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Here we present a semiclassical analysis of spontaneous and stimulated radiative emission from unmodulated and optically-modulated electron quantum wavepackets. We show that the radiative emission/absorption and corresponding…

Quantum Physics · Physics 2018-11-28 Yiming Pan , Avraham Gover

This paper describes a method to do ab initio molecular dynamics in electronically excited systems within the random phase approximation (RPA). Using a dynamical variational treatment of the RPA frequency, which corresponds to the…

Condensed Matter · Physics 2009-10-31 Eric R. Bittner , D. S. Kosov

Spontaneous emission (SE) from a two-level atom in a photonic crystal (PC) with anisotropic one-band model is investigated using the fractional calculus. Analytically solving the kinetic equation in terms of the fractional exponential…

Other Condensed Matter · Physics 2015-05-13 Jing-Nuo Wu , Chih-Hsien Huang , Szu-Cheng Cheng , Wen-Feng Hsieh

We analyze the decay of classically chaotic quantum systems in the presence of fast ballistic escape routes on the Ehrenfest time scale. For a continuous excitation process, the form factor of the decay cross section deviates from the…

Chaotic Dynamics · Physics 2007-08-01 T. Gorin , D. F. Martinez , H. Schomerus

The interplay of quantum fluctuations with nonlinear dynamics is a central topic in the study of open quantum systems, connected to fundamental issues (such as decoherence and the quantum-classical transition) and practical applications…

Quantum Physics · Physics 2009-11-13 Michael A. Armen , Hideo Mabuchi

The dynamical generation of entanglement in closed bipartite systems is investigated in the semiclassical regime. We consider a model of two particles, initially prepared in a product of coherent states, evolving in time according to a…

Quantum Physics · Physics 2015-05-19 A. D. Ribeiro , R. M. Angelo

Quantum simulations of photoexcited low-dimensional systems are pivotal for understanding how to functionalize and integrate novel two-dimensional (2D) materials in next-generation optoelectronic devices. First principles predictions are…

Mesoscale and Nanoscale Physics · Physics 2023-05-15 Enrico Perfetto , Gianluca Stefanucci

In this paper we develop a picture of Quantum Mechanics based on the description of physical observables in terms of expectation value functions, generalizing thus the so called Ehrenfest theorems for quantum dynamics. Our basic technical…

Quantum Physics · Physics 2013-07-26 J. Clemente-Gallardo , G. Marmo

Motivated by quantum gravity, semi-classical theory, and quantum theory on curved spacetimes, we study the system of an oscillator coupled to two spin-1/2 particles. This model provides a prototype for comparing three types of dynamics: the…

Quantum Physics · Physics 2022-09-21 Viqar Husain , Irfan Javed , Suprit Singh

Linear and nonlinear electronic spectra provide an important tool to probe the absorption and transfer of electronic energy. Here we introduce a pure state Ehrenfest approach to obtain accurate linear and nonlinear spectra that is…

Chemical Physics · Physics 2022-12-15 Austin O. Atsango , Andrés Montoya-Castillo , Thomas E. Markland

Electronic energy transfer in the condensed phase, such as that occurring in photosynthetic complexes, frequently occurs in regimes where the energy scales of the system and environment are similar. This situation provides a challenge to…

Statistical Mechanics · Physics 2015-06-03 Timothy C. Berkelbach , Thomas E. Markland , David R. Reichman

Starting from a many-body classical system governed by a trace-form entropy we derive, in the stochastic quantization picture, a family of non linear and non-Hermitian Schroedinger equations describing, in the mean filed approximation, a…

Statistical Mechanics · Physics 2007-05-23 A. M. Scarfone

Measurement-induced state disturbance is a major challenge in obtaining quantum statistics at multiple time points. We propose a method to extract dynamic information from a quantum system at intermediate time points, namely snapshotting…

We investigate the spontaneous emission of a two-level system coupled to a photonic waveguide, showing that dynamical dephasing in the photon modes profoundly alters the decay law. In the absence of dephasing, the emitter displays…

Quantum Physics · Physics 2026-01-12 Stefano Longhi

Processes involving ultrafast laser driven electron-phonon dynamics play a fundamental role in the response of quantum systems in a growing number of situations of interest, as evidenced by phenomena such as strongly driven phase…

Materials Science · Physics 2024-03-01 Kevin Lively , Shunsuke A. Sato , Guillermo Albareda , Angel Rubio , Aaron Kelly

Electron Transfer (ET) reactions are modeled by the dynamics of a quantum two-level system (representing the electronic state) coupled to a thermalized bath of classical harmonic oscillators (representing the nuclei degrees of freedom).…

Chemical Physics · Physics 2014-11-24 Serge Aubry

We present a theory of magnetotransport through a system of two coupled electronic orbitals, where the electron spin interacts with a (large) local magnetic moment via an exchange interaction. For the physical realization of such a set-up…

Mesoscale and Nanoscale Physics · Physics 2012-11-06 Klemens Mosshammer , Gerold Kiesslich , Tobias Brandes

Highly excited vibrational states of an isolated molecule encode the vibrational energy flow pathways in the molecule. Recent studies have had spectacular success in understanding the nature of the excited states mainly due to the extensive…

Chemical Physics · Physics 2009-11-07 A. Semparithi , V. Charulatha , S. Keshavamurthy

We review properties of open chaotic mesoscopic systems with a finite Ehrenfest time tau_E. The Ehrenfest time separates a short-time regime of the quantum dynamics, where wave packets closely follow the deterministic classical motion, from…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Henning Schomerus , Philippe Jacquod

We propose a novel quantum electrodynamics (QED) platform where quantum emitters interact with a Hofstadter-ladder waveguide. We demonstrate several intriguing phenomena stemming from the exotic dispersion relation and vacuum mode…

Quantum Physics · Physics 2022-10-06 Xin Wang , Zhao-Min Gao , Jia-Qi Li , Huai-Bing Zhu , Hong-Rong Li