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What is the correct low-energy spin Hamiltonian description of $\alpha$-RuCl$_3$? The material is a promising Kitaev spin liquid candidate, but is also known to order magnetically, the description of which necessitates additional…

Strongly Correlated Electrons · Physics 2020-01-13 Pontus Laurell , Satoshi Okamoto

$\alpha$-RuCl$_3$ has attracted enormous attention since it has been proposed as a prime candidate to study fractionalized magnetic excitations akin to Kitaev's honeycomb-lattice spin liquid. We have performed a detailed specific-heat…

Strongly Correlated Electrons · Physics 2017-07-19 A. U. B. Wolter , L. T. Corredor , L. Janssen , K. Nenkov , S. Schönecker , S. -H. Do , K. -Y. Choi , R. Albrecht , J. Hunger , T. Doert , M. Vojta , B. Büchner

Honeycomb lattice Kitaev magnets exhibit exotic magnetic properties governed by the Kitaev interaction. This study delves into $\alpha$-RuCl$_3$, a prototypical example described by effective Hamiltonians encompassing bond-dependent Kitaev…

Strongly Correlated Electrons · Physics 2025-05-29 Hamid Mosadeq , Mohammad-Hossein Zare

Fractionalized excitations are of considerable interest in recent condensed-matter physics. Fractionalization of the spin degrees of freedom into localized and itinerant Majorana fermions are predicted for the Kitaev spin liquid, an exactly…

Strongly Correlated Electrons · Physics 2019-03-18 S. Widmann , V. Tsurkan , D. A. Prishchenko , V. G. Mazurenko , A. A. Tsirlin , A. Loidl

Kitaev-type interactions between neighbouring magnetic moments emerge in the honeycomb material ${\alpha}$-RuCl3. It is debated however whether these Kitaev interactions are ferromagnetic or antiferromagnetic. With electron energy loss…

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

We have investigated the longitudinal thermal conductivity of $\alpha$-RuCl$_{3}$, the magnetic state of which is considered to be proximate to a Kitaev honeycomb model, along with the spin susceptibility and magnetic specific heat. We…

Strongly Correlated Electrons · Physics 2017-06-28 Daichi Hirobe , Masahiro Sato , Yuki Shiomi , Hidekazu Tanaka , Eiji Saitoh

The frustrated magnet $\alpha$-RuCl$_3$ constitutes a fascinating quantum material platform that harbors the intriguing Kitaev physics. However, a consensus on its intricate spin interactions and field-induced quantum phases has not been…

Strongly Correlated Electrons · Physics 2021-07-16 Han Li , Hao-Kai Zhang , Jiucai Wang , Han-Qing Wu , Yuan Gao , Dai-Wei Qu , Zheng-Xin Liu , Shou-Shu Gong , Wei Li

Mott insulators with strong spin-orbit coupling display a strongly anisotropic response to applied magnetic fields. This applies in particular to Kitaev materials, with $\alpha$-RuCl$_3$ and Na$_2$IrO$_3$ representing two important…

Strongly Correlated Electrons · Physics 2020-10-06 Eric C. Andrade , Lukas Janssen , Matthias Vojta

$\alpha$-RuCl3 is a magnetic insulator exhibiting quantum spin liquid phases possibly found in the Kitaev honeycomb model. Much of the effort towards determining Hamiltonian parameters has focused on low magnetic field ordered phases. We…

Strongly Correlated Electrons · Physics 2023-01-05 Michael J. Lawler , Kimberly A. Modic , B. J. Ramshaw

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

Topologically ordered states of matter are generically characterized by excitations with quantum number fractionalization. A prime example is the spin liquid realized in Kitaev's honeycomb-lattice compass model where spin-flip excitations…

Strongly Correlated Electrons · Physics 2018-11-12 C. Wellm , J. Zeisner , A. Alfonsov , A. U. B. Wolter , M. Roslova , A. Isaeva , T. Doert , M. Vojta , B. Büchner , V. Kataev

In RuCl$_3$, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the…

$\alpha$-RuCl$_3$ is a leading material for proximate Kitaev magnetism. We address the origin of the broad, $\Gamma$-point centered excitation continuum observed by inelastic neutron scattering at elevated temperatures in this compound.…

Materials Science · Physics 2026-02-12 Chaebin Kim , Martin Mourigal

We investigate the dynamical properties of ${\rm Na_2IrO_3}$. For five effective models proposed for ${\rm Na_2IrO_3}$, we numerically calculate dynamical structure factors (DSFs) with an exact diagonalization method. An effective model…

Strongly Correlated Electrons · Physics 2015-11-25 Takafumi Suzuki , Takuto Yamada , Youhei Yamaji , Sei-ichiro Suga

We present a spin-rotation-invariant Green-function theory for the dynamic spin susceptibility in the spin-1/2 antiferromagnetic Heisenberg model on a stacked honeycomb lattice. Employing a generalized mean-field approximation for arbitrary…

Strongly Correlated Electrons · Physics 2017-03-27 A. A. Vladimirov , D. Ihle , N. M. Plakida

Mott insulators with strong spin-orbit coupling have been proposed to host unconventional magnetic states, including the Kitaev quantum spin liquid. The 4$d$ system $\alpha$-RuCl$_3$ has recently come into view as a candidate Kitaev system,…

The Kitaev model is a rare example of an analytically solvable and physically instantiable Hamiltonian yielding a topological quantum spin liquid ground state. Here we report signatures of Kitaev spin liquid physics in the honeycomb magnet…

Strongly Correlated Electrons · Physics 2021-01-04 Hector K. Vivanco , Benjamin A. Trump , Craig M. Brown , Tyrel M. McQueen

Recent studies have brought $\alpha$-RuCl$_3$ to the forefront of experimental searches for materials realizing Kitaev spin-liquid physics. This material exhibits strongly anisotropic exchange interactions afforded by the spin-orbit…

Strongly Correlated Electrons · Physics 2018-02-21 Stephen M. Winter , Kira Riedl , David Kaib , Radu Coldea , Roser Valenti

We study the field-induced magnetization processes of extended Heisenberg-Kitaev models on the honeycomb lattice, taking into account off-diagonal and longer-range exchange interactions, using a combination of Monte-Carlo simulations,…

Strongly Correlated Electrons · Physics 2017-09-04 Lukas Janssen , Eric C. Andrade , Matthias Vojta
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