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By means of density functional theory plus dynamical mean-field theory (DFT+DMFT) calculations and resonant inelastic x-ray scattering (RIXS) experiments, we investigate the high-pressure phases of the spin-orbit-coupled $J_{\rm{eff}}=3/2$…

The electronic states near the Fermi level of recently discovered superconductor Ba$_2$CuO$_{4-\delta}$ consist primarily of the Cu $d_{x^2-y^2}$ and $d_{3z^2-r^2}$ orbitals. We investigate the electronic correlation effect and the orbital…

Strongly Correlated Electrons · Physics 2021-06-23 Yu Ni , Ya-Min Quan , Jingyi Liu , Yun Song , Liang-Jian Zou

Recent studies establish that the cuprate pseudogap phase is susceptible at low temperatures to forming not only a $d$-symmetry superconducting (SC) state, but also a $d$-symmetry form factor (dFF) density wave (DW) state. The concurrent…

Electronic structure has been studied in lightly electron doped correlated spin-orbit insulator Sr$_2$IrO$_4$ by angle-resolved photoelectron spectroscopy. We have observed coexistence of the lower Hubbard band and the in-gap band, the…

We present an interacting model for the electronic and magnetic behavior of a strained $(001)$ atomic layer of Sr$_2$FeMoO$_6,$ which shows room-temperature ferrimagnetism and magnetoresistance with potential spintronics application in the…

Strongly Correlated Electrons · Physics 2020-07-22 Masahiko G. Yamada , George Jackeli

Sr3Ir2O7 exhibits a novel Jeff=1/2 insulating state that features a splitting between Jeff=1/2 and 3/2 bands due to spin-orbit interaction. We report a metal-insulator transition in Sr3Ir2O7 via either dilute electron doping (La3+ for Sr2+)…

Strongly Correlated Electrons · Physics 2015-06-15 L. Li , P. P. Kong , T. F. Qi , C. Q. Jin , S. J. Yuan , L. E. DeLong , P. Schlottmann , G. Cao

We report the results of a combined muon spin rotation and neutron scattering study on La2-xSrxCuO4 in the vicinity of the so-called 1/8-anomaly. Application of a magnetic field drives the system towards a magnetically ordered…

The mixing of orbital and spin character in the wave functions of the $5d$ iridates has led to predictions of strong couplings among their lattice, electronic and magnetic degrees of freedom. As well as realizing a novel spin-orbit assisted…

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

Using x-ray absorption spectroscopy at the Ru-$L_{2,3}$ edge we reveal that the Ru$^{4+}$ ions remain in the $S$=1 spin state across the rare 4d-orbital ordering transition and spin-gap formation. We find using local spin density…

Doped Mott insulators are the starting point for interesting physics such as high temperature superconductivity and quantum spin liquids. For multi-band Mott insulators, orbital selective ground states have been envisioned. However, orbital…

We report neutron scattering studies on single crystals of the electron-doped (n-type) superconducting cuprate Nd2-xCexCuO4 (x=0.15) with Tc = 18 K and 25 K. Unlike the hole-doped (p-type) superconducting cuprates where incommensurate…

Strongly Correlated Electrons · Physics 2009-11-07 K. Yamada , K. Kurahashi , T. Uefuji , M. Fujita , S. Park , S. -H. Lee , Y. Endoh

We study possible superconductivity in a carrier-doped iridium oxide insulator Sr$_{2}$IrO$_{4}$ based on an effective $t_{2g}$ three-orbital Hubbard model on the square lattice with a large spin-orbit coupling (SOC). Numerically solving…

Superconductivity · Physics 2019-09-02 Kazutaka Nishiguchi , Tomonori Shirakawa , Hiroshi Watanabe , Ryotaro Arita , Seiji Yunoki

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

A model of CuO$_2$ planes of cuprate perovskites, containing $d_{x^2-y^2}$ copper orbitals and symmetric combinations of oxygen $p_\sigma$ orbitals, is investigated using the strong coupling diagram technique. This approach allows one to…

Strongly Correlated Electrons · Physics 2020-09-01 Alexei Sherman

A series of polycrystalline samples of Sr2-xIrO4 have been synthesized by a solid-state reaction method. The crystal structure of this doped system can be explained on the basis of the extended nature of 5d electrons and strontium vacancies…

Strongly Correlated Electrons · Physics 2016-11-09 Jimei Kong , S. L. Liu , Jie Cheng , Haiyun Wang , Xing ao Li , Z. H. Wang

Resonant x-ray diffraction experiments were performed for the metallic iridium oxide IrO$_{2}$. We observed anisotropic tensor of susceptibility (ATS) scattering, the spectrum of which shows a sharp contrast between the $L_{3}$ and $L_{2}$…

Strongly Correlated Electrons · Physics 2015-06-12 Yasuyuki Hirata , Kenya Ohgushi , Jun-ichi Yamaura , Hiroyuki Ohsumi , Soshi Takeshita , Masaki Takata , Takahisa Arima

The unusual magnetic and electronic ground states of 5d iridates has been shown to be driven by intrinsically enhanced spin-orbit coupling (SOC). The influence of appreciable but reduced SOC in creating the manifested magnetic insulating…

Strongly Correlated Electrons · Physics 2015-12-01 S. Calder , L. Li , S. Okamoto , Y. Choi , R. Mukherjee , D. Haskel , D. Mandrus

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

In order to investigate the electronic state in the normal state of high-Tc cuprates in a wide range of temperature and hole-concentration, specific-heat, electrical-resistivity, magnetization and muon-spin-relaxation (muSR) measurements…

Superconductivity · Physics 2015-05-19 K. Suzuki , T. Adachi , Y. Tanabe , Y. Koike , T. Kawamata , Risdiana , T. Suzuki , I. Watanabe
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