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We characterize the optical response of a three-level atom subjected to an incoherent pump and continuously illuminated with a weak, quasi-resonant probe field. To this end, we apply a wavefunction approach based on QED Hamiltonian…

Quantum Physics · Physics 2021-10-27 Manuel Donaire

We study theoretically and experimentally the electronic relaxation of NO2 molecules excited by absorption of one ~400 nm pump photon. Semi-classical simulations based on trajectory surface hopping calculations are performed. They predict…

Several powerful techniques exist to detect topologically protected surface states of weakly-interacting electronic systems. In contrast, surface modes of strongly interacting systems which do not carry electric charge are much harder to…

Strongly Correlated Electrons · Physics 2016-08-24 Brent Perreault , Johannes Knolle , Natalia B. Perkins , F. J. Burnell

We demonstrate the novel effect of gain-induced spectral shifts in the type-II parametric down-conversion (PDC) process, which results in a transition from degenerate to non-degenerate PDC with increasing parametric gain. This effect,…

Resonant inelastic (Raman) light scattering off neutral GaAs quantum dots which contain a mean number, N=42, of electron-hole pairs is computed. We find Raman amplitudes corresponding to strongly collective final states (charge-density…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Alain Delgado , Augusto Gonzalez , Eduardo Menendez-Proupin

The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a material's crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives…

Materials Science · Physics 2021-07-07 Guru Khalsa , Nicole A. Benedek , Jeffrey Moses

Multi-photon emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multi-level atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has…

We theoretically study transmission in nanowaveguide coupled to high-quality plasmon resonances for which the metal loss is overcompensated by gain. The on-resonance transmission can vary widely from lower than --20dB to higher than 20dB…

Optics · Physics 2015-07-29 Song-Jin Im , Gum-Song Ho

We report modifications to the optical properties of fluorophores in the vicinity of noble metal nanotips. The fluorescence from small clusters of quantum dots has been imaged using an apertureless scanning near-field optical microscope.…

Other Condensed Matter · Physics 2008-04-28 N. I. Cade , F. Culfaz , L. Eligal , T. Ritman-Meer , F-M. Huang , F. Festy , D. Richards

We theoretically demonstrate control of the plasma-like effective response of a metamaterial composed of aligned metallic nanorods when the electric field of the incident radiation is parallel to the nanorods. By embedding this metamaterial…

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

Quantum Physics · Physics 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…

In this paper we show how transmission metallic gratings with very narrow and deep enough slits can exhibit transmission resonances for wavelengths larger than the period of the grating. By using a transfer matrix formalism and a…

Materials Science · Physics 2009-10-31 J. A. Porto , F. J. Garcia-Vidal , J. B. Pendry

In a non-reciprocal optical amplifier, gain depends on whether the light propagates forwards or backwards through the device. Typically, one requires either the magneto-optical effect, a temporal modulation, or an optical nonlinearity to…

Resonant Raman scattering of degenerate interacting two-channel quantum wire is studied. {\it All} collective excitations of two-channel quantum wire are shown to give rise to peaks in the polarized Raman spectra near resonance. If there…

Strongly Correlated Electrons · Physics 2009-11-07 Hyun C. Lee

We report on the generation of a Raman cascade spanning the wavelength range of 523 to 1750 nm wavelength range, in a standard telecommunication graded-index multimode optical fiber. Despite the highly multimode nature of the pump, the…

Optics · Physics 2013-12-13 Hamed Pourbeyram , Govind P. Agrawal , Arash Mafi

We demonstrate superluminal light propagation using two frequency multiplexed pump beams to produce a gain doublet in a photorefractive crystal of Ce:BaTiO3. The two gain lines are obtained by two-wave mixing between a probe field and two…

Quantum Physics · Physics 2008-09-24 H. N. Yum , M. Salit , G. S. Pati , S. Tseng , P. R. Hemmer , M. S. Shahriar

We demonstrate a Raman amplifier for matter-waves, where the amplified atoms and the gain medium are in two different hyperfine states. This amplifier is based on a novel form of superradiance that arises from self-stimulated Raman…

The random lasing (RL) emission of dyed vesicular polymeric films in diffusive regime of light propagation was investigated under helium temperature. It represents itself the coupling effect of stimulated emission and stimulated Raman…

Optics · Physics 2010-08-27 V. P. Yashchuk , E. A. Tikhonov , O. A. Prygodiuk

Results of room temperature Raman scattering studies of ultrathin graphitic films supported on Si (111)/SiO2 substrates are reported. The results are significantly different from those known for graphite. Spectra were collected using 514 nm…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Awnish Gupta , Gugang Chen , P. Joshi , S. Tadigadapa , P. C. Eklund