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Based on ab initio software packages using nonorthogonal localized orbitals, we develop a general scheme of calculating response functions. We test the performance of this method by calculating nonlinear optical responses of materials, like…

Materials Science · Physics 2019-09-05 Chong Wang , Sibo Zhao , Xiaomi Guo , Xinguo Ren , Bing-Lin Gu , Yong Xu , Wenhui Duan

We present a technique for partitioning the total energy from a semi-local density functional theory calculation into contributions from individual electronic states in a localized Wannier basis. We use our technique to reveal the key role…

Materials Science · Physics 2025-10-15 Ethan T. Ritz , Guru Khalsa , Hsin-Yu Ko , Ju-an Zhang , Robert A. DiStasio , Nicole A. Benedek

The theory for the generation of Wannier functions within the generalized Pipek--Mezey approach [Lehtola, S.; J\'onsson, H. J. Chem. Theory Comput. 2014, 10, 642] is presented and an implementation thereof is described. Results are…

Materials Science · Physics 2017-02-15 Elvar Ö. Jónsson , Susi Lehtola , Martti Puska , Hannes Jónsson

The WS time delay matrix relates a lossless and reciprocal system's scattering matrix to its frequency derivative, and enables the synthesis of modes that experience well-defined group delays when interacting with the system. The elements…

Computational Physics · Physics 2021-07-28 Utkarsh R. Patel , Eric Michielssen

We present a code-independent compact representation of one-electron wavefunctions and other volumetric data (electron density, electrostatic potential, etc.) produced by electronic-structure calculations. The compactness of the…

Materials Science · Physics 2019-02-08 Sergey V. Levchenko , Matthias Scheffler

Wave function collapse models are considered as the modified theories of standard quantum mechanics at the macroscopic level. By introducing nonlinear stochastic terms in the Schr\"odinger equation, these models make predictions,…

Quantum Physics · Physics 2017-02-02 Jing Zhang , Tiancai Zhang , Jie Li

In this article new bounds on weighted p-norms of ambiguity functions and Wigner functions are derived. Such norms occur frequently in several areas of physics and engineering. In pulse optimization for Weyl--Heisenberg signaling in…

Information Theory · Computer Science 2016-11-17 Peter Jung

We discuss a maximally localized Wannier function approach for constructing lattice models from first-principles electronic structure calculations, where the effective Coulomb interactions are calculated in the constrained…

Strongly Correlated Electrons · Physics 2009-11-13 Takashi Miyake , F. Aryasetiawan

Nonlocal modeling has drawn more and more attention and becomes steadily more powerful in scientific computing. In this paper, we demonstrate the superiority of a first-principle nonlocal model -- Wigner function -- in treating singular…

Quantum Physics · Physics 2023-01-19 Sihong Shao , Lili Su

A standard method to obtain information on a quantum state is to measure marginal distributions along many different axes in phase space, which forms a basis of quantum state tomography. We theoretically propose and experimentally…

To obtain a local description from highly accurate density functional theory codes that are based on modified plane wave bases, a transformation to a local orthonormal Wannier function basis is required. In order to do so while enforcing…

Materials Science · Physics 2024-03-20 K. Koepernik , O. Janson , Yan Sun , J. van den Brink

Transition metal dichalcogenide materials $MX_2 (M=Mo,W;X=S,Se)$ are being thoroughly studied due to their novel two-dimensional structure, that is associated with exceptional optical and transport properties. From a computational point of…

Materials Science · Physics 2020-02-12 James Sifuna , Pablo García-Fernández , George S. Manyali , George Amolo , Javier Junquera

In this work, we investigate conditions which ensure the existence of an exponentially localized Wannier basis for a given periodic hamiltonian. We extend previous results in [Pan07] to include periodic zero flux magnetic fields which is…

Mathematical Physics · Physics 2013-03-26 Giuseppe De Nittis , Max Lein

Koopmans spectral functionals aim to describe simultaneously ground state properties and charged excitations of atoms, molecules, nanostructures and periodic crystals. This is achieved by augmenting standard density functionals with simple…

Materials Science · Physics 2022-07-25 Nicola Colonna , Riccardo De Gennaro , Edward Linscott , Nicola Marzari

The method used earlier for analysis of correlated nanoscopic systems is extended to infinite (periodic) s-band like systems described by the Hubbard model and its extensions. The optimized single-particle wave functions contained in the…

Strongly Correlated Electrons · Physics 2009-02-18 Jan Kurzyk , Włodzimierz Wójcik , Jozef Spałek

In systems undergoing localization-delocalization quantum phase transitions due to disorder or monitoring, there is a crucial need for robust methods capable of distinguishing phases and uncovering their intrinsic properties. In this work,…

Disordered Systems and Neural Networks · Physics 2024-07-16 Marcin Szyniszewski

Recent studies have theoretically investigated the atomic excitation and ionization induced by the dark matter (DM)-nucleus scattering, and it is found that the suddenly recoiled atom is much more likely to excite or lose its electrons than…

Mesoscale and Nanoscale Physics · Physics 2020-08-27 Zheng-Liang Liang , Lin Zhang , Fawei Zheng , Ping Zhang

We introduce a general, variational scheme applied to Kohn-Sham density functional theory that allows for partitioning of the ground-state density matrix into distinct spectral domains, each of which spanned by an independent diagonal…

Plasma Physics · Physics 2023-08-29 Babak Sadigh , Daniel Aberg , John Pask

Within this paper we outline a method able to generate truly minimal basis sets which describe either a group of bands, a band, or even just the occupied part of a band accurately. These basis sets are the so-called NMTOs, Muffin Tin…

Strongly Correlated Electrons · Physics 2009-09-29 Eva Zurek , Ove Jepsen , Ole K. Andersen

The systematic underestimation of band gaps is one of the most fundamental challenges in semilocal density functional theory (DFT). In addition to hindering the application of DFT to predicting electronic properties, the band gap problem is…

Chemical Physics · Physics 2024-08-27 Kyle Bystrom , Stefano Falletta , Boris Kozinsky
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