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Using a three-dimensional quasiclassical technique we explore the double ionization pathways of a diatomic molecule driven by an intense infrared (800nm) ultrashort laser pulse. For intensities corresponding to the tunneling regime, we find…

Atomic Physics · Physics 2009-02-26 Agapi Emmanouilidou

We examine a regime in which a linearly-polarized laser pulse with relativistic intensity irradiates a sub-critical plasma for much longer than the characteristic electron response time. A steady-state channel is formed in the plasma in…

Plasma Physics · Physics 2016-05-25 A. V. Arefiev , V. N. Khudik , A. P. L. Robinson , G. Shvets , L. Willingale , M. Schollmeier

Propagation of extremely short unipolar pulses of electromagnetic field ("videopulses") is considered in the framework of a model in which the material medium is represented by anharmonic oscillators (approximating bound electrons) with…

Pattern Formation and Solitons · Physics 2009-10-31 Elena Kazantseva , Andrey Maimistov , Boris Malomed

The nonlinear interaction between intense laser light and a quantum plasma is modeled by a collective Dirac equation coupled with the Maxwell equations. The model is used to study the nonlinear propagation of relativistically intense laser…

Plasma Physics · Physics 2015-05-28 Bengt Eliasson , Padma K. Shukla

In our model the electron dynamics are described by a two-state approximation. This might appear a rough approximation since it neglects coupling through excited electronic states and ionization channels. However at high intensity (laser…

Atomic Physics · Physics 2007-05-23 J F McCann , Liang-You Peng , I D Williams

An absorption of a weak pulse by two identical atoms moving in a trap is investigated. Based on atom-light interactions we present a microscopic model of a two-body wave function diagnosis. We study the influence of pulse properties on the…

Quantum Gases · Physics 2017-11-22 Rafał Ołdziejewski , Kazimierz Rzążewski

The radiative acceleration of particles and the electrostatic potential fields that arise in low density plasmas hit by radiation produced by a transient, compact source are investigated. We calculate the dynamical evolution and asymptotic…

Astrophysics · Physics 2009-11-07 L. Zampieri , R. Turolla , L. Foschini , A. Treves

We study non-linear adiabatic connection paths in density-functional theory using modified electron-electron interactions that perform a long-range/short-range separation of the Coulomb interaction. These adiabatic connections allows to…

Chemical Physics · Physics 2009-11-11 Julien Toulouse , Francois Colonna , Andreas Savin

We theoretically investigate the interaction of moderate intensity near-infrared few cycle laser pulses with nano-scale metal tips. Local field enhancement in a nanometric region around the tip apex triggers coherent electron emission on…

Mesoscale and Nanoscale Physics · Physics 2014-08-26 Georg Wachter , Christoph Lemell , Joachim Burgdoerfer

The processing of energy by transfer and redistribution plays a key role in the evolution of dynamical systems. At the ultrasmall and ultrafast scale of nanosystems, quantum coherence could in principle also play a role and has been…

We study the quantum dynamics of a two-level system driven by a pulse that starts near-resonant for small amplitudes, yielding nonadiabatic evolution, and induces an adiabatic evolution for larger amplitudes. This problem is analyzed in…

Quantum Physics · Physics 2009-11-10 L. P. Yatsenko , S. Guerin , H. R. Jauslin

The motion of electrons and ions in medium-sized rare gas clusters (1000 atoms) exposed to intense laser pulses is studied microscopically by means of classical molecular dynamics using a hierarchical tree code. Pulse parameters for optimum…

Atomic and Molecular Clusters · Physics 2007-05-23 Ulf Saalmann , Jan-Michael Rost

We consider the full driven quantum dynamics of a qubit realized as spin of electron in a one-dimensional double quantum dot with spin-orbit coupling. The driving perturbation is taken in the form of a single half-period pulse of electric…

Mesoscale and Nanoscale Physics · Physics 2010-09-28 D. V. Khomitsky , E. Ya. Sherman

The interaction of a weakly bound Rydberg electron with an electromagnetic half-cycle pulse (HCP) is described with the help of a multidimensional semiclassical treatment. This approach relates the quantum evolution of the electron to its…

Quantum Physics · Physics 2009-10-31 O. Zobay , G. Alber

We examine time-resolved X-ray diffraction from molecules in the gas phase which undergo nonadiabatic avoided-crossing dynamics involving strongly coupled electrons and nuclei. Several contributions to the signal are identified,…

Chemical Physics · Physics 2017-05-30 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…

The combined quantum electron-nuclear dynamics is often associated with the Born-Huang expansion of the molecular wave function and the appearance of nonadiabatic effects as a perturbation. On the other hand, native multicomponent…

Recent advances in strong x-ray laser techniques enable the study of nonlinear multiphoton ionization in extreme high-frequency fields. Although the stabilization regime in such fields is theoretically established, its modified properties…

Atomic Physics · Physics 2026-02-17 Aleksandr V. Boitsov , Karen Z. Hatsagortsyan , Christoph H. Keitel

Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…

Atomic Physics · Physics 2017-11-21 V. Mosert , D. Bauer

Nonadiabatic molecular dynamics is an effective method for modeling nonradiative decay in electronically excited molecules. Its accuracy depends strongly on the quality of the potential energy surfaces, and its affordability for long…

Chemical Physics · Physics 2024-10-11 Matthew R. Hennefarth , Donald G. Truhlar , Laura Gagliardi