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Transition metal dichalcogenide monolayers are promising candidates for exploring new electronic and optical phenomena and for realizing atomically thin optoelectronic devices. They host tightly bound electron-hole pairs (excitons) that can…

Monolayer group VI transition metal dichalcogenides have recently emerged as semiconducting alternatives to graphene in which the true two-dimensionality (2D) is expected to illuminate new semiconducting physics. Here we investigate…

Mesoscale and Nanoscale Physics · Physics 2014-03-05 Jason S Ross , Sanfeng Wu , Hongyi Yu , Nirmal J Ghimire , Aaron M Jones , Grant Aivazian , Jiaqiang Yan , David G. Mandrus , Di Xiao , Wang Yao , Xiaodong Xu

In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek

We analyze the dielectric-function spectra of low dimensional transition metal dichalcogenides (TMDCs) using a fully analytical model of the complex dielectric function that is applicable in fractional dimensional space. We extract the…

Materials Science · Physics 2018-12-04 A. Thilagam

Excitons in atomically-thin semiconductors necessarily lie close to a surface, and therefore their properties are expected to be strongly influenced by the surrounding dielectric environment. However, systematic studies exploring this role…

Mesoscale and Nanoscale Physics · Physics 2016-12-06 Andreas V. Stier , Nathan P. Wilson , Genevieve Clark , Xiaodong Xu , Scott A. Crooker

Monolayers of semiconducting transition metal dichalcogenides are a strongly emergent platform for exploring quantum phenomena in condensed matter, building novel opto-electronic devices with enhanced functionalities. Due to their atomic…

Exciton resonances in monolayer transition-metal dichalcogenides (TMDs) provide exceptionally strong light-matter interaction at room temperature. Their spectral line shape is critical in the design of a myriad of optoelectronic devices,…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Jorik van de Groep , Qitong Li , Jung-Hwan Song , Pieter G. Kik , Mark L. Brongersma

Monolayers of transition-metal dichalcogenides such as WSe2 have become increasingly attractive due to their potential in electrical and optical applications. Because the properties of these 2D systems are known to be affected by their…

The interaction between off-resonant laser pulses and excitons in monolayer transition metal dichalcogenides is attracting increasing interest as a route for the valley-selective coherent control of the exciton properties. Here, we extend…

Exciton dissociation plays a crucial role in the performance of optoelectronic devices based on two-dimensional (2D) transition metal dichalcogenides (TMDs). In this work, we investigate the effect of an in-plane electric field on the…

Materials Science · Physics 2024-10-11 Tao Zhu , Chenhang Zheng , Lei Xu , Ming Yang

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

Monolayered MoSe2 is a promising new material to investigate advanced light-matter coupling as it hosts stable and robust excitons with comparably narrow optical resonances. In this work, we investigate the evolution of the lowest lying…

Mesoscale and Nanoscale Physics · Physics 2017-03-28 N. Lundt , A. Maryński , E. Cherotchenko , A. Pant , X. Fan , G. Sęk , S. Tongay , A. V. Kavokin , S. Höfling , C. Schneider

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

The intricate interplay between optically dark and bright excitons governs the light-matter interaction in transition metal dichalcogenide monolayers. We have performed a detailed investigation of the "spin-forbidden" dark excitons in WSe2…

We present low temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field $B$ applied to monolayers of different semiconducting transition metal dichalcogenides. For…

Mesoscale and Nanoscale Physics · Physics 2017-01-18 M. R. Molas , C. Faugeras , A. O. Slobodeniuk , K. Nogajewski , M. Bartos , D. M. Basko , M. Potemski

Monolayer transition metal dichalcogenides feature Coulomb-bound electron-hole pairs (excitons) with exceptionally large binding energy and coupled spin and valley degrees of freedom. These unique attributes have been leveraged for…

Atomically thin two-dimensional crystals have revolutionized materials science. In particular, monolayer transition metal dichalcogenides promise novel optoelectronic applications, due to their direct energy gaps in the optical range. Their…

Excitons in monolayer transition metal dichalcogenide (TMD) provide a paradigm of composite Boson in 2D system. This letter reports a photoluminescence and reflectance study of excitons in monolayer molybdenum diselenide (MoSe2) with…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Ke Xiao , Tengfei Yan , Qiye Liu , Siyuan Yang , Chiming Kan , Ruihuan Duan , Zheng Liu , Xiaodong Cui

Two-dimensional excitons formed in quantum materials such as monolayer transition-metal dichalcogenides and their strong light-matter interaction have attracted unrivalled attention by the research community due to their extraordinarily…

Mesoscale and Nanoscale Physics · Physics 2018-12-31 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

The monolayers of semiconducting transition metal dichalcogenides host strongly bound excitonic complexes and are an excellent platform for exploring many-body physics. Here we demonstrate a controlled kinetic manipulation of the…

Mesoscale and Nanoscale Physics · Physics 2022-04-05 Suman Chatterjee , Sarthak Das , Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar
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