig Pryor , Michael E. Flatte'

The thickness dependence of spin-orbit torque and magnetoresistance in ferromagnet/heavy-metal bilayers is studied using the first-principles non-equilibrium Green's function formalism combined with the Anderson disorder model. A systematic…

Mesoscale and Nanoscale Physics · Physics 2020-01-22 K. D. Belashchenko , Alexey A. Kovalev , M. van Schilfgaarde

The inverse spinels CoFe2O4 and NiFe2O4, which have been of particular interest over the past few years as building blocks of artificial multiferroic heterostructures and as possible spin-filter materials, are investigated by means of…

Materials Science · Physics 2015-05-19 Daniel Fritsch , Claude Ederer

Density functional theory (DFT), including its extensions designed to treat strongly correlated localized electron systems such as DFT+$U$ and DFT+dynamical mean field theory, has proven exceedingly useful in studying the magnetic…

Materials Science · Physics 2025-06-09 Y. Lee , Z. Ning , R. Flint , R. J. McQueeney , I. I. Mazin , Liqin Ke

The description of the molecular solid phase of O$_2$, especially its ground-state antiferromagnetic insulating phase, is known to be quite unsatisfactory within the conventional local and semilocal density functional approximations used in…

Materials Science · Physics 2017-12-18 Shusuke Kasamatsu , Takeo Kato , Osamu Sugino

Accurately modeling compounds with partially filled $d$ and $f$ shells remains a hard challenge for density-functional theory, due to large self-interaction errors stemming from local or semi-local exchange-correlation functionals. Hubbard…

Materials Science · Physics 2026-01-19 Kinga Warda , Eric Macke , Iurii Timrov , Lucio Colombi Ciacchi , Piotr M. Kowalski

We present a theoretical investigation of epitaxial strain effects on the magnetic fluctuation properties of Mn$_3$Sn noncollinear antiferromagnets. Employing density functional theory (DFT), we uncover significant strain-induced…

Materials Science · Physics 2025-07-31 Mohammad M. Rahman , Farzad Mahfouzi , Matthew W. Daniels , Mark D. Stiles

We analyze the various approaches to construct exchange-correlation functionals which are able to describe states of definite spin multiplicity in the DFT realm and outline the characteristics of possible functionals consistent with the…

Chemical Physics · Physics 2019-01-04 A. L. Tchougréeff , J. G. Ángyán

We present a detailed mean-field study to address the fundamental discrepancy in the ground state magnetization of $\mathrm{Sr_{2}CoO_{4}}$ (SCO). In contrast to the ferromagnetic metallic ground state obtained from density functional…

Strongly Correlated Electrons · Physics 2024-01-11 Shivani Bhardwaj , Sudhir K. Pandey