Related papers: Voronoi Glass-Forming Liquids : A Structural Study
Glass formation is one of the most interesting phenomena in the condensed matter field. Considerable effort has gone into understanding and predicting the glass formability. However, the previous prediction requires the glass first made…
Glass forming liquids exhibit a rich phenomenology upon confinement. This is often related to the effects arising from wall-fluid interactions. Here we focus on the interesting limit where the separation of the confining walls becomes of…
This paper introduces a new approach toward characterizing local structural features of two-dimensional particle systems. The approach can accurately identify and characterize defects in high-temperature crystals, distinguish a wide range…
When liquids are cooled, their dynamics are slowed, and if crystallization is avoided, they will solidify into an amorphous structure referred to as a glass. Experiments show that chemically distinct glass-forming liquids have universal…
Using molecular dynamics simulations we study the slow dynamics of a hard sphere fluid confined in a disordered porous matrix. The presence of both discontinuous and continuous glass transitions as well as the complex interplay between…
We address the interesting temperature range of a glass forming system where the mechanical properties are intermediate between those of a liquid and a solid. We employ an efficient Monte-Carlo method to calculate the elastic moduli, and…
Contact of a fluid with a solid or an elastic wall is investigated. The wall exerts molecular forces on the fluid which is locally strongly nonhomogeneous. The problem is approached with a fluid energy of the second gradient form and a wall…
In this talk I present some of the recent theoretical results that have been obtained on glassy systems like spin glasses or structural glasses. The physical principles at the basis of the theory are explained in a simple language (without…
Building on the recently derived inhomogeneous mode-coupling theory, we extend the generalised mode-coupling theory of supercooled liquids to inhomogeneous environments. This provides a first-principles-based, systematic and rigorous way of…
A unified fluid-structure interaction (FSI) formulation is presented for solid, liquid and mixed membranes. Nonlinear finite elements (FE) and the generalized-alpha scheme are used for the spatial and temporal discretization. The membrane…
Soft materials such as colloidal suspensions, polymer solutions and liquid crystals are constituted by mesoscopic entities held together by weak forces. Their mechanical moduli are several orders of magnitude lower than those of atomic…
Minimization diagrams encompass a large class of diagrams of interest in the literature, such as generalized Voronoi diagrams. We develop an abstract perturbation theory and perform a sensitivity analysis for functions depending on sets…
In the present paper we discuss the properties of Voronoi polygons in several monatomic glass-forming systems and compare them with those of the Kob-Andersen mixture. We show that two mechanisms of glass formation are possible: smearing of…
An analysis of the dynamics is performed, of exactly solvable models for fragile and strong glasses, exploiting the partitioning of the free energy landscape in inherent structures. The results are compared with the exact solution of the…
In this paper we consider the linearized version of a system of partial differential equations arising from a fluid-structure interaction model. We prove the existence and the uniqueness of the solution under natural regularity assumptions.
The physics of glasses can be studied from many viewpoints, from material scientists interested in the development of new materials to statistical physicists inventing new theoretical tools to deal with disordered systems. In these lectures…
The theory developed in our previous papers is applied in this paper to investigate the dependence of slowing down of dynamics of glass-forming liquids on the attractive and repulsive parts of intermolecular interactions. Through an…
We propose a simple theory for the dynamics of model glass-forming fluids, which should be solvable using a mean-field-like approach. The theory is based on transparent physical assumptions, which can be tested in computer simulations. The…
We review a theoretical perspective of the dynamics of glass forming liquids and the glass transition. It is a perspective we have developed with our collaborators during this decade. It is based upon the structure of trajectory space. This…
Isomorph theory is one of the promising theories to understand the quasi-universal relationship between thermodynamic, dynamic and structural characteristics. Based on the hidden scale invariance of the inverse power law potentials, it…