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We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…

We present AC and DC magnetometry, heat capacity, muon spin relaxation ($\mu$SR) and resonant inelastic X-ray scattering (RIXS) studies of the pyrochlore osmate Y$_2$Os$_2$O$_7$. We observe a non-zero effective moment governed by…

Geometrical frustration is a central challenge in contemporary condensed matter physics, a crucible favourable to the emergence of novel physics. The pyrochlore magnets, with rare earth magnetic moments localized at the vertices of…

Strongly Correlated Electrons · Physics 2015-05-30 Sylvain Petit , Pierre Bonville , Isabelle Mirebeau , Hannu Mutka , Julien Robert

We have investigated the spin dynamics in the bilayered perovskite Sr3Ru2O7 as a function of magnetic field and temperature using 17O-NMR. This system sits close to a metamagnetic quantum critical point (MMQCP) for the field perpendicular…

Strongly Correlated Electrons · Physics 2007-05-23 Kentaro Kitagawa , Kenji Ishida , Robin S. Perry , Takashi Tayama , Toshiro Sakakibara , Yoshiteru Maeno

DC-magnetization data measured down to 40 mK speak against conventional freezing and reinstate YbMgGaO$_4$ as a triangular spin-liquid candidate. Magnetic susceptibility measured parallel and perpendicular to the $c$-axis reaches constant…

Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…

Strongly Correlated Electrons · Physics 2013-06-18 Lucile Savary , Leon Balents

We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb$_{2}$Mo$_{2}$O$_{7}$, $T$$_{g}$$\simeq$24 K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass…

Strongly Correlated Electrons · Physics 2013-09-17 D. K. Singh , Y. S. Lee

Muon spin relaxation measurements on some quantum spin ice candidate materials, the insulating pyrochlores Pr2B2O7 (B = Sn, Zr, Hf), have been performed for temperatures in the range 0.05-280 K. The results are indicative of a static…

Strongly Correlated Electrons · Physics 2015-06-22 F. R. Foronda , F. Lang , J. S. Möller , T. Lancaster , A. T. Boothroyd , F. L. Pratt , S. R. Giblin , D. Prabhakaran , S. J. Blundell

We investigate the electron and nuclear spin coherence properties of ytterbium ($\mathrm{Yb}^{3+}$) ions with non-zero nuclear spin, within an yttrium orthosilicate (Y$_2$SiO$_5$) crystal, with a view to their potential application in…

Quantum Physics · Physics 2019-08-06 Hee-Jin Lim , Sacha Welinski , Alban Ferrier , Philippe Goldner , J. J. L. Morton

In this paper we present a comprehensive study of magnetic dynamics in the rare-earth orthoferrite YbFeO$_3$ at temperatures below and above the spin-reorientation (SR) transition $T_{\mathrm{SR}}=7.6$ K, in magnetic fields applied along…

An adiabatic demagnetization process is studied in Gd2Ti2O7, a geometrically frustrated antiferromagnet on a pyrochlore lattice. In contrast to conventional paramagnetic salts, this compound can exhibit a temperature decrease by a factor of…

Strongly Correlated Electrons · Physics 2007-05-23 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , A. I. Golov , I. B. Berkutov , O. A. Petrenko , G. Balakrishnan , M. E. Zhitomirsky

Pr$_2$Zr$_2$O$_7$ is a pyrochlore quantum spin-ice candidate. Using Raman scattering spectroscopy we probe crystal electric field excitations of Pr$^{3+}$, and demonstrate the importance of their interactions with the lattice. We identify a…

Strongly Correlated Electrons · Physics 2021-09-03 Yuanyuan Xu , Huiyuan Man , Nan Tang , Santu Baidya , Hongbin Zhang , Satoru Nakatsuji , David Vanderbilt , Natalia Drichko

From a microscopic model for the pyrochlore antiferromagnet Tb2Sn2O7, including the crystal field Hamiltonian and interactions between the angular momenta, we compute an effective pseudospin-1/2 Hamiltonian Heff$ that incorporates…

Statistical Mechanics · Physics 2010-11-30 Paul A. McClarty , Pawel Stasiak , Michel J. P. Gingras

The quantum pyrochlore antiferromagnet is studied by perturbative expansions and exact diagonalization of small clusters. We find that the ground state is a spin-liquid state: The spin-spin correlation functions decay exponentially with…

Strongly Correlated Electrons · Physics 2009-10-31 Benjamin Canals , Claudine Lacroix

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

Strongly Correlated Electrons · Physics 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

We investigate ytterbium gallium garnet Yb$_{3}$Ga$_{5}$O$_{12}$ in the paramagnetic phase above the supposed magnetic transition at $T_{\lambda} \approx 54$ mK. Our study combines susceptibility and specific heat measurements with neutron…

Strongly Correlated Electrons · Physics 2021-07-28 E. Lhotel , L. Mangin-Thro , E. Ressouche , P. Steffens , E. Bichaud , G. Knebel , J. -P. Brison , C. Marin , S. Raymond , M. E. Zhitomirsky

We review recent studies of spin dynamics in rare-earth orthorhombic perovskite oxides of the type $RM$O$_3$, where $R$ is a rare-earth ion and $M$ is a transition-metal ion, using single-crystal inelastic neutron scattering (INS). After a…

Strongly Correlated Electrons · Physics 2021-07-28 A. Podlesnyak , S. Nikitin , G. Ehlers

The very nature of the ground state of the pyrochlore compound Yb$_2$Ti$_2$O$_7$ is much debated, as experimental results demonstrate evidence for both a disordered or a long-range ordered ground state. Indeed, the delicate balance of…

Strongly Correlated Electrons · Physics 2014-05-13 E. Lhotel , S. R. Giblin , M. R. Lees , G. Balakrishnan , L. J. Chang , Y. Yasui

An effective quantum pseudospin-1/2 Hamiltonian for Yb_2TM_2O_7 (TM = Ti and Sn) is obtained in terms of the atomic Kramers ground doublet of the LS coupling and the crystalline electric field, which is almost described with J^z=\pm 1/2. It…

Strongly Correlated Electrons · Physics 2015-05-20 Shigeki Onoda