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Rate coefficients for inelastic Mg+H collisions are calculated for all transitions between the lowest seven levels and the ionic state (charge transfer). The rate coefficients are based on cross-sections from full quantum scattering…

Solar and Stellar Astrophysics · Physics 2015-06-04 P. S. Barklem , A. K. Belyaev , A. Spielfiedel , M. Guitou , N. Feautrier

A theoretical method for the estimation of cross sections and rates for excitation and charge transfer processes in low-energy hydrogen atom collisions with neutral atoms, based on an asymptotic two-electron model of ionic-covalent…

Atomic Physics · Physics 2016-05-04 Paul S. Barklem

OH is a cornerstone molecule in the chemistry of interstellar and circumstellar media and is ubiquitously detected in warm gas thanks to its infrared rotational lines. However, the excitation processes of OH remain poorly characterized. We…

Quantum scattering calculations for strongly interacting molecular systems are computationally demanding due to the large number of molecular states coupled by the anisotropy of atom - molecule interactions. We demonstrate that thermal rate…

Chemical Physics · Physics 2026-01-06 Xuyang Guo , Kirk W. Madison , James L. Booth , Roman V. Krems

Rate coefficients for inelastic Na+H collisions are calculated for all transitions between the ten levels up to and including the ionic state (ion-pair production), namely Na(3s,3p,4s,3d,4p,5s,4d,4f,5p)+H(1s) and Na+ + H-. The calculations…

Solar and Stellar Astrophysics · Physics 2015-05-19 P. S. Barklem , A. K. Belyaev , A. S. Dickinson , F. X. Gadea

Different methods to extract the temperature and density in heavy ion collisions are compared using a statistical model tailored to reproduce many experimental features at low excitation energy. The model assumes a sequential decay of an…

Nuclear Theory · Physics 2014-11-04 H. Zheng , G. Bonasera , J. Mabiala , P. Marini , A. Bonasera

We discuss the formation of molecular oxygen in ultracold collisions between hydroxyl radicals and atomic oxygen. A time-independent quantum formalism based on hyperspherical coordinates is employed for the calculations. Elastic, inelastic…

Chemical Physics · Physics 2009-02-06 Goulven Quéméner , Naduvalath Balakrishnan , Brian K. Kendrick

Rate coefficients for collisional processes such as rotational and vibrational excitation are essential inputs in many astrophysical models. When rate coefficients are unknown, they are often estimated using known values from other systems.…

Astrophysics of Galaxies · Physics 2015-06-22 Kyle M. Walker , B. H. Yang , P. C. Stancil , N. Balakrishnan , R. C. Forrey

-We have performed a new efficient method to calculate numerically the transport coefficients at high temperature. The collision theory was treated to study singularities that occur when evaluating the collision cross section. The transport…

Plasma Physics · Physics 2015-01-30 Ali Mahfouf , Pascal André , Géraldine Faure

Aim: We present an improved database of temperature dependent rate coefficients for rotational state-to-state transitions in H$_{2}$O + H$_{2}$O collisions. The database includes 231 transitions between the lower $para$- and 210 transitions…

Chemical Physics · Physics 2023-10-19 Bikramaditya Mandal , Dmitri Babikov

We present analytical expressions for direct evaluation of $\ell$-mixing rate coefficients in proton-excited hydrogen atom collisions and describe a software package for efficient numerical evaluation of the collisional rate coefficients.…

Instrumentation and Methods for Astrophysics · Physics 2019-07-17 D. Vrinceanu , R. Onofrio , J. B. R. Oonk , P. Salas , H. R. Sadeghpour

We present calculated rate coefficients for ro-vibrational transitions of CO in collisions with H atoms for a gas temperature range of 10 K $\leq T \leq$ 3000 K, based on the recent three-dimensional ab initio H-CO interaction potential of…

Astrophysics of Galaxies · Physics 2015-11-23 L. Song , N. Balakrishnan , K. M. Walker , P. C. Stancil , W. F. Thi , I. Kamp , A. van der Avoird , G. C. Groenenboom

We present quantum dynamical calculations that describe the rotational excitation of H$_2$O due to collisions with H atoms. We used a recent, high accuracy potential energy surface, and solved the collisional dynamics with the…

Astrophysics of Galaxies · Physics 2015-06-23 F. Daniel , A. Faure , P. J. Dagdigian , M. -L. Dubernet , F. lique , G. Pineau des forêts

Experimental measurements and theoretical calculations of state-to-state rate coefficients for rotational energy transfer of CO in collision with H$_2$ are reported at the very low temperatures prevailing in dense interstellar clouds (5 -…

Carbon monoxide is a simple molecule present in many astrophysical environments, and collisional excitation rate coefficients due to the dominant collision partners are necessary to accurately predict spectral line intensities and extract…

Astrophysics of Galaxies · Physics 2015-11-17 Kyle M. Walker , L. Song , B. H. Yang , G. C. Groenenboom , A. van der Avoird , N. Balakrishnan , R. C. Forrey , P. C. Stancil

We have studied the fundamental rotational relaxation and excitation collision of OH- J=0 <-> 1 with helium at different collision energies. Using state-selected photodetachment in a cryogenic ion trap, the collisional excitation of the…

Excitation and charge transfer in low-energy O+H collisions is studied; it is a problem of importance for modelling stellar spectra and obtaining accurate oxygen abundances in late-type stars including the Sun. The collisions have been…

Solar and Stellar Astrophysics · Physics 2018-02-28 P. S. Barklem

Cold molecules are important for many applications, from fundamental precision measurements, quantum information processing, quantum-controlled chemistry, to understanding the cold interstellar medium. Molecular ions are known to be cooled…

The temperature dependence of the rate of the reaction CH_4+H \to CH_3+H_2 is studied using classical collision theory with a temperature-dependent effective potential derived from a path integral analysis. Analytical expressions are…

Chemical Physics · Physics 2016-09-08 David Z. Goodson , Dustin W. Roelse , Wan-Ting Chiang , Steven M. Valone , J. D. Doll

Modeling environments that are not in local thermal equilibrium, such as protoplanetary disks or planetary atmospheres, with molecular spectroscopic data from space telescopes requires knowledge of the rate coefficients of rovibrationally…

Atomic Physics · Physics 2023-10-10 Taha Selim , Ad van der Avoird , Gerrit C. Groenenboom
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