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Next-generation lithium-ion batteries with silicon anodes have positive characteristics due to higher energy densities compared to state-of-the-art graphite anodes. However, the large volume expansion of silicon anodes can cause high…

Numerical Analysis · Mathematics 2024-04-03 R. Schoof , G. F. Castelli , W. Dörfler

The development of silicon anodes to replace conventional graphite in efforts to increase energy densities of lithium-ion batteries has been largely impeded by poor interfacial stability against liquid electrolytes. Here, stable operation…

Ferroelectrics and ionic conductors are important functional materials, each supporting a plethora of applications in information and energy technology. The underlying physics governing their functional properties is ionic motion, and yet…

Materials Science · Physics 2023-12-22 Liyang Ma , Jing Wu , Tianyuan Zhu , Yiwei Huang , Qiyang Lu , Shi Liu

The dependence of the superconducting transition temperature T_{c} on nearly hydrostatic pressure has been determined to 67 GPa in an ac susceptibility measurement for a Li sample embedded in helium pressure medium. With increasing…

Superconductivity · Physics 2009-11-10 Shanti Deemyad , James S. Schilling

We report the successful growth of high quality single crystals of LiFeAs with lateral sizes up to 5 x 5 mm2 by the Sn-flux method. Electrical resistivity studies reveal that the superconducting onset temperature is 18.2 K with a transition…

Superconductivity · Physics 2010-10-20 Bumsung Lee , Seunghyun Khim , Jung Soo Kim , G. R. Stewart , Kee Hoon Kim

Solid-state electrolyte batteries are expected to replace liquid electrolyte lithium-ion batteries in the near future thanks to their higher theoretical energy density and improved safety. However, their adoption is currently hindered by…

Superconductivity of YBa$_2$Cu$_3$O$_{7-\delta}$ single crystals was investigated in small magnetic fields. In magnetic measurements the superconducting transition for $\textbf{H} \| c$ appears 0.4 K higher than for $\textbf{H} \bot c$. In…

Superconductivity · Physics 2019-11-13 V. I. Nizhankovskiy , K. Rogacki

Ensuring solid-state lithium batteries perform well across a wide temperature range is crucial for their practical use. Molecular dynamics (MD) simulations can provide valuable insights into the temperature dependence of the battery…

Materials Science · Physics 2024-03-22 Zicun Li , Jianxing Huang , Xinguo Ren , Jinbin Li , Ruijuan Xiao , Hong Li

Li2FeSiO4 is an important alternative cathode for next generation Li-ion batteries due to its high theoretical capacity (330 mA h/g). However, its development has faced significant challenges arising from structural complexity and poor…

Materials Science · Physics 2016-11-15 P. Vajeeston , H. Fjellvåg

Mott metal-insulator transitions possess electronic, magnetic, and structural degrees of freedom promising next generation energy-efficient electronics. We report a previously unknown, hierarchically ordered state during a Mott transition…

We demonstrated X-ray structural analysis of the pressure-induced superconductor, $\beta'$-ET$_2$ICl$_2$ under extremely high-pressure conditions, where ET denotes bis(ethylenedithio)tetrathiafulvalene. This material has been known as the…

Superconductivity · Physics 2025-09-29 T. Kobayashi , K. Yoshimi , H. Ma , S. Sekine , H. Taniguchi , N. Matsunaga , A. Kawamoto , Y. Uwatoko

We investigated the temperature dependence of the superlattice intensity and thermal diffuse scattering intensity of BaAl2O4, which has a network structure with corner-sharing AlO4 tetrahedra, via synchrotron X-ray diffraction experiments.…

Materials Science · Physics 2016-04-27 Y. Ishii , S. Mori , Y. Nakahira , C. Moriyoshi , H. Taniguchi , H. Moriwake , Y. Kuroiwa

We conduct first-principles simulations of La$_3$Ni$_2$O$_7$, a nickelate in which recent experiments have shown signs of high-temperature superconductivity. Within the hydrostatic pressure range where superconductivity is observed, we find…

Superconductivity · Physics 2026-02-25 Daan Verraes , Tom Braeckevelt , Nick Bultinck , Veronique Van Speybroeck

We use spatially-resolved transport techniques to investigate the superconducting properties of single crystals La$_{2-x}$Ba$_x$CuO$_4$. We find a new superconducting transition temperature $T_{cs}$ associated with the ab-plane surface…

Superconductivity · Physics 2017-03-01 X. Y. Tee , T. Ito , T. Ushiyama , Y. Tomioka , I. Martin , C. Panagopoulos

We studied the electrical transport on $\beta$-Fe$_{4+\delta}$Se$_{5}$ single-crystal nanowires, exhibiting $\sqrt{5}\times\sqrt{5}$ Fe-vacancy order and mixed valence of Fe. We observed a first-order metal-insulator transition of the…

The effects of Co-substitution on Ba(Ni$_{1-x}$Co$_x$)$_2$As$_2$ ($0\leq x\leq 0.251$) single crystals grown out of Pb flux are investigated via transport, magnetic, and thermodynamic measurements. BaNi$_2$As$_2$ exhibits a first order…

We report a detailed magnetotransport study of the highly anisotropic quasi-one-dimensional oxide Li$_{0.9}$Mo$_6$O$_{17}$ whose in-chain electrical resistivity diverges below a temperature $T_{\rm min} \sim$ 25 K. For $T < T_{\rm min}$, a…

Strongly Correlated Electrons · Physics 2010-06-16 X. Xu , A. F. Bangura , J. G. Analytis , J. D. Fletcher , M. M. J. French , N. Shannon , J. He , S. Zhang , D. Mandrus , R. Jin , N. E. Hussey

In this paper for the first time we report the results of molecular dynamics simulation of electrode/electrolyte interface of Li-O2 cathode under potential close to experimental values in 1M dimethyl sulfoxide (DMSO) solution of LiPF6 salt.…

Chemical Physics · Physics 2017-01-10 Artem Sergeev , Alexander Chertovich , Daniil Itkis , Anik Sen , Axel Gross , Alexei Khokhlov

We investigate the pressure-temperature ($p$-$T$) phase diagram of elemental lithium (Li) up to multiterapascal (TPa) pressures using ab-initio random structure search (AIRSS) and density functional theory (DFT). At zero temperature, beyond…

Materials Science · Physics 2024-03-21 Jack Whaley-Baldwin , Miguel Martinez-Canales , Chris J. Pickard

A phase diagram for a 2D metal with variable carrier density has been derived. It consists of a normal phase, where the order parameter is absent; a so-called ``abnormal normal'' phase where this parameter is also absent but the mean number…

Superconductivity · Physics 2009-10-30 Valery P. Gusynin , Vadim M. Loktev , Sergei G. Sharapov