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In this work, we provide a method which allows to compute exactly the multipoint and multi-time correlation functions of a one-dimensional stochastic model of dimer adsorption-evaporation with random (uncorrelated) initial states. In…

Statistical Mechanics · Physics 2016-08-31 Mauro Mobilia

A formula is derived for stiffness of a polymer chain in terms of the distribution function of end-to-end vectors. This relationship is applied to calculate the stiffness of Gaussian chains (neutral and carrying electric charges at the…

Statistical Mechanics · Physics 2007-05-23 A. D. Drozdov

Using Poisson-Boltzmann equation and linear response theory, we derive an effective interaction potential due to a fixed charge distribution in a solution containing polyelectrolytes and point salt. We obtain an expression for the effective…

Soft Condensed Matter · Physics 2016-01-08 Sandipan Dutta , and Y. S. Jho

We consider the increase of the spatial variance of some inhomogeneous, non-equilibrium density (particles, energy, etc.) in a periodic quantum system of condensed matter-type. This is done for a certain class of initial quantum states…

Statistical Mechanics · Physics 2009-10-23 Robin Steinigeweg , Hannu Wichterich , Jochen Gemmer

The endpoint distribution and dynamics of semiflexible fibers is studied by numerical simulation. A brief overview is given over the analytical theory of flexible and semiflexible polymers. In particular, a closed expression is given for…

Soft Condensed Matter · Physics 2013-06-13 Robert D. Groot

We study the autocorrelation function of different types of eigenfunctions in quantum mechanical systems with either chaotic or mixed classical limits. We obtain an expansion of the autocorrelation function in terms of the correlation…

Chaotic Dynamics · Physics 2009-11-07 Arnd Bäcker , Roman Schubert

Using a continuum description, we account for fluctuations in the ionic solvent surrounding a Gaussian, charged chain and derive an effective short-ranged potential between the charges on the chain. This potential is repulsive at short…

Soft Condensed Matter · Physics 2009-11-10 Shirish M. Chitanvis

A microscopic theory for cation diffusion in polymer electrolytes is presented. Based on a thorough analysis of molecular dynamics simulations on PEO with LiBF$_4$ the mechanisms of cation dynamics are characterised. Cation jumps between…

Soft Condensed Matter · Physics 2009-11-13 A. Maitra , A. Heuer

We study the interplay of intrinsic-electronic and environmental factors on long-range charge transport across molecular chains with up to $N\sim 80$ monomers. We describe the molecular electronic structure of the chain with a tight-binding…

Mesoscale and Nanoscale Physics · Physics 2022-09-21 Francisco Lai Liang , Dvira Segal

Within Kirkwood theory, we study the translational diffusion coefficient of a single polymer chain in dilute solution, and focus on the small difference between the short--time Kirkwood value $D^{(K)}$ and the asymptotic long--time value…

Soft Condensed Matter · Physics 2009-11-10 Bo Liu , Burkhard Duenweg

After a brief review of previous work, two exactly solvable two-dimensional models of a finite Coulomb fluid in a disc are studied. The charge correlation function near the boundary circle is computed. When the disc radius is large compared…

Statistical Mechanics · Physics 2009-11-07 B. Jancovici

A numerical method is proposed to remove the quenched randomness from a data sequence of numbers. A polymer chain of beads is introduced with both a hard core interaction and an appropriate energy associated with the data sequence. The…

Soft Condensed Matter · Physics 2024-11-11 Theo Odijk

We consider an inextensible, semiflexible polymer or worm-like chain which is confined in the transverse direction by a parabolic potential and subject to a longitudinal force at the ends, so that the polymer is stretched out and…

Soft Condensed Matter · Physics 2015-05-28 Theodore W. Burkhardt

In this paper we show how an infinite system of coupled Toda-type nonlinear differential equations derived by one of us can be used efficiently to calculate the time-dependent pair-correlations in the Ising chain in a transverse field. The…

Statistical Mechanics · Physics 2015-05-13 Jacques H. H. Perk , Helen Au-Yang

We study the dynamics and conformation of polymers composed by active monomers. By means of Brownian dynamics simulations we show that when the direction of the self-propulsion of each monomer is aligned with the backbone, the polymer…

Soft Condensed Matter · Physics 2018-11-28 Valentino Bianco , Emanuele Locatelli , Paolo Malgaretti

We investigate the length distribution of self-assembled, long and stiff polymers at thermal equilibrium. Our analysis is based on calculating the partition functions of stiff polymers of variable lengths in the elastic regime. Our…

Soft Condensed Matter · Physics 2012-09-06 Chiu Fan Lee

We investigate the Rubinstein-Duke model for polymer reptation by means of density-matrix renormalization group techniques both in absence and presence of a driving field. In the former case the renewal time \tau and the diffusion…

Statistical Mechanics · Physics 2009-11-07 Enrico Carlon , Andrzej Drzewinski , J. M. J. van Leeuwen

Polymer entanglements lead to complicated topological constraints and interactions between neighbouring chains in a dense solution or melt. Entanglements can be treated in a mean field approach, within the famous reptation model, since they…

Soft Condensed Matter · Physics 2007-05-23 S. Kutter , E. M. Terentjev

We present data of Monte Carlo simulations for monodisperse linear polymer chains in dense melts with degrees of polymerization between N=16 and N=512. The aim of this study is to investigate the crossover from Rouse-like dynamics for short…

Soft Condensed Matter · Physics 2009-10-31 T. Kreer , J. Baschnagel , M. Mueller , K. Binder

Theoretical considerations based on chain connectivity and conformational variability of polymers have lead to an uncomplicated relation for the dependence of the Flory-Huggins interaction parameter, chi, on the volume fraction of the…

Soft Condensed Matter · Physics 2015-06-24 A. Schneider , N. Schuld , M. Bercea , B. A. Wolf