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We use the ``isoconfigurational ensemble'' [Phys. Rev. Lett. {\bf 93}, 135701 (2004)] to analyze both dynamical and structural properties in simulations of a glass forming molecular liquid. We show that spatially correlated clusters of low…

Materials Science · Physics 2009-11-11 Gurpreet S. Matharoo , M. S. Gulam Razul , Peter H. Poole

We present molecular dynamics results for a two component, two-dimensional Lennard-Jones supercooled liquid near the glass transition. We find that the supercooled liquid is spatially heterogeneous and that there are long-lived clusters…

Disordered Systems and Neural Networks · Physics 2009-10-31 Gregory Johnson , Andrew I. Melcuk , Harvey Gould , W. Klein , Raymond D. Mountain

The emergence of nanoscience has increased the importance of experiments able to probe the very local structure of materials, especially for disordered and heterogeneous systems. This is technologically important; for example, the nanoscale…

Soft Condensed Matter · Physics 2015-05-13 R. Casalini , C. M. Roland

By characterizing the dynamics of idealized lattice models with a tunable kinetic constraint, we explore the different ways in which dynamical facilitation manifests itself within the local dynamics of glassy materials. Dynamical…

Statistical Mechanics · Physics 2012-06-25 Yael S. Elmatad , Aaron S. Keys

The presence of fluctuating local relaxation times, $\tau_r(t)$ has been used for some time as a conceptual tool to describe dynamical heterogeneities in glass-forming systems. However, until now no general method is known to extract the…

Disordered Systems and Neural Networks · Physics 2015-05-01 Gcina A. Mavimbela , Azita Parsaeian , Horacio E. Castillo

There is growing evidence that the flow of driven amorphous solids is not homogeneous, even if the macroscopic stress is constant across the system. Via event driven molecular dynamics simulations of a hard sphere glass, we provide the…

Soft Condensed Matter · Physics 2015-06-04 Suvendu Mandal , Markus Gross , Dierk Raabe , Fathollah Varnik

Spatio-temporal processes in environmental applications are often assumed to follow a Gaussian model, possibly after some transformation. However, heterogeneity in space and time might have a pattern that will not be accommodated by…

Applications · Statistics 2021-10-15 Thaís C. O. da Fonseca , Viviana G. R. Lobo , Alexandra M. Schmidt

As one increases the concentration of a colloidal suspension, the system exhibits a dramatic increase in viscosity. Structurally, the system resembles a liquid, yet motions within the suspension are slow enough that it can be considered…

Soft Condensed Matter · Physics 2012-05-22 Gary L. Hunter , Eric R. Weeks

We study by molecular dynamics computer simulation a binary soft-sphere mixture that shows a pronounced decoupling of the species' long-time dynamics. Anomalous, power-law-like diffusion of small particles arises, that can be understood as…

Statistical Mechanics · Physics 2013-05-29 Th. Voigtmann , J. Horbach

We study the low temperature dynamics of a two dimensional short-range spin system with uniform ferromagnetic interactions, which displays glassiness at low temperatures despite the absence of disorder or frustration. The model has a dual…

Disordered Systems and Neural Networks · Physics 2009-10-31 Juan P. Garrahan , M. E. J. Newman

Despite the enormous theoretical and application interests, a fundamental understanding of the glassy dynamics remains elusive. The static properties of glassy and ordinary liquids are similar, but their dynamics are dramatically different.…

Soft Condensed Matter · Physics 2023-11-21 Puneet Pareek , Monoj Adhikari , Chandan Dasgupta , Saroj Kumar Nandi

Spatially localized states play an important role in transition to turbulence in shear flows (Kawahara, Uhlmann & van Veen, Annu. Rev. Fluid Mech. 44, 203 (2012)). Despite the fact that some of them are attractors on the separatrix between…

Fluid Dynamics · Physics 2016-04-18 Rishabh Gvalani , Cédric Beaume

The mass transport in soft-sphere mixtures of small and big particles as well as in the disordered Lorentz gas (LG) model is studied using molecular dynamics (MD) computer simulations. The soft-sphere mixture shows anomalous small-particle…

Statistical Mechanics · Physics 2010-11-19 Jürgen Horbach , Thomas Voigtmann , Felix Höfling , Thomas Franosch

Glass transitions are widely observed in various types of soft matter systems. However, the physical mechanism of these transitions remains {elusive}, despite years of ambitious research. In particular, an important unanswered question is…

Disordered Systems and Neural Networks · Physics 2022-12-20 Norihiro Oyama , Shihori Koyama , Takeshi Kawasaki

We discuss the relaxation dynamics of a simple lattice gas model for glass-forming systems and show that with increasing density of particles this dynamics slows down very quickly. By monitoring the trajectory of tagged particles we find…

Soft Condensed Matter · Physics 2010-05-07 Pinaki Chaudhuri , Ludovic Berthier , Srikanth Sastry , Walter Kob

All liquids are topologically disordered materials; however, the degree of disorder can vary as a result of internal fluctuations in structure and topology. These fluctuations depend on both the composition and temperature of the system.…

Statistical Mechanics · Physics 2018-08-15 Katelyn A. Kirchner , Seong H. Kim , John C. Mauro

We propose an alternative theory for the relaxation of density fluctuations in glass-forming fluids. We derive an equation of motion for the density correlation function which is local in time and is similar in spirit to the equation of…

Soft Condensed Matter · Physics 2022-06-01 Grzegorz Szamel

Dynamic heterogeneity has often been modeled by assuming that a single-particle observable, fluctuating at a molecular scale, is influenced by its coupling to environmental variables fluctuating on a second, perhaps slower, time scale.…

Condensed Matter · Physics 2009-11-07 Gregor Diezemann , Gerald Hinze , Hans Sillescu

In this talk I will present a complete theory for the behaviour of large-scale dynamical heterogeneities in glasses. Following the work arXiv:1001.1746 I will show that we can write a (physically motivated) simple stochastic differential…

Disordered Systems and Neural Networks · Physics 2010-09-09 Silvio Franz , Giorgio Parisi , Federico Ricci-Tersenghi , Tommaso Rizzo

Complex fluids such as water exhibits many anomalous phenomena, and research suggests these properties are closely tied to critical fluctuations near the liquid-liquid phase transition critical point (LLCP). However, whether a similar LLCP…

Soft Condensed Matter · Physics 2026-05-06 Lin Ma , Xiaodong Yang , Xinjia Zhou , Gang Sun , Zhen Wei Wu