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Low-temperature spin-polarized scanning tunneling microscopy is employed to study spin transport across single Cobalt-Phathalocyanine molecules adsorbed on well characterized magnetic nanoleads. A spin-polarized electronic resonance is…

Materials Science · Physics 2014-09-25 C. Iacovita , M. V. Rastei , B. W. Heinrich , T. Brumme , J. Kortus , L. Limot , J. P. Bucher

We used the theory of finite periodic systems to explain the photoluminescence spectra dependence on the average diameter of nanocrystals embedded in oxide matrices. Because of the broad matrix band gap, the photoluminescence response is…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 C. Estrada , J. A. Gonzalez , A. Kunold , J. A Reyes-Esqueda , P. Pereyra

The combination of single photon emitters (quantum dots) and tailored metal nanoparticles with defined size and shape allows a detailed study of the interaction between light and matter. The enhanced optical near-field of the nanoparticles…

Mesoscale and Nanoscale Physics · Physics 2017-04-21 Gernot Schaffernak , Christian Gruber , Joachim R. Krenn , Markus Krug , Marija Gašparić , Martin Belitsch , Andreas Hohenau

Nanometric inclusions filled with nitrogen, located adjacent to FenN (n = 3 or 4) nanocrystals within (Ga,Fe)N layers, are identified and characterized using scanning transmission electron microscopy (STEM) and electron energy-loss…

We simulate the localized surface plasmon resonances of an Au nanoparticle within tunneling proximity of a Au substrate and demonstrate that the modes may be identified with those responsible for light emission from a scanning tunneling…

Mesoscale and Nanoscale Physics · Physics 2012-07-18 J. Mitra , Lei Feng , Michael G. Boyle , P. Dawson

Two-dimensional (2D) ferroelectric materials provide a promising platform for the electrical control of quantum states. In particular, due to their 2D nature, they are suitable for influencing the quantum states of deposited molecules via…

Space charge layers (SCLs) at grain boundaries play a crucial role in modulating local electric fields and influencing the functional properties of materials, such as oxygen vacancy migration and ionic conductivity in oxide ceramics.…

The capability to excite, probe, and manipulate vibrational modes is essential for understanding and controlling chemical reactions at the molecular level. Recent advancements in tip-enhanced Raman spectroscopies have enabled the probing of…

Sub-micrometer scale light patterns play a pivotal role in various fields, including biology, biophysics, and AMO physics. High-resolution, in situ observation of light profiles is essential for their design and application. However,…

Electric Scanning Probe Microscopies are used to characterize the surface behavior of ferroelectric materials. The effects of local charge density on the chemistry and physics of ferroelectric surfaces are investigated. The kinetics and…

Materials Science · Physics 2007-05-23 Sergei V. Kalinin , Dawn A. Bonnell

The physical properties of ultrathin NaCl overlayers on the stepped Cu(311) surface have been characterized using scanning tunneling microscopy (STM) and spectroscopy, and density functional calculations. Simulations of STM images and…

Materials Science · Physics 2009-11-10 F. E. Olsson , M. Persson , J. Repp , G. Meyer

Electrically connected and plasmonically enhanced molecular junctions combine the optical functionalities of high field confinement and enhancement (cavity function), and of high radiative efficiency (antenna function) with the electrical…

In a recent experiment by Eichmann et al., polarization-sensitive measurements of the fluorescence from two four-level ions driven by a linearly polarized laser were made. Depending on the polarization chosen, different degrees of…

Atomic Physics · Physics 2009-10-30 T. Wong , S. M. Tan , M. J. Collett , D. F. Walls

Two-dimensional crystals and their heterostructures unlock access to a class of photonic devices, bringing nanophotonics from the nanometer scale down to the atomic level where quantum effects are relevant. Single-photon emitters (SPEs) are…

Electrons in atoms and molecules move on attosecond time scales. Deciphering their quantum dynamics in space and time calls for high-resolution microscopy at this speed. While scanning tunnelling microscopy (STM) driven with terahertz…

Upon the discovery of the superatom states in endohedral metallofullerenes (EMFs), the superatom properties have become attractive, because ultrafast motion of the trapped atom modifies the charge distribution in the fullerene cage.…

Mesoscale and Nanoscale Physics · Physics 2020-10-28 Shaoqing Du , Ya Zhang , Kenji Yoshida , Kazuhiko Hirakawa

We demonstrate that nanocavity plasmons generated a few nanometers away from a molecule can induce molecular motion. For this, we study the well-known rapid shuttling motion of zinc phthalocyanine molecules adsorbed on ultrathin NaCl films…

Mesoscale and Nanoscale Physics · Physics 2021-07-07 Tzu-Chao Hung , Brian Kiraly , Julian H. Strik , Alexander A. Khajetoorians , Daniel Wegner

Scanning tunneling spectroscopy measures how a single electron with definite energy propagates between a sample surface and the tip of a scanning tunneling microscope. In the simplest description, the differential conductance measured is…

Mesoscale and Nanoscale Physics · Physics 2019-05-07 Mikko M. Ervasti , Fabian Schulz , Peter Liljeroth , Ari Harju

The analysis of the electronic surface properties of transition metal oxides being key materials for future nanoelectronics requires a direct characterization of the conductivity with highest spatial resolution. Using local conductivity…

Mesoscale and Nanoscale Physics · Physics 2021-10-15 C. Rodenbücher , G. Bihlmayer , W. Speier , J. Kubacki , M. Wojtyniak , M. Rogala , D. Wrana , F. Krok , K. Szot

Understanding the oxidation and reduction mechanisms of catalytically active transition metal nanoparticles is important to improve their application in a variety of chemical processes. In nanocatalysis the nanoparticles can undergo…

Chemical Physics · Physics 2017-05-18 Alec Lagrow , Michael Ward , David Lloyd , Pratibha Gai , Edward Boyes