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Despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K, the Tb2Ti2O7 pyrochlore magnetic material lacks long range magnetic order down to at least $T^*\approx 50$ mK. It has recently been proposed that the low temperature collective…

Statistical Mechanics · Physics 2009-05-07 Hamid R. Molavian , Michel J. P. Gingras

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

Detailed $^{195}$Pt- and $^{171}$Yb nuclear magnetic resonance (NMR) studies on the heterogeneous mixed valence system YbPtGe$_2$ are reported. The temperature dependence of the $^{195}$Pt-NMR shift $^{195}K(T)$ indicates the opening of an…

Strongly Correlated Electrons · Physics 2013-11-05 R. Sarkar , R. Gumeniuk , A. Leithe-Jasper , W. Schnelle , Y. Grin , C. Geibel , M. Baenitz

The pyrochlore magnet Tb$_{2}$Ti$_{2}$O$_{7}$ shows a lack of magnetic order to low temperatures and is considered to be a quantum spin liquid candidate. We perform time-domain THz spectroscopy on high quality Tb$_{2}$Ti$_{2}$O$_{7}$…

Strongly Correlated Electrons · Physics 2021-04-21 Xinshu Zhang , Yi Luo , T. Halloran , J. Gaudet , Huiyuan Man , S. M. Koohpayeh , N. P. Armitage

We present a parametric study of the diffuse magnetic scattering at (1/2,1/2,1/2) positions in reciprocal space, ascribed to a frozen antiferromagnetic spin ice state in single crystalline Tb2Ti2O7. Our high-resolution neutron scattering…

Strongly Correlated Electrons · Physics 2015-06-18 K. Fritsch , E. Kermarrec , K. A. Ross , Y. Qiu , J. R. D. Copley , D. Pomaranski , J. B. Kycia , H. A. Dabkowska , B. D. Gaulin

We present muon spin relaxation ($\mu$SR) and specific-heat versus temperature $C(T)$ measurements on polycrystalline and single-crystal samples of the pyrochlore magnet Yb$_2$Ti$_2$O$_7$. $C(T)$ exhibits a sharp peak at a $T_\mathrm{C}$ of…

Strongly Correlated Electrons · Physics 2014-05-28 Lieh-Jeng Chang , Martin R. Lees , Isao Watanabe , Adrian D. Hillier , Yukio Yasui , Shigeki Onoda

We report detailed measurements of the low temperature magnetic phase diagram of Er$_2$Ti$_2$O$_7$. Heat capacity and time-of-flight neutron scattering studies of single crystals, subject to magnetic fields applied along the…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , J. P. Clancy , A. Bourque , M. A. White , M. Ramazanoglu , J. S. Gardner , Y. Qiu , J. R. D. Copley , H. A. Dabkowska , B. D. Gaulin

The Coulombic quantum spin liquid in quantum spin ice is an exotic quantum phase of matter that emerges on the pyrochlore lattice and is currently actively searched for. Motivated by recent experiments on the Yb-based breathing pyrochlore…

Strongly Correlated Electrons · Physics 2016-08-23 Lucile Savary , Xiaoqun Wang , Hae-Young Kee , Yong Baek Kim , Yue Yu , Gang Chen

The pyrochlore oxides Dy$_{2}$Ti$_{2}$O$_{7}$ and Ho$_{2}$Ti$_{2}$O$_{7}$ are well studied spin ice systems and have shown the evidences of magnetic monopole excitations. Unlike these, Dy$_{2}$Zr$_{2}$O$_{7}$ is reported to crystallize in a…

Strongly Correlated Electrons · Physics 2020-08-26 Sheetal , Anzar Ali , Sarita Rajput , Yogesh Singh , Tulika Maitra , C. S. Yadav

The pyrochlore magnet $\rm Yb_2Ti_2O_7$ has been proposed as a quantum spin ice candidate, a spin liquid state expected to display emergent quantum electrodynamics with gauge photons among its elementary excitations. However, $\rm…

