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Ultrasound irradiation is a commonly used technique for non-destructive diagnostics or targeted destruction. We report on a new versatile sonication device that fits in a variety of standard sample environments for neutron and X-ray…

Soft Condensed Matter · Physics 2018-01-26 Sudipta Gupta , Markus Bleuel , Gerald J. Schneider

The precipitate shape, size and distribution are crucial factors which determine the properties of several technologically important alloys. Elastic interactions between the inclusions modify their morphology and align them along…

Materials Science · Physics 2019-06-25 Sandeep Sugathan , Saswata Bhattacharya

We study the magnetic excitation spectra of resonant inelastic x-ray scattering (RIXS) at the $L$-edge from undoped cuprates beyond the fast collision approximation. We analyse the effect of the symmetry breaking ground state on the RIXS…

Strongly Correlated Electrons · Physics 2015-06-24 Jun-ichi Igarashi , Tatsuya Nagao

Attosecond pulses from X-ray free-electron laser (XFEL) have opened new opportunities for probing ultrafast electronic dynamics on the Angstrom--attosecond spatiotemporal scale. Most attosecond XFEL concepts rely on generating an ultrashort…

Accelerator Physics · Physics 2026-04-22 Chenzhi Xu , Jiawei Yan , Ye Chen , Winfried Decking , Marc Guetg , Tianyun Long , Bingyang Yan , Haixiao Deng

We measure the resonant forward scattering of light by a highly saturated atomic medium through the flashes emitted immediately after an abrupt extinction of the probe beam. The experiment is done in a dilute regime where the phenomena are…

Atomic Physics · Physics 2021-01-05 C. C. Kwong , T. Wellens , K. Pandey , D. Wilkowski

A self-consistent radiation-hydrodynamics model of an accretion channel of subcritical X-ray pulsars is constructed. The influence of the presence of resonance in the scattering cross-section on the accretion process and radiation transfer…

High Energy Astrophysical Phenomena · Physics 2024-03-01 I. D. Markozov , A. D. Kaminker , A. Y. Potekhin

We show that the momentum flexibility of inelastic x-ray scattering may be exploited to invert its loss function, alowing real time imaging of density disturbances in a medium. We show the disturbance arising from a point source in liquid…

Condensed Matter · Physics 2009-11-10 P. Abbamonte , K. D. Finkelstein , M. D. Collins , S. M. Gruner

We assess the performance of different protocols for simulating excited-state X-ray absorption spectra. We consider three different protocols based on equation-of-motion coupled-cluster singles and doubles, two of them combined with the…

Chemical Physics · Physics 2022-11-24 Shota Tsuru , Marta L. Vidal , Mátyás Pápai , Anna I. Krylov , Klaus B. Møller , Sonia Coriani

Collective excitations contain rich information about photoinduced transient states in correlated systems. In a Mott insulator, charge degrees of freedom are frozen, but can be activated by photodoping. The energy-momentum distribution of…

Strongly Correlated Electrons · Physics 2020-04-23 Yao Wang , Yuan Chen , Chunjing Jia , Brian Moritz , Thomas P. Devereaux

We present a theoretical study of temporal, spectral, and spatial reshaping of intense, ultrafast x-ray pulses propagating through a resonant medium. Our calculations are based on the solution of a 3D time-dependent Schr\"odinger-Maxwell…

Atomic Physics · Physics 2020-12-30 Kai Li , Marie Labeye , Phay J. Ho , Mette B. Gaarde , Linda Young

Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

Single molecule X-ray scattering experiments with free electron lasers have opened a new route to the structure determination of biomolecules. Because typically only very few photons per scattering image are recorded and thus the…

Computational Physics · Physics 2023-04-17 Steffen Schultze , Helmut Grubmüller

The interaction of a femtosecond optical pulse with a Fe$_{1}$/(MgO)$_{3}$(001) metal/oxide heterostructure is investigated using time-dependent density functional theory (TDDFT) calculations in the real-time domain. We systematically study…

Materials Science · Physics 2022-06-22 Elaheh Shomali , Markus E. Gruner , Rossitza Pentcheva

Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…

Absorbing a focused, femtosecond X-ray pulse from a Free-Electron Laser (FEL) can lead to extreme electronic excitations in solids. This excitation drives changes of the electronic system over the course of the pulse duration and the…

Materials Science · Physics 2023-12-12 Robin Y. Engel , Markus Scholz , Jan O. Schunck , Martin Beye

Research on actinide materials, both basic and applied, has been greatly advanced by the general techniques available from high-intensity photon beams from x-ray synchrotron sources. The most important single reason is that such x-ray…

Materials Science · Physics 2023-03-15 R. Caciuffo , G. H. Lander , G. van der Laan

The transition from the amplification of spontaneous emission to superfluorescence in a three-level and swept-gain medium excited by an X-ray free electron laser pulse is theoretically investigated. Given the specific time scale of X-ray…

Quantum Physics · Physics 2020-02-25 Yu-Hung Kuan , Wen-Te Liao

Recent advancements in ultrashort and intense X-ray sources have enabled the utilisation of resonant inelastic X-ray scattering (RIXS) as a probing technique for monitoring photoinduced dynamics in molecular systems. To account for dynamic…

Chemical Physics · Physics 2024-03-19 Antonia Freibert , David Mendive-Tapia , Oriol Vendrell , Nils Huse