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We demonstrate femtosecond pump-probe transient absorption spectroscopy using a programmable dispersive filter as an ultra-fast delay line. Combined with fast synchronous detection this delay line allows for recording of 6 ps decay traces…

Optics · Physics 2018-06-22 Xavier Audier , Naveen Balla , Herve Rigneault

Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…

Atomic Physics · Physics 2023-06-06 Nickolas H. Pilgram , Arian Jadbabaie , Chandler J. Conn , Nicholas R. Hutzler

Positronium and muonium, as purely leptonic atoms without internal structure, provide ideal systems for high-precision tests of quantum electrodynamics (QED) and measurements of fundamental constants. However, the high velocities of these…

The possibility of refining the energy of the 8.36-eV 229mTh nuclear isomer -- the most likely candidate for the role of a nuclear frequency standard -- by means of resonant optical pumping is discussed. Attention is focused on considering…

Nuclear Theory · Physics 2024-03-26 F. F. Karpeshin

We simulate the transition from amplified spontaneous emission (ASE) to lasing in random systems with varying degrees of mode overlap. This is accomplished by solving the stochastic Maxwell-Bloch equations with the finite-difference…

Optics · Physics 2010-12-30 Jonathan Andreasen , Hui Cao

We report on a new optical implementation of primary gas thermometry based on laser absorption spectrometry in the near infrared. The method consists in retrieving the Doppler broadening from highly accurate observations of the line shape…

Statistical Mechanics · Physics 2009-11-13 G. Casa , A. Castrillo , G. Galzerano , R. Wehr , A. Merlone , D. Di Serafino , P. Laporta , L. Gianfrani

We put forward a first-principle NonEquilibrium Green's Function (NEGF) approach to calculate the transient photoabsorption spectrum of optically thin samples. The method can deal with pump fields of arbitrary strength, frequency and…

Atomic Physics · Physics 2015-09-30 E. Perfetto , A. -M. Uimonen , R. van Leeuwen , G. Stefanucci

Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…

Atomic Physics · Physics 2012-10-02 Nicholas R. Hutzler , Hsin-I Lu , John M. Doyle

We propose a technique that makes it possible to transform the intensity of a quasi-monochromatic single-photon wave packet, emitted by a radioactive M\"ossbauer gamma-ray source, into a sequence of short bursts with an arbitrary number of…

Optics · Physics 2024-10-22 I. R. Khairulin , Y. V. Radeonychev

Partial-transfer absorption imaging is a tool that enables optimal imaging of atomic clouds for a wide range of optical depths. In contrast to standard absorption imaging, the technique can be minimally-destructive and can be used to obtain…

Microwave-optical quantum transduction is a key enabling technology in quantum networking, but has been plagued by a formidable technical challenge. As most microwave-optical-transduction techniques rely on three-wave mixing processes, the…

A new smoothing method for the improvement on the identification and quantification of spectral functions based on the previous knowledge of the signals that are expected to be quantified, is presented. These signals are used as weighted…

Atomic Physics · Physics 2017-01-31 Leonardo Bennun

Resonance fluorescence of natural or artificial atoms constitutes a prime method for generating non-classical light. While most efforts have focused on producing single-photons, multi-photon emission is unavoidably present in the resonant…

We show that in parametrically driven systems and, more generally, in systems in coherent states, off-resonant pumping can cause a transition from a continuum energy spectrum of the system to a discrete one, and result in quantum revivals…

Quantum Physics · Physics 2009-11-06 G. S. Agarwal , J. Banerji

Existing super-resolution methods of optical imaging hold a solid place as an application in natural sciences, but many new developments allow for beating the diffraction limit in a more subtle way. One of the recently explored strategies…

Quantum Physics · Physics 2022-02-08 Mateusz Mazelanik , Adam Leszczyński , Michał Parniak

The recoil effects of spontaneous photon emissions during optical pumping of a trapped three-level atom are exactly calculated. Without resort to the Lamb-Dicke approximation, and considering arbitrary detuning and saturation of the pump…

Quantum Physics · Physics 2009-11-13 S. Wallentowitz , P. E. Toschek

We present methods which allow orders of magnitude increase in the number of modes in linear optics experiments by moving from spatial encoding to temporal encoding and using dispersion. This enables significant practical advantages for…

Quantum Physics · Physics 2016-05-17 Mihir Pant , Dirk Englund

Standard optical pump-probe methods analyze a system's temporal response to a laser pulse within sub-femtoseconds to several nanoseconds, constrained by the optical delay line's length. While resistance is a sensitive detector in various…

Instrumentation and Detectors · Physics 2024-04-26 M. I. Blumenau , A. Yu. Kuntsevich

Achieving non-reciprocal light propagation via stimuli that break time-reversal symmetry, without magneto-optics, remains a major challenge for integrated nanophotonic devices. Recently, optomechanical microsystems in which light and…

Optics · Physics 2018-02-02 Donggyu B Sohn , Seunghwi Kim , Gaurav Bahl

The last decade has witnessed a rapid advancement in laser technology, enabling the direct monitoring and control of electronic motion on its natural attosecond to sub-femtosecond timescales. Ultrafast processes are conventionally studied…

Chemical Physics · Physics 2026-05-27 Torsha Moitra