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Nearly magnetic metals often have layered lattice structures, consisting of coupled planes. In such a situation, physical properties will display, upon decreasing temperature or energy, a dimensional crossover from two-dimensional (2d) to…

Strongly Correlated Electrons · Physics 2009-11-13 Markus Garst , Lars Fritz , Achim Rosch , Matthias Vojta

We investigate the structural, magnetocrystalline anisotropy, critical behaviour, and magnetocaloric effect in the layered room-temperature monoclinic ferromagnet Cr$_{1.38}$Te$_2$. The critical behavior is studied by employing various…

The two-dimensional (2D) van der Waals ferromagnetic semiconductors, such as CrI$_3$ and Cr$_2$Ge$_2$Te$_6$, and the 2D ferromagnetic metals, such as Fe$_3$GeTe$_2$ and MnSe$_2$, have been obtained in recent experiments and attracted a lot…

Materials Science · Physics 2023-12-29 Jia-Wen Li , Zhen Zhang , Jing-Yang You , Bo Gu , Gang Su

Intrinsic, two-dimensional (2D) ferromagnetic semiconductors are an important class of materials for spintronics applications. Cr$_2$X$_2$Te$_6$ (X = Si and Ge) semiconductors show 2D Ising-like ferromagnetism, which is preserved in…

Strongly Correlated Electrons · Physics 2019-01-10 Yu Liu , C. Petrovic

We report anisotropic magnetocaloric effect and magnetic critical behavior in van der Waals crystal CrCl$_3$. The maximum magnetic entropy change $-\Delta S_M^{max} \sim 14.6$ J kg$^{-1}$ K$^{-1}$ and the relative cooling power $RCP \sim…

Materials Science · Physics 2020-07-16 Yu Liu , C. Petrovic

The critical properties of flux-grown single-crystalline quasi-two-dimensional weak itinerant ferromagnet Cr$_{0.62}$Te were investigated by bulk dc magnetization around the paramagnetic (PM) to ferromagnetic (FM) phase transition. Critical…

Strongly Correlated Electrons · Physics 2018-03-14 Yu Liu , C. Petrovic

The critical properties and magnetocaloric effect of semiconducting ferrimagnet Mn$_3$Si$_2$Te$_6$ single crystals have been investigated by bulk magnetization and heat capacity around $T_c$. Critical exponents $\beta = 0.41\pm0.01$ with a…

Strongly Correlated Electrons · Physics 2018-08-30 Yu Liu , C. Petrovic

Phase transitions and critical phenomena, which are dominated by fluctuations and correlations, are one of the fields replete with physical paradigms and unexpected discoveries. Especially for two-dimensional magnetism, the limitation of…

Mesoscale and Nanoscale Physics · Physics 2021-01-08 Zefang Li , Dong-Hong Xu , Xue Li , Hai-Jun Liao , Xuekui Xi , Yi-Cong Yu , Wenhong Wang

Magnetic anisotropy is crucially important for the stabilization of two-dimensional (2D) magnetism, which is rare in nature but highly desirable in spintronics and for advancing fundamental knowledge. Recent works on CrI$_3$ and CrGeTe$_3$…

Materials Science · Physics 2018-11-14 Changsong Xu , Junsheng Feng , Hongjun Xiang , L. Bellaiche

Layered van der Waals ferromagnets are promising candidates for designing new spintronic devices. Here we investigated the critical properties and magnetocaloric effect connected with ferromagnetic transition in layered van der Waals VI$_3$…

Materials Science · Physics 2020-01-15 Yu Liu , Milinda Abeykoon , C. Petrovic

Identifying intrinsic low-dimensional ferromagnets with high transition temperature and electrically tunable magnetism is crucial for the development of miniaturized spintronics and magnetoelectrics. Recently long-range 2D ferromagnetism…

Materials Science · Physics 2020-08-27 Hua Wang , Jingshan Qi , Xiaofeng Qian

Intrinsic, two-dimensional ferromagnetic semiconductors are an important class of materials for overcoming the limitations of dilute magnetic semiconductors for spintronics applications. CrSiTe$_3$ is a particularly interesting member of…

Strongly Correlated Electrons · Physics 2015-10-06 T. J. Williams , A. A. Aczel , M. D. Lumsden , S. E. Nagler , M. B. Stone , J. -Q. Yan , D. Mandrus

Through advanced experimental techniques on CrI$_{3}$ single crystals, we derive a previously not discussed pressure-temperature phase diagram. We find that $T_{c}$ increases to $\sim$ 66\,K with pressure up to $\sim$ 3\,GPa followed by a…

Low-dimensional magnetic materials have attracted much attention due to their novel properties and high potential for spintronic applications. In this work, we study the electronic structure and magnetic properties of the pseudo…

Materials Science · Physics 2021-12-22 Guangyu Wang , Lu Liu , Ke Yang , Hua Wu

We propose two-dimensional (2D) Ising-type ferromagnetic semiconductors TcSiTe3, TcGeSe3, and TcGeTe3 with high Curie temperatures around 200-0500 K. Owing to large spin-orbit couplings, the large magnetocrystalline anisotropy energy (MAE),…

Materials Science · Physics 2020-01-07 Jing-Yang You , Zhen Zhang , Xue-Juan Dong , Bo Gu , Gang Su

The marked interplay between the crystalline, electronic, and magnetic structure of atomically thin magnets has been regarded as the key feature for designing next-generation magneto-optoelectronic devices. In this respect, a detailed…

Strongly Correlated Electrons · Physics 2020-05-25 Michele Pizzochero , Ravi Yadav , Oleg V. Yazyev

We report on a combined experimental and theoretical study on CrI3 single crystals by employing the polarization dependence of resonant inelastic X-ray scattering (RIXS). Our investigations reveal multiple Cr 3d orbital splitting (dd…

Two-dimensional (2D) ferromagnets with high Curie temperature have long been the pursuit for electronic and spintronic applications. CrI3 is a rising star of intrinsic 2D ferromagnets, however, it suffers from weak exchange coupling. Here…

Materials Science · Physics 2020-09-22 Yu Guo , Nanshu Liu , Yanyan Zhao , Xue Jiang , Si Zhou , Jijun Zhao

CrI$_{3}$ is considered to be a promising candidate for spintronic devices and data storage. We derived the Heisenberg Hamiltonian for CrI$_{3}$ from density functional calculations using the Liechtenstein formula. Moreover, the…

Materials Science · Physics 2023-04-24 Hung Ba Tran , Hiroyoshi Momida , Yu-ichiro Matsushita , Koun Shirai , Tamio Oguchi

Among the recently widely studied van der Waals layered magnets CrX3 (X=Cl, Br, I), CrCl3 monolayer (ML) is particularly puzzling as it is solely shown by experiments to have an in-plane magnetic easy axis and, furthermore, all of previous…

Materials Science · Physics 2020-01-08 Feng Xue , Yusheng Hou , Zhe Wang , Ruqian Wu