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We present a microscopic picture rationalizing the surprisingly steep decrease of the band gap with temperature in insulators, crystalline or otherwise. The gap narrowing largely results from fluctuations of long-wavelength optical…

Materials Science · Physics 2019-07-24 Vassiliy Lubchenko , Arkady Kurnosov

Optical and Hall-effect measurements have been performed on single crystals of Pb$_{0.77}$Sn$_{0.23}$Se, a IV-VI mixed chalcogenide. The temperature dependent (10--300 K) reflectance was measured over 40--7000 cm$^{-1}$ (5--870 meV) with an…

Strongly Correlated Electrons · Physics 2014-12-31 Naween Anand , Zhiguo Chen , Sanal Buvaev , Kamal Choudhary , C. Martin , Genda Gu , S. B. Sinnott , Zhiqiang Li , A. F. Hebard , D. B. Tanner

Surface electronic properties of undoped hydrogen terminated diamond covered with adsorbates or in electrolyte solutions are summarized. The formation of a conductive layer at the surface of diamond is discussed based on Hall effect,…

Materials Science · Physics 2020-05-11 Christoph E. Nebel

We have derived algebraic, analytic expressions for the chemical potential without any restriction on temperature for all types of doped, or extrinsic, gapped Dirac cone materials including gapped graphene, silicene, germanene and…

Mesoscale and Nanoscale Physics · Physics 2017-07-28 Andrii Iurov , Godfrey Gumbs , Danhong Huang , Ganesh Balakrishnan

We study the low temperature thermal conductivity of single-layer transition metal dichalcogenides. In the low temperature regime where heat is carried primarily through transport of electrons, thermal conductivity is linked to electrical…

Materials Science · Physics 2017-10-11 Parijat Sengupta

We use recent theoretical advances to develop a new functional form for interatomic forces in bulk silicon. The theoretical results underlying the model include a novel analysis of elastic properties for the diamond and graphitic structures…

Materials Science · Physics 2016-08-31 Martin Z. Bazant , Efthimios Kaxiras , J. F. Justo

We have investigated the finite temperature elastic properties of AlRE (RE=Y, Tb, Pr, Nd, Dy) with B2-type structures from first principles. The phonon free energy and thermal expansion is obtained from the quasiharmonic approach based on…

Materials Science · Physics 2011-11-08 Rui Wang , Shaofeng Wang , Xiaozhi Wu

We present a study of the thermodynamic and physical properties of Tl5Te3, BiTl9Te6 and SbTl9Te6 compounds by means of density functional theory based calculations. The optimized lattice constants of the compounds are in good agreement with…

Materials Science · Physics 2011-11-04 Xiaoma Taoa , Philippe Jund , Romain Viennois , Jean-Claude Tédenac

We present a general harmonic theory for the temperature dependence of phonon-renormalized properties of solids. Firstly, we formulate a perturbation theory in phonon-phonon interactions to calculate the phonon renormalization of physical…

Materials Science · Physics 2015-10-28 Bartomeu Monserrat , G. J. Conduit , R. J. Needs

Heat capacity measurements of the delta-phase stabilized alloy Pu-Al suggest that strong electron-phonon coupling is required to explain the moderate renormalization of the electronic density of states near the Fermi energy. We calculate…

Materials Science · Physics 2011-04-08 M. J. Graf , T. Lookman , J. M. Wills , D. C. Wallace , J. C. Lashley

Hard X-ray angle-resolved photoemission spectroscopy reveals significant alterations in the valence band states of EuPd$_2$Si$_2$ at a temperature $T_V$, where the Eu ions undergo a temperature-induced valence crossover from a magnetic…

The electron and phonon temperature distribution function are calculated in semiconductors. We solved the coupled one-dimensional heat-diffussion equations in the linear approximation in which the physical parameters on the sample are…

Condensed Matter · Physics 2009-10-28 G. Gonzalez de la Cruz , Yu. G. Gurevich

Heusler type compounds have long been recognized as potential thermoelectric (TE) materials. Here, the experimentally observed TE properties of Fe$_{2}$VAl are understood through electronic structure calculations in the temperature range of…

Materials Science · Physics 2022-04-20 Shamim Sk , P. Devi , Sanjay Singh , Sudhir K. Pandey

We use the quasiclassical theory of superconductivity to calculate the electronic contribution to the thermal conductivity. The theory is formulated for low temperatures when heat transport is limited by electron scattering from random…

Condensed Matter · Physics 2009-10-28 M. J. Graf , S. -K. Yip , J. A. Sauls , D. Rainer

The reliable calculation of electronic structures and understanding of electrical properties depends on an accurate model of the crystal structure. Here, we have reinvestigated the crystal structure of the high-zT thermoelectric material…

Materials Science · Physics 2018-08-14 I. Loa , S. R. Popuri , A. D. Fortes , J. W. G. Bos

The ultrathin one-dimensional sp3 diamond nanothreads (NTHs), as successfully synthesised recently, have greatly augmented the interests from the carbon community. In principle, there can exist different stable NTH structures. In this work,…

Materials Science · Physics 2018-03-20 Haifei Zhan , Gang Zhang , John M. Bell , Yuantong Gu

Phonons, the quanta of lattice vibrations, are primary heat carriers for semiconductors and dielectrics. The demand of effective phonon manipulation urgently emerges, because the thermal management is crucial for the ongoing development of…

Rutile TiO2 is a paradigmatic transition metal oxide with applications in optics, electronics, photocatalysis, etc., that are subject to pervasive electron-phonon interaction. To understand how energies of its electronic bands, and in…

Metal-halide perovskites are promising materials for future optoelectronic applications. One intriguing property, important for many applications, is the tunability of the band gap via compositional engineering. While experimental reports…

Materials Science · Physics 2019-06-27 Shuxia Tao , Ines Schmidt , Geert Brocks , Junke Jiang , Ionut Tranca , Klaus Meerholz , Selina Olthof

Motivated by recent experiments, we present here a systematic ab-initio study of the length dependence of the thermal conductance of single-molecule junctions. We make use of a combination of density functional theory with non-equilibrium…

Mesoscale and Nanoscale Physics · Physics 2016-11-30 J. C. Klöckner , M. Bürkle , J. C. Cuevas , F. Pauly