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The compression of SH$_2$ and its subsequent decomposition to SH$_3$, presumably in a cubic Im$\overline{3}$m structure, has lead to the discovery of conventional superconductivity with the highest measured and confirmed $T_c$ to date, 203…

Materials Science · Physics 2019-02-20 Maximilian Amsler

The ionization energy theory is used to calculate the evolution of the resistivity and specific heat curves with respect to different doping elements in the recently discovered superconducting Pnictide materials. Subsequently, the…

Superconductivity · Physics 2009-11-05 Andrew Das Arulsamy , Kostya "Ken" Ostrikov

As all-solid-state batteries (SSBs) develop as an alternative to traditional cells, a thorough theoretical understanding of driving forces behind battery operation is needed. We present a fully first-principles-informed model of potential…

Materials Science · Physics 2019-05-01 Michael W. Swift , Yue Qi

We have investigated the elastoresistance of two FeSe${}_{1-x}$Te${}_{x}$ (x about 0.4 - 0.5) compounds that have a close chemical composition but differ significantly in electronic properties. The first compound has a negative temperature…

Superconductivity · Physics 2020-09-23 Y. A. Ovchenkov , D. A. Chareev , D. E. Presnov , I. G. Puzanova , O. S. Volkova , A. N. Vasiliev

It is shown that continuously occurring electrolyte-reduction reaction on freshly-exposed electrode surfaces during lithiation/delithiation cycles causes the lowering of cycling efficiency, and hence, capacity fade in well-cycled silicon…

Materials Science · Physics 2020-02-19 Vijay A. Sethuraman

This paper reports thermopower and conductivity measurements through the metal-insulator transition for 2-dimensional electron gases in high mobility Si-MOSFETs. At low temperatures both thermopower and conductivity show critical behaviour…

Strongly Correlated Electrons · Physics 2009-11-07 R. Fletcher , V. M. Pudalov , A. D. B. Radcliffe , C. Possanzini

Silicon is a promising anode material for next-generation lithium-ion batteries. However, the volume change and the voltage hysteresis during lithiation and delithiation are two substantial drawbacks to their lifetime and performance. We…

Chemical Physics · Physics 2024-02-19 Lukas Köbbing , Arnulf Latz , Birger Horstmann

Understanding the mechanical interplay between silicon anodes and their surrounding solid-electrolyte interphase (SEI) is essential to improve the next generation of lithium-ion batteries. We model and simulate a 2D elliptical silicon…

Applied Physics · Physics 2024-09-13 Raphael Schoof , Lukas Köbbing , Arnulf Latz , Birger Horstmann , Willy Dörfler

Deep eutectic solvents with admixed lithium salts are considered as electrolytes in electrochemical devices like batteries or supercapacitors. Compared to eutectic mixtures of hydrogen-bond donors and lithium salts, their raw-material costs…

Soft Condensed Matter · Physics 2024-04-22 A. Schulz , P. Lunkenheimer , A. Loidl

The correlated electron system SmNiO3 exhibits a metal-insulator phase transition at 130 {\deg}C. Using an ionic liquid as an electric double layer (EDL) gate on three-terminal ultrathin SmNiO3 devices, we investigate gate control of the…

Materials Science · Physics 2013-05-10 Sieu D. Ha , Ulrich Vetter , Jian Shi , Shriram Ramanathan

It is of great importance to develop inorganic solid electrolytes with high ionic conductivity, thus enabling solid state Li-ion batteries to address the notorious safety issue about the current technology due to use of highly flammable…

Chemical Physics · Physics 2017-07-17 Zhuo Wang , Min Jie Xuan , Hong Jie Xu , Guosheng Shao

The process of deriving an interatomic potentials represents an attempt to integrate out the electronic degrees of freedom from the full quantum description of a condensed matter system. In practice it is the derivatives of the interatomic…

Materials Science · Physics 2016-06-23 G. J. Ackland

Charge lost per unit surface area of a silicon electrode due to the formation of solid-electrolyte-interphase (SEI) layer during initial lithiation was quantified, and the species that constitute this layer were identified. Coin cells made…

Electrides as a unique class of emerging materials exhibit fascinating properties and hold important significance for understanding the matter under extreme conditions, which is characterized by valence electrons localized into the…

Materials Science · Physics 2025-01-28 D. Wang , H. Song , Q. Hao , G. Yang , H. Wang , L. Zhang , Y. Chen , X. Chen , Hua Y. Geng

This letter reports thermopower and conductivity measurements through the metal-insulator transition for 2-dimensional electron gases in high mobility Si-MOSFET's. At low temperatures both thermopower and conductivity show critical behavior…

Disordered Systems and Neural Networks · Physics 2007-05-23 R. Fletcher , V. M. Pudalov , A. D. B. Radcliffe , C. Possanzini

These compounds have long been known as promising thermoelectric materials. Recently it was revealed, that they also have unconventional electronic topology. This renewed interest to the investigation of their transport properties. In order…

Mesoscale and Nanoscale Physics · Physics 2018-11-14 D. A. Pshenay-Severin , Y. V. Ivanov , A. T. Burkov

We first present a comparative analysis of temperature evolution of the excess thermodynamic potentials (state functions), the enthalpy $\Delta H$, entropy $\Delta S$ and Gibbs free energy $\Delta \Phi$, determined for \textit{i})…

Disordered Systems and Neural Networks · Physics 2025-07-04 A. S. Makarov , R. A. Konchakov , N. P. Kobelev , V. A. Khonik

This is the first quantitative analysis of mechanical reliability of all-solid state batteries. Mechanical degradation of the solid electrolyte (SE) is caused by intercalation-induced expansion of the electrode particles, within the…

Materials Science · Physics 2017-03-16 Giovanna Bucci , Tushar Swamy , Yet-Ming Chiang , W. Craig Carter

Models for strongly interacting fermions in disordered clusters forming an array, with electron hopping between sites, reproduce the linear dependence on temperature of the resistivity, typical of the strange metal phase of High Temperature…

Strongly Correlated Electrons · Physics 2021-12-17 F. Salvati , A. Tagliacozzo

HII region electron temperatures are a critical ingredient in metallicity determinations and recent observations reveal systematic variations in the temperatures measured using different ions. We present electron temperatures ($T_e$)…