Related papers: X-Ray sum frequency generation; direct imaging of …
Time-resolved ultrafast x-ray scattering is an emerging approach to probe the temporally evolving electronic charge distribution in real-space and in real-time. In this contribution, time-resolved ultrafast x-ray scattering from an…
A setup of a unique x-ray source is put forward employing a relativistic electron beam interacting with two counter-propagating laser pulses in the nonlinear few-photon regime. In contrast to Compton scattering sources, the envisaged x-ray…
The optimal properties for single photons may vary drastically between different quantum technologies. Along with central frequency conversion, control over photonic temporal waveforms will be paramount to the effective coupling of…
Streak cameras are one of the most common and convenient devices to measure pulsed emission e.g. from semiconductor lightsources with picosecond time resolution. However, they are most sensitive in the visible range and possess low or…
X-ray free electron lasers (XFELs) generate sequences of ultra-short, spatially coherent pulses of x-ray radiation. We propose the diffraction focusing spectrometer (DFS), which is able to measure the whole energy spectrum of the radiation…
Modern X-ray spectroscopy has proven itself as a robust tool for probing the electronic structure of atoms in complex environments. Despite working on energy scales that are much larger than those corresponding to nuclear motions, taking…
Understanding and controlling ultrafast non-equilibrium charge carrier dynamics is of fundamental importance in diverse fields of (quantum) science and technology. Here, we create a three-dimensional hot electron gas through two-photon…
We fine-tuned a foundational stable diffusion model using X-ray scattering images and their corresponding descriptions to generate new scientific images from given prompts. However, some of the generated images exhibit significant…
Up to now, experiments involving M\"ossbauer nuclei have been restricted to the low-excitation regime. The reason for this is the narrow spectral line width of the nuclei. This defining feature enables M\"ossbauer spectroscopy with…
Understanding the complex plasma dynamics in ultra-intense relativistic laser-solid interactions is of fundamental importance to the applications of laser plasma-based particle accelerators, creation of high energy-density matter,…
Two-color X-ray imaging with Free Electron Laser pulses offers a powerful approach for probing ultrafast structural dynamics in nanoscale systems, combining (near-)atomic spatial resolution with femtosecond temporal precision. The first…
The time-and-frequency resolved nonlinear light scattering (NLS) signals from a time evolving charge distribution of valence electrons prepared by impulsive X-ray pulses are calculated using a superoperator Green's function formalism. The…
The advent of accelerator-driven free-electron lasers (FEL) has opened new avenues for high-resolution structure determination via diffraction methods that go far beyond conventional x-ray crystallography methods. These techniques rely on…
X-ray absorption spectroscopy (XAS) is a powerful and well established technique with sensitivity to elemental and chemical composition. Despite these advantages, its implementation has not kept pace with the development of ultrafast pulsed…
Nonlinear processes lie at the heart of many technologies such as frequency converters and entangled photon sources. Historically, observation and manipulation of these processes, for instance through nanostructures, has been limited to…
We demonstrate a motion-free intensity diffraction tomography technique that enables direct inversion of 3D phase and absorption from intensity-only measurements for weakly scattering samples. We derive a novel linear forward model,…
We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are…
We introduce a phase imaging mechanism for scanning transmission electron microscopy that exploits the complementary intensity changes of transmitted disks at different scattering angles. For scanning transmission electron microscopy, this…
The nonlinear quantum interaction of a linearly polarized x-ray probe beam with a focused intense standing laser wave is studied theoretically. Because of the tight focusing of the standing laser pulse, diffraction effects arise for the…
The routine atomic-resolution structure determination of single particles is expected to have profound implications for probing the structure-function relationship in systems ranging from energy materials to biological molecules.…