Strongly Correlated Electrons · Physics 2018-06-20 Gabriele Sala , Dalini D. Maharaj , Matthew B. Stone , Hanna A. Dabkowska , Bruce D. Gaulin

The spin ice materials, including Ho2Ti2O7 and Dy2Ti2O7, are rare earth pyrochlore magnets which, at low temperatures, enter a constrained paramagnetic state with an emergent gauge freedom. Remarkably, the spin ices provide one of very few…

Strongly Correlated Electrons · Physics 2014-07-29 Michel J. P. Gingras , Paul A. McClarty

A quantum melting of the spin ice is proposed for pyrochlore-lattice magnets Pr$_2TM_2$O$_7$ ($TM=$Ir, Zr, and Sn). The quantum superexchange Hamiltonian having a nontrivial magnetic anisotropy is derived in the basis of atomic non-Kramers…

Strongly Correlated Electrons · Physics 2010-07-26 Shigeki Onoda , Yoichi Tanaka

We study magnetic behaviour of the Yb$^{3+}$ ions on a frustrated pyrochlore lattice in the spinel {\CYS}. The crystal-electric field parameters deduced from high-energy inelastic neutron scattering reveal well-isolated ytterbium ground…

Strongly Correlated Electrons · Physics 2019-09-18 K. Guratinder , Jeffrey G. Rau , V. Tsurkan , C. Ritter , J. Embs , T. Fennell , H. C. Walker , M. Medarde , T. Shang , A. Cervellino , Ch. Rüegg , O. Zaharko

We report the 77Se-nuclear magnetic resonance (NMR) results of trivalent Yb zigzag chain compound YbAgSe2, which is a sister compound of YbCuS2. The 77Se-NMR spectrum was reproduced by considering two different Se sites with negative Knight…

Strongly Correlated Electrons · Physics 2024-11-15 Fumiya Hori , Shunsaku Kitagawa , Kenji Ishida , Souichiro Mizutani , Yudai Ohmagari , Takahiro Onimaru

The spin-liquid phase of two highly frustrated pyrochlore magnets Gd2Ti2O7 and Gd2Sn2O7 is probed using electron spin resonance in the temperature range 1.3 - 30 K. The deviation of the absorption line from the paramagnetic position \nu…

Strongly Correlated Electrons · Physics 2013-05-29 S. S. Sosin , L. A. Prozorova , A. I. Smirnov , P. Bonville , G. Jasmin - Le Bras , O. A. Petrenko

We present an experimental study of the quantum spin ice candidate pyrochlore coumpound \przr\ by means of magnetization measurements, specific heat and neutron scattering up to 12 T and down to 60 mK. When the field is applied along the…

We report neutron scattering studies of the spin correlations of the geometrically frustrated pyrochlore Tb2Mo2O7 using single crystal samples. This material undergoes a spin-freezing transition below Tg~24 K, similar to Y2Mo2O7, and has…

Strongly Correlated Electrons · Physics 2009-11-13 D. K. Singh , J. S. Helton , S. Chu , T. H. Han , C. J. Bonnoit , S. Chang , H. J. Kang , J. W. Lynn , Y. S. Lee

The "spin ice" state found in the rare earth pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7 offers a beautiful realisation of classical magnetostatics, complete with magnetic monopole excitations. It has been suggested that in "quantum spin ice"…

Strongly Correlated Electrons · Physics 2015-06-04 Owen Benton , Olga Sikora , Nic Shannon

The ground state of the quantum spin ice candidate magnet Yb2Ti2O7 is known to be sensitive to weak disorder at the 1 percent level which occurs in single crystals grown from the melt. Powders produced by solid state synthesis tend to be…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , K. A. Ross , E. Kermarrec , N. P. Butch , G. Ehlers , H. A. Dabkowska , B. D. Gaulin

Recent work has highlighted remarkable effects of classical thermal fluctuations in the dipolar spin ice compounds, such as "artificial magnetostatics", manifesting as Coulombic power-law spin correlations and particles behaving as…

Strongly Correlated Electrons · Physics 2011-10-11 Kate A. Ross , Lucile Savary , Bruce D. Gaulin , Leon Balents