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The study of individual quantum systems in solids, for use as quantum bits (qubits) and probes of decoherence, requires protocols for their initialization, unitary manipulation, and readout. In many solid-state quantum systems, these…

Quantum sensors have attracted broad interest in the quest towards sub-micronscale NMR spectroscopy. Such sensors predominantly operate at low magnetic fields. Instead, however, for high resolution spectroscopy, the high-field regime is…

Two-dimensional Nuclear Magnetic Resonance (NMR) is essential in molecular structure determination. The Nitrogen-Vacancy (NV) center in diamond has been proposed and developed as an outstanding quantum sensor to realize NMR in nanoscale. In…

Solid-state spin defects, such as color centers in diamond, are among the most promising candidates for scalable and integrated quantum technologies. In particular, the good optical properties of silicon-vacancy centers in diamond combined…

Quantum Physics · Physics 2024-09-20 Marco Klotz , Andreas Tangemann , Alexander Kubanek

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

The nuclear spins in nanostructured semiconductors play a central role in quantum applications. The nuclear spins represent a useful resource for generating local magnetic fields but nuclear spin noise represents a major source of dephasing…

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with…

Quantum Physics · Physics 2017-03-06 Zhen-Yu Wang , Jorge Casanova , Martin B. Plenio

Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the…

Efficiently detecting and characterizing individual spins in solid-state hosts is an essential step to expand the fields of quantum sensing and quantum information processing. While selective detection and control of a few 13C nuclear spins…

Quantum Physics · Physics 2020-10-22 Hyunseok Oh , Jiwon Yun , M. H. Abobeih , Kyung-Hoon Jung , Kiho Kim , T. H. Taminiau , Dohun Kim

Nuclear spin imaging at the atomic level is essential for the understanding of fundamental biological phenomena and for applications such as drug discovery. The advent of novel nano-scale sensors has given hope of achieving the…

Quantum Physics · Physics 2015-11-25 Ashok Ajoy , Ulf Bissbort , Mikhail D. Lukin , Ronald L. Walsworth , Paola Cappellaro

Quantum registers of nuclear spins coupled to electron spins of individual solid-state defects are a promising platform for quantum information processing. Pioneering experiments selected defects with favourably located nuclear spins having…

Mesoscale and Nanoscale Physics · Physics 2014-03-17 T. H. Taminiau , J. Cramer , T. van der Sar , V. V. Dobrovitski , R. Hanson

Hybrid photoelectric detection of NV magnetic resonances (PDMR) is anticipated to lead to scalable quantum chip technology. To achieve this goal, it is crucial to prove that PDMR readout is compatible with the coherent spin control. Here we…

The sensing capability of a single optically bright electronic spin in diamond can be enhanced by making use of proximal dark nuclei as ancillary spins. Such systems, so far only realized in bulk diamond, provide orders of magnitude higher…

Quantum Physics · Physics 2017-10-04 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

Coherent manipulation of nuclear spins is a highly desirable tool for both quantum metrology and quantum computation. However, most of the current techniques to control nuclear spins lack of being fast impairing their robustness against…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 Raul Coto , Vincent Jacques , Gabriel Hétet , Jerónimo R. Maze

The ability to control and manipulate spins via electrical, magnetic and optical means has generated numerous applications in metrology and quantum information science in recent years. A promising alternative method for spin manipulation is…

Mesoscale and Nanoscale Physics · Physics 2013-04-04 Sungkun Hong , Michael S. Grinolds , Patrick Maletinsky , Ronald L. Walsworth , Mikhail D. Lukin , Amir Yacoby

We experimentally demonstrate the use of a single electronic spin to measure the quantum dynamics of distant individual nuclear spins from within a surrounding spin bath. Our technique exploits coherent control of the electron spin,…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Shimon Kolkowitz , Quirin P. Unterreithmeier , Steven D. Bennett , Mikhail D. Lukin

Nuclear spins in solid-state platforms are promising for building rotation sensors due to their long coherence times. Among these platforms, nitrogen-vacancy centers have attracted considerable attention with ambient operating conditions.…

Charged boron vacancies (V$_\text{B}^-$) in hexagonal boron nitride (hBN) have emerged as a promising platform for quantum nanoscale sensing and imaging. While these primarily involve electron spins, nuclear spins provide an additional…

The nitrogen-vacancy (NV) centre in diamond is a leading platform for nanoscale sensing and imaging, as well as quantum information processing in the solid state. To date, individual control of two NV electronic spins at the nanoscale has…

Nuclear spins in the proximity of electronic spin defects in solids are promising platforms for quantum information processing due to their ability to preserve quantum states for a remarkably long time. Here we report a comprehensive study…

Quantum Physics · Physics 2023-10-03 Mykyta Onizhuk , Giulia Galli