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Controlling exciton recombination in atomically thin semiconductors is central to their optoelectronic functionality, as the competition between radiative and non-radiative decay channels governs emission efficiency. Existing approaches,…

In 1H monolayer transition metal dichalcogenide, the inversion symmetry is broken, while the reflection symmetry is maintained. On the contrary, in the bilayer, the inversion symmetry is restored, but the reflection symmetry is broken. As a…

Optically dark excitonic states play a critical role in the valleytronic, electronic, and optical properties of monolayer semiconducting transition metal dichalcogenides. Here, we investigate how electrostatic doping affects the in-plane…

The optical properties of two-dimensional transition metal dichalcogenide monolayers such as MoS$_2$ or WSe$_2$ are dominated by excitons, Coulomb bound electron-hole pairs. Screening effects due the presence of hexagonal-BN surrounding…

Materials Science · Physics 2018-12-26 Iann C. Gerber , Xavier Marie

Interlayer exciton diffusion is studied in atomically-reconstructed MoSe2/WSe2 heterobilayers with suppressed disorder. Local atomic registry is confirmed by characteristic optical absorption, circularly-polarized photoluminescence, and…

In van der Waals (vdW) heterostructures formed by stacking two monolayer semiconductors, lattice mismatch or rotational misalignment introduces an in-plane moir\'e superlattice. While it is widely recognized that a moir\'e superlattice can…

The interlayer couplings in commensurate and incommensurate bilayer structures of transition metal dichalcogenides are investigated with perturbative treatment. The interlayer coupling in \pm K valleys can be decomposed into a series of…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 Yong Wang , Zhan Wang , Wang Yao , Gui-Bin Liu , Hongyi Yu

We analyze the lineshape of the quasiparticle photoluminescence of monolayer and bilayer molybdenum ditelluride in temperature- and excitation intensity-dependent experiments. We confirm the existence of a negatively charged trion in the…

Using resonant 2-photon excitation of interlayer electrons in twisted bilayer graphene (tBLG), we resolve photoluminescence (PL) that tunes spectrally with stacking angle, {\theta}. This weak signal is 4- 5$\times$ larger than the…

Mesoscale and Nanoscale Physics · Physics 2019-04-01 Hiral Patel , Lujie Huang , Cheol-Joo Kim , Jiwoong Park , Matt W. Graham

Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide (i)…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 E. Mostaani , M. Szyniszewski , C. H. Price , R. Maezono , M. Danovich , R. J. Hunt , N. D. Drummond , V. I. Fal'ko

Screening due to surrounding dielectric medium reshapes the electron-hole interaction potential and plays a pivotal role in deciding the binding energies of strongly bound exciton complexes in quantum confined monolayers of transition metal…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Garima Gupta , Sangeeth Kallatt , Kausik Majumdar

Transition metal dichalcogenide monolayers are highly interesting for potential valleytronic applications due to the coupling of spin and valley degrees of freedom and valley-selective excitonic transitions. However, ultrafast recombination…

Mesoscale and Nanoscale Physics · Physics 2017-09-05 Markus Schwemmer , Philipp Nagler , Andreas Hanninger , Christian Schüller , Tobias Korn

Moir\'e heterostructures are rapidly emerging as a tunable platform to study correlated electronic phenomena. Discovery of exotic quantum phases in moir\'e systems requires novel probes of charge and spin order. Unlike detection schemes…

Mesoscale and Nanoscale Physics · Physics 2021-11-19 Weijie Li , Luka M. Devenica , Jin Zhang , Yang Zhang , Xin Lu , Kenji Watanabe , Takashi Taniguchi , Angel Rubio , Ajit Srivastava

Motivated by the recent excitement around the physics of twisted transition metal dichalcogenide (TMD) multilayer systems, we study strongly correlated phases of TMD heterobilayers under the influence of light. We consider both waveguide…

Strongly Correlated Electrons · Physics 2022-12-20 Michael Vogl , Swati Chaudhary , Gregory A. Fiete

We combine linear and non-linear optical spectroscopy at 4K with ab initio calculations to study the electronic bandstructure of MoSe2 monolayers. In 1-photon photoluminescence excitation (PLE) and reflectivity we measure a separation…

Materials Science · Physics 2015-11-05 G. Wang , I. C. Gerber , L. Bouet , D. Lagarde , A. Balocchi , M. Vidal , E. Palleau , T. Amand , X. Marie , B. Urbaszek

In commensurate twisted homobilayers, purely radial Rashba spin-orbit fields can emerge. We employ first-principles calculations to investigate the band structures and the spin-orbit fields close to the high-symmetry points $K$ and $\Gamma$…

Mesoscale and Nanoscale Physics · Physics 2026-01-30 Thomas Naimer , Paulo E. Faria Junior , Klaus Zollner , Jaroslav Fabian

Vertical and lateral heterostructures of van der Waals materials provide tremendous flexibility for band structure engineering. Since electronic bands are sensitively affected by defects, strain, and interlayer coupling, the edge and…

Controlling the charge carrier density provides an efficient way to trigger phase transitions and modulate the optoelectronic properties in natural materials. This approach could be used to induce topological transitions in the optical…

We study exciton energy spectrum and their propagation in moir\'e superlattices formed in transition metal dichalcogenide heterobilayers. In such structures, as a result of weak interlayer interaction, an effective, moir\'e, potential…

Mesoscale and Nanoscale Physics · Physics 2025-01-07 A. M. Shentsev , M. M. Glazov

Twisted van der Waals heterostructures and the corresponding superlattices, moire superlattices, are remarkable new material platforms, in which electron interactions and excited-state properties can be engineered. Particularly, the band…

Mesoscale and Nanoscale Physics · Physics 2019-11-13 Xiaobo Lu , Xiaoqin Li , Li Yang