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Realistic charged macromolecules are characterized by discrete (rather than homogeneous) charge distributions. We investigate the effects of surface charge discretization on the counterion distribution at the level of mean-field theory…

Soft Condensed Matter · Physics 2007-05-23 Mark L. Henle , Christian D. Santangelo , Deena M. Patel , Philip A. Pincus

Counterion distributions at charged soft membranes are studied using perturbative analytical and simulation methods in both weak coupling (mean-field or Poisson-Boltzmann) and strong coupling limits. The softer the membrane, the more…

Biological Physics · Physics 2009-11-10 Christian Fleck , Roland Netz

We study a classical system of identically charged counter-ions near a planar wall carrying a uniform surface charge density. The equilibrium statistical mechanics of the system depends on a single dimensionless coupling parameter. A new…

Soft Condensed Matter · Physics 2019-01-21 I. Palaia , M. Trulsson , L. Samaj , E. Trizac

We consider counterions in the presence of a single planar surface with a spatially inhomogeneous charge distribution using Monte-Carlo simulations and strong-coupling theory. For high surface charges, multivalent counterions, or pronounced…

Soft Condensed Matter · Physics 2009-11-07 Andre G Moreira , Roland R Netz

Screening of a strongly charged macroion by multivalent counterions is considered. It is shown that counterions form a strongly correlated liquid at the surface of the macroion. Cohesive energy of this liquid leads to additional attraction…

Soft Condensed Matter · Physics 2009-10-31 B. I. Shklovskii

Screening of a strongly charged macroion by its multivalent counterions can not be described in the framework of mean field Poisson-Boltzmann (PB) theory because multivalent counterions form a strongly correlated liquid (SCL) on the surface…

Soft Condensed Matter · Physics 2010-04-27 M. S. Loth , B. I. Shklovskii

We report the coupled effects of macroion charge discretization and counterion valence in the primitive model for spherical colloids. Instead of considering a uniformly charged surface, as it is traditionally done, we consider a more…

Soft Condensed Matter · Physics 2009-11-07 Rene Messina

Poisson-Boltzmann theory is the cornerstone for soft matter electrostatics. We provide novel exact analytical solutions to this non-linear mean-field approach, for the diffuse layer of ions in the vicinity of a planar or a cylindrical…

Soft Condensed Matter · Physics 2020-01-29 L. Samaj , E. Trizac

The screening of plate-plate interactions by counterions is an age-old problem. We revisit this classic question when counterions exhibit a distribution of charges. While it is expected that the long-distance regime of interactions is…

Statistical Mechanics · Physics 2018-01-08 M. Trulsson , L. Samaj , E. Trizac

A model for ionic solutions with an attractive short-range pair interaction between the ions is presented. The short-range interaction is accounted for by adding a quadratic non-local term to the Poisson-Boltzmann free energy. The model is…

Soft Condensed Matter · Physics 2009-10-31 Yoram Burak , David Andelman

We present a model for the ion distribution near a charged surface, based on the response of the ions to the presence of a single test particle. Near an infinite planar surface this model produces the exact density profile in the limits of…

Soft Condensed Matter · Physics 2009-11-10 Y. Burak , D. Andelman , H. Orland

Using a generalization of the Poisson-Boltzmann equation, dynamics of counterion condensation is studied. For a single charged plate in the presence of counterions, it is shown that the approach to equilibrium is diffusive. In the far from…

Soft Condensed Matter · Physics 2009-10-31 Ramin Golestanian

We study discrete solvent effects on the interaction of two parallel charged surfaces in ionic aqueous solution. These effects are taken into account by adding a bilinear non-local term to the free energy of Poisson-Boltzmann theory. We…

Soft Condensed Matter · Physics 2009-10-31 Yoram Burak , David Andelman

We study nonlinear wave phenomena in self-gravitating fluid systems, with a particular emphasis on applications to molecular clouds. This paper presents analytical results for one spatial dimension. We show that a large class of physical…

Astrophysics · Physics 2009-10-22 Fred C. Adams , Marco Fatuzzo , Richard Watkins

An effective pair potential for systems of uniformly charged lamellar colloids in the presence of an electrolytic solution of microscopic co- and counterions is derived. The charge distribution on the discs is expressed as a collection of…

Soft Condensed Matter · Physics 2009-10-31 D. G. Rowan , J. -P. Hansen , E. Trizac

Screening of a macroion by multivalent counterions is considered. It is shown that ions form strongly correlated liquid at the macroion surface. Cohesive energy of this liquid leads to strong additional attraction of counterions to the…

Soft Condensed Matter · Physics 2009-10-31 V. I. Perel , B. I. Shklovskii

A theory is presented which allows us to accurately calculate the density profile of monovalent and multivalent counterions in suspensions of polarizable colloids or nano-particles. In the case of monovalent ions, we derive a weak-coupling…

Soft Condensed Matter · Physics 2011-09-23 Amin Bakhshandeh , Alexandre Pereira dos Santos , Yan Levin

We study the ionic distribution near a charged surface. A new method for performing Monte Carlo simulations in this geometry is discussed. A theory is then presented that allows us to accurately reproduce the density profiles obtained in…

Chemical Physics · Physics 2012-11-09 Alexandre P. dos Santos , Yan Levin

The distribution of counterions and the electrostatic interaction between two similarly charged dielectric slabs is studied in the strong coupling limit. Dielectric inhomogeneities and discreteness of charge on the slabs have been taken…

Biological Physics · Physics 2015-06-12 Weria Pezeshkian , Narges Nikoofard , Davood Norouzi , Farshid Mohammad-Rafiee , Hossein Fazli

We consider a set of identical mobile point-like charges (counter-ions) confined to a domain with curved hard walls carrying a uniform fixed surface charge density, the system as a whole being electroneutral. Three domain geometries are…

Soft Condensed Matter · Physics 2016-03-24 Ladislav Samaj , E. Trizac
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