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We present a real-time path integral theory for the rate of electron transfer reactions. Using graph theoretic techniques, the dynamics is expressed in a formally exact way as a set of integral equations. With a simple approximation for the…

chem-ph · Physics 2009-10-28 Juergen T. Stockburger , C. H. Mak

We investigate the dynamical phase evolution of Coulomb-focused electrons in strong-field ionization. We diffract the electrons with an ultrashort standing light wave to track their time-dependent phase. Our findings show that low-energy…

We present a detailed experimental and theoretical study on the relativistic non-dipole effects in strong-field atomic ionisation by near-infrared linearly-polarised few-cycle laser pulses in the intensity range 1014 -1015 W/cm2. We record…

Laser-generated plasma gratings are dynamic optical elements for the manipulation of coherent light at high intensities, beyond the damage threshold of solid-stated based materials. Their formation, evolution and final collapse require a…

Plasma Physics · Physics 2020-01-01 H. Peng , C. Riconda , M. Grech , J. -Q. Su , S. Weber

We report the first experimental demonstration that two light pulses were made motionless and interacted with each other via a medium. The interaction time is, in principle, as long as possible and a considerable efficiency can be achieved…

The uncorrelated (``sequential'') and correlated (``nonsequential'') double ionization of the H2 molecule in strong laser pulses is investigated using the tools of nonlinear dynamics. We focus on the phase-space dynamics of this system,…

Chaotic Dynamics · Physics 2009-11-30 François Mauger , Cristel Chandre , T. Uzer

Non-adiabatic molecular phenomena, arising from the breakdown of the Born-Oppenheimer approximation, govern the fate of virtually all photo-physical and photochemical processes and limit the quantum efficiency of molecules and other…

Quantum Physics · Physics 2024-05-15 N. S. Bassler , M. Reitz , R. Holzinger , A. Vibók , G. J. Halász , B. Gurlek , C. Genes

We consider the final stage of double ionization of $\rm O_2$ molecules by short linearly polarized laser pulses. The saddles of the effective adiabatic potential energy close to which simultaneous escape of electrons from a molecule takes…

Atomic Physics · Physics 2007-05-23 Jakub S. Prauzner-Bechcicki , Krzysztof Sacha , Bruno Eckhardt

The interaction between electronic and vibrational degrees of freedom is an important mechanism in nonequilibrium charge transport through molecular nanojunctions. While adiabatic polaron-type coupling has been studied in great detail, new…

Mesoscale and Nanoscale Physics · Physics 2022-06-10 Christoph Kaspar , André Erpenbeck , Jakob Bätge , Christian Schinabeck , Michael Thoss

We consider weakly ionized plasma where frequent elastic scattering of electrons on neutrals change the individual acts and the rate of electron-electron collisions significantly. In this case, the kinetics of electron thermalization is…

Plasma Physics · Physics 2021-03-31 B. Breizman , G. Stupakov , G. Vekstein

The exact nuclear time-dependent potential energy surface arises from the exact decomposition of electronic and nuclear motion, recently presented in [A. Abedi, N. T. Maitra, and E. K. U. Gross, Phys. Rev. Lett. 105, 123002 (2010)]. Such…

Chemical Physics · Physics 2015-06-16 Federica Agostini , Ali Abedi , Yasumitsu Suzuki , E. K. U. Gross

We provide theoretical investigations of the response of the Ar and H atoms to an intense elliptically polarized few-cycle laser pulse, as a function of light ellipticity. The time-dependent Schr{\"o}dinger equation describing the…

Atomic Physics · Physics 2010-04-23 M. Abu-samha , L. B. Madsen

The electron dynamics of rare gas clusters in laser fields is investigated quantum mechanically by means of time-dependent density functional theory. The mechanism of early inner and outer ionization is revealed. The formation of an…

Atomic Physics · Physics 2009-11-10 D. Bauer , A. Macchi

We present an efficient method for modeling the single and double ionization dynamics of the H$_2$ molecule in ultrashort intense laser fields. This method is based on a semi-analytical approach to calculate the time-dependent single and…

Quantum Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , Thanh-Tung Nguyen Dang , Eric Charron

The method of the envelope Hamiltonian [K. Toyota, U. Saalmann, and J. M. Rost, New J. Phys. {\bf 17}, 073005~(2015)] is applied to further study a detachment dynamics of a model negative ion in one-dimension in high-frequency regime. This…

Atomic Physics · Physics 2016-10-19 Koudai Toyota

The electron dynamics in counter-propagating laser waves is investigated by employing a novel approach, where the new Hamiltonian is time-independent when the perturbative laser wave is absent. The physical picture of stochastic electron…

Plasma Physics · Physics 2019-08-05 Yanzeng Zhang , Sergei Krasheninnikov

The angular dependence of the differential cross section of unpolarized light-by-light scattering summed over final polarizations is the same in any low-energy effective theory of quantum electrodynamics and also in Born-Infeld…

High Energy Physics - Phenomenology · Physics 2017-04-25 A. Rebhan , G. Turk

We propose a theoretical and computational approach to investigate temporal behavior of a nonlinear polarization in perturbative regime induced by an intense and ultrashort pulsed electric field. First-principles time-dependent density…

Optics · Physics 2019-03-27 Mitsuharu Uemoto , Yuki Kuwabara , Shunsuke A. Sato , Kazuhiro Yabana

Ionization by relativistically intense laser pulses of finite duration is considered in the framework of strong-field quantum electrodynamics. Our main focus is on the formation of ionization supercontinua. More specifically, when studying…

Atomic Physics · Physics 2016-07-13 K. Krajewska , J. Z. Kamiński

Electron dynamics in the bulk of large band gap dielectric crystals induced by intense femtosecond laser pulses at 800 nm is studied. With laser intensities under the ablation threshold (a few 10 TW/cm\textsuperscript{2}), electrons with…

